Controlled transitions between metastable states of 2D magnetocapillary crystals
Abstract Magnetocapillary interactions between particles allow to self-assemble floating crystals along liquid interfaces. For a fixed number of particles, different states possessing different symmetrical features, known as metastable states, coexist. In this paper, we demonstrate how to trigger th...
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Nature Portfolio
2022-09-01
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Series: | Scientific Reports |
Online Access: | https://doi.org/10.1038/s41598-022-20035-8 |
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author | Ylona Collard Franco N. Piñan Basualdo Aude Bolopion Michaël Gauthier Pierre Lambert Nicolas Vandewalle |
author_facet | Ylona Collard Franco N. Piñan Basualdo Aude Bolopion Michaël Gauthier Pierre Lambert Nicolas Vandewalle |
author_sort | Ylona Collard |
collection | DOAJ |
description | Abstract Magnetocapillary interactions between particles allow to self-assemble floating crystals along liquid interfaces. For a fixed number of particles, different states possessing different symmetrical features, known as metastable states, coexist. In this paper, we demonstrate how to trigger the transition from one state to another, either by rearranging the crystal, or by controlling its growth. First, we show that externally controlled magnetic fields can squeeze the entire crystal to induce structural modifications, that upon relaxation can lead to a modified state. Second, we propose localized laser-induced thermocapillary flows that can be used to guide new particles towards an existing crystal in a desired direction, thus favoring a particular resulting state. The control of the formation of metastable states is a key ingredient to functionalize such assemblies, paving the way to self-assembled microrobots. |
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institution | Directory Open Access Journal |
issn | 2045-2322 |
language | English |
last_indexed | 2024-04-12T16:52:58Z |
publishDate | 2022-09-01 |
publisher | Nature Portfolio |
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series | Scientific Reports |
spelling | doaj.art-a40eb28d80bd44808ecc9c9add09503f2022-12-22T03:24:19ZengNature PortfolioScientific Reports2045-23222022-09-011211910.1038/s41598-022-20035-8Controlled transitions between metastable states of 2D magnetocapillary crystalsYlona Collard0Franco N. Piñan Basualdo1Aude Bolopion2Michaël Gauthier3Pierre Lambert4Nicolas Vandewalle5GRASP, Institute of Physics B5a, Université de LiègeTIPs, École Polytechnique de Bruxelles, Université Libre de BruxelleFEMTO-ST, CNRS, Université Bourgogne Franche-ComtéFEMTO-ST, CNRS, Université Bourgogne Franche-ComtéTIPs, École Polytechnique de Bruxelles, Université Libre de BruxelleGRASP, Institute of Physics B5a, Université de LiègeAbstract Magnetocapillary interactions between particles allow to self-assemble floating crystals along liquid interfaces. For a fixed number of particles, different states possessing different symmetrical features, known as metastable states, coexist. In this paper, we demonstrate how to trigger the transition from one state to another, either by rearranging the crystal, or by controlling its growth. First, we show that externally controlled magnetic fields can squeeze the entire crystal to induce structural modifications, that upon relaxation can lead to a modified state. Second, we propose localized laser-induced thermocapillary flows that can be used to guide new particles towards an existing crystal in a desired direction, thus favoring a particular resulting state. The control of the formation of metastable states is a key ingredient to functionalize such assemblies, paving the way to self-assembled microrobots.https://doi.org/10.1038/s41598-022-20035-8 |
spellingShingle | Ylona Collard Franco N. Piñan Basualdo Aude Bolopion Michaël Gauthier Pierre Lambert Nicolas Vandewalle Controlled transitions between metastable states of 2D magnetocapillary crystals Scientific Reports |
title | Controlled transitions between metastable states of 2D magnetocapillary crystals |
title_full | Controlled transitions between metastable states of 2D magnetocapillary crystals |
title_fullStr | Controlled transitions between metastable states of 2D magnetocapillary crystals |
title_full_unstemmed | Controlled transitions between metastable states of 2D magnetocapillary crystals |
title_short | Controlled transitions between metastable states of 2D magnetocapillary crystals |
title_sort | controlled transitions between metastable states of 2d magnetocapillary crystals |
url | https://doi.org/10.1038/s41598-022-20035-8 |
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