Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China

A Nationwide Nitrogen Deposition Monitoring Network (NNDMN) containing 43 monitoring sites was established in China to measure gaseous NH<sub>3</sub>, NO<sub>2</sub>, and HNO<sub>3</sub> and particulate NH<sub>4</sub><sup>+</sup> and NO<...

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Main Authors: W. Xu, X. S. Luo, Y. P. Pan, L. Zhang, A. H. Tang, J. L. Shen, Y. Zhang, K. H. Li, Q. H. Wu, D. W. Yang, Y. Y. Zhang, J. Xue, W. Q. Li, Q. Q. Li, L. Tang, S. H. Lu, T. Liang, Y. A. Tong, P. Liu, Q. Zhang, Z. Q. Xiong, X. J. Shi, L. H. Wu, W. Q. Shi, K. Tian, X. H. Zhong, K. Shi, Q. Y. Tang, L. J. Zhang, J. L. Huang, C. E. He, F. H. Kuang, B. Zhu, H. Liu, X. Jin, Y. J. Xin, X. K. Shi, E. Z. Du, A. J. Dore, S. Tang, J. L. Collett Jr., K. Goulding, Y. X. Sun, J. Ren, F. S. Zhang, X. J. Liu
Format: Article
Language:English
Published: Copernicus Publications 2015-11-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/15/12345/2015/acp-15-12345-2015.pdf
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author W. Xu
X. S. Luo
Y. P. Pan
L. Zhang
A. H. Tang
J. L. Shen
Y. Zhang
K. H. Li
Q. H. Wu
D. W. Yang
Y. Y. Zhang
J. Xue
W. Q. Li
Q. Q. Li
L. Tang
S. H. Lu
T. Liang
Y. A. Tong
P. Liu
Q. Zhang
Z. Q. Xiong
X. J. Shi
L. H. Wu
W. Q. Shi
K. Tian
X. H. Zhong
K. Shi
Q. Y. Tang
L. J. Zhang
J. L. Huang
C. E. He
F. H. Kuang
B. Zhu
H. Liu
X. Jin
Y. J. Xin
X. K. Shi
E. Z. Du
A. J. Dore
S. Tang
J. L. Collett Jr.
K. Goulding
Y. X. Sun
J. Ren
F. S. Zhang
X. J. Liu
author_facet W. Xu
X. S. Luo
Y. P. Pan
L. Zhang
A. H. Tang
J. L. Shen
Y. Zhang
K. H. Li
Q. H. Wu
D. W. Yang
Y. Y. Zhang
J. Xue
W. Q. Li
Q. Q. Li
L. Tang
S. H. Lu
T. Liang
Y. A. Tong
P. Liu
Q. Zhang
Z. Q. Xiong
X. J. Shi
L. H. Wu
W. Q. Shi
K. Tian
X. H. Zhong
K. Shi
Q. Y. Tang
L. J. Zhang
J. L. Huang
C. E. He
F. H. Kuang
B. Zhu
H. Liu
X. Jin
Y. J. Xin
X. K. Shi
E. Z. Du
A. J. Dore
S. Tang
J. L. Collett Jr.
K. Goulding
Y. X. Sun
J. Ren
F. S. Zhang
X. J. Liu
author_sort W. Xu
collection DOAJ
description A Nationwide Nitrogen Deposition Monitoring Network (NNDMN) containing 43 monitoring sites was established in China to measure gaseous NH<sub>3</sub>, NO<sub>2</sub>, and HNO<sub>3</sub> and particulate NH<sub>4</sub><sup>+</sup> and NO<sub>3</sub><sup>&minus;</sup> in air and/or precipitation from 2010 to 2014. Wet/bulk deposition fluxes of N<sub>r</sub> species were collected by precipitation gauge method and measured by continuous-flow analyzer; dry deposition fluxes were estimated using airborne concentration measurements and inferential models. Our observations reveal large spatial variations of atmospheric N<sub>r</sub> concentrations and dry and wet/bulk N<sub>r</sub> deposition. On a national basis, the annual average concentrations (1.3–47.0 μg N m<sup>&minus;3</sup>) and dry plus wet/bulk deposition fluxes (2.9–83.3 kg N ha<sup>−1</sup> yr<sup>&minus;1</sup>) of inorganic N<sub>r</sub> species are ranked by land use as urban > rural > background sites and by regions as north China > southeast China > southwest China > northeast China > northwest China > Tibetan Plateau, reflecting the impact of anthropogenic N<sub>r</sub> emission. Average dry and wet/bulk N deposition fluxes were 20.6 ± 11.2 (mean ± standard deviation) and 19.3 ± 9.2 kg N ha<sup>−1</sup> yr<sup>−1</sup> across China, with reduced N deposition dominating both dry and wet/bulk deposition. Our results suggest atmospheric dry N deposition is equally important to wet/bulk N deposition at the national scale. Therefore, both deposition forms should be included when considering the impacts of N deposition on environment and ecosystem health.
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spelling doaj.art-a555d8de79424cfcb4c8f9863f005a6d2022-12-22T03:45:12ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242015-11-011521123451236010.5194/acp-15-12345-2015Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across ChinaW. Xu0X. S. Luo1Y. P. Pan2L. Zhang3A. H. Tang4J. L. Shen5Y. Zhang6K. H. Li7Q. H. Wu8D. W. Yang9Y. Y. Zhang10J. Xue11W. Q. Li12Q. Q. Li13L. Tang14S. H. Lu15T. Liang16Y. A. Tong17P. Liu18Q. Zhang19Z. Q. Xiong20X. J. Shi21L. H. Wu22W. Q. Shi23K. Tian24X. H. Zhong25K. Shi26Q. Y. Tang27L. J. Zhang28J. L. Huang29C. E. He30F. H. Kuang31B. Zhu32H. Liu33X. Jin34Y. J. Xin35X. K. Shi36E. Z. Du37A. J. Dore38S. Tang39J. L. Collett Jr.40K. Goulding41Y. X. Sun42J. Ren43F. S. Zhang44X. J. Liu45College of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaCollege of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaState Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, ChinaLaboratory for Climate and Ocean-Atmosphere Studies, Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing 100871, ChinaCollege of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaInstitute of Subtropical Agriculture, Chinese Academy of Sciences, Changsha 4410125, ChinaCollege of Nature Conservation, Beijing Forestry University, Beijing 100083, ChinaXinjiang Institute of Ecology and Geography, Chinese Academy of Sciences, Urumqi 830011, ChinaCollege of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaCollege of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaCollege of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaCollege of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaFujian Institute of Tobacco Agricultural Sciences, Fuzhou 350003, ChinaCollege of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaCollege of Resources and Environmental Sciences, Yunnan Agricultural University, Kunming 650224, ChinaSoil and Fertilizer Institute, Sichuan Academy of Agricultural Sciences, Chengdu 610066, ChinaNature Resource and Environment College, Northwest A&F University, Yangling 712100, ChinaNature Resource and Environment College, Northwest A&F University, Yangling 712100, ChinaInstitute of Agricultural Environment and Resource, Shanxi Academy of Agricultural Sciences, Taiyuan 030031, ChinaInstitute of Agricultural Environment and Resource, Shanxi Academy of Agricultural Sciences, Taiyuan 030031, ChinaCollege of Resources and Environmental Sciences, Nanjing Agricultural University, Nanjing 210009, ChinaCollege of Resources and Environment, Southwest University, Chongqing 400716, ChinaCollege of Environmental and Resource Sciences, Zhejiang University, Hangzhou 310029, ChinaSouth Subtropical Crops Research Institute, Chinese Academy of Tropical Agricultural Science, Zhanjiang 524091, ChinaRice Research Institute, Guangdong Academy of Agricultural Sciences, Guangzhou 510640, ChinaRice Research Institute, Guangdong Academy of Agricultural Sciences, Guangzhou 510640, ChinaCollege of Environmental and Chemical Engineering, Dalian Jiaotong University, Dalian 116028, ChinaCollege of Agriculture, Hunan Agricultural University, Changsha 410128, ChinaCollege of Resources and Environment, Agricultural University of Hebei, Baoding 071001, ChinaCollege of Plant Science and Technology, Huazhong Agricultural University, Wuhan 430070, ChinaInstitute of Geographic Sciences and Natural Resources, Chinese Academy of Sciences, Beijing 100101, ChinaInstitute of Mountain, Hazards and Environment, Chinese Academy of Sciences, Chengdu 610041, ChinaInstitute of Mountain, Hazards and Environment, Chinese Academy of Sciences, Chengdu 610041, ChinaResearch Institute of Soil & Fertilizer and Agricultural Water Conservation, Xinjiang Academy of Agricultural Sciences, Urumqi 830091, ChinaThe Bureau of Qinghai Meteorology, Xining 810001, ChinaThe Bureau of Qinghai Meteorology, Xining 810001, ChinaAgriculture, Forestry and Water Department of Changdao County, Changdao 265800, ChinaState Key Laboratory of Earth Surface Processes and Resource Ecology, and College of Resources Science & Technology, Beijing Normal University, Beijing 100875, ChinaCentre for Ecology & Hydrology Edinburgh, Bush Estate, Penicuik, Midlothian EH26 0QB, UKCentre for Ecology & Hydrology Edinburgh, Bush Estate, Penicuik, Midlothian EH26 0QB, UKDepartment of Atmospheric Science, Colorado State University, Fort Collins, CO 80523, USAThe Sustainable Soils and Grassland Systems Department, Rothamsted Research, Harpenden AL5 2JQ, UKInstitute of Soil and Fertilizer, Anhui Academy of Agricultural Sciences, Hefei 230031, ChinaInstitute of Soil and Fertilizer, Jilin Academy of Agricultural Sciences, Changchun 130124, ChinaCollege of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaCollege of Resources and Environmental Sciences, China Agricultural University, Beijing 100193, ChinaA Nationwide Nitrogen Deposition Monitoring Network (NNDMN) containing 43 monitoring sites was established in China to measure gaseous NH<sub>3</sub>, NO<sub>2</sub>, and HNO<sub>3</sub> and particulate NH<sub>4</sub><sup>+</sup> and NO<sub>3</sub><sup>&minus;</sup> in air and/or precipitation from 2010 to 2014. Wet/bulk deposition fluxes of N<sub>r</sub> species were collected by precipitation gauge method and measured by continuous-flow analyzer; dry deposition fluxes were estimated using airborne concentration measurements and inferential models. Our observations reveal large spatial variations of atmospheric N<sub>r</sub> concentrations and dry and wet/bulk N<sub>r</sub> deposition. On a national basis, the annual average concentrations (1.3–47.0 μg N m<sup>&minus;3</sup>) and dry plus wet/bulk deposition fluxes (2.9–83.3 kg N ha<sup>−1</sup> yr<sup>&minus;1</sup>) of inorganic N<sub>r</sub> species are ranked by land use as urban > rural > background sites and by regions as north China > southeast China > southwest China > northeast China > northwest China > Tibetan Plateau, reflecting the impact of anthropogenic N<sub>r</sub> emission. Average dry and wet/bulk N deposition fluxes were 20.6 ± 11.2 (mean ± standard deviation) and 19.3 ± 9.2 kg N ha<sup>−1</sup> yr<sup>−1</sup> across China, with reduced N deposition dominating both dry and wet/bulk deposition. Our results suggest atmospheric dry N deposition is equally important to wet/bulk N deposition at the national scale. Therefore, both deposition forms should be included when considering the impacts of N deposition on environment and ecosystem health.http://www.atmos-chem-phys.net/15/12345/2015/acp-15-12345-2015.pdf
spellingShingle W. Xu
X. S. Luo
Y. P. Pan
L. Zhang
A. H. Tang
J. L. Shen
Y. Zhang
K. H. Li
Q. H. Wu
D. W. Yang
Y. Y. Zhang
J. Xue
W. Q. Li
Q. Q. Li
L. Tang
S. H. Lu
T. Liang
Y. A. Tong
P. Liu
Q. Zhang
Z. Q. Xiong
X. J. Shi
L. H. Wu
W. Q. Shi
K. Tian
X. H. Zhong
K. Shi
Q. Y. Tang
L. J. Zhang
J. L. Huang
C. E. He
F. H. Kuang
B. Zhu
H. Liu
X. Jin
Y. J. Xin
X. K. Shi
E. Z. Du
A. J. Dore
S. Tang
J. L. Collett Jr.
K. Goulding
Y. X. Sun
J. Ren
F. S. Zhang
X. J. Liu
Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China
Atmospheric Chemistry and Physics
title Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China
title_full Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China
title_fullStr Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China
title_full_unstemmed Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China
title_short Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China
title_sort quantifying atmospheric nitrogen deposition through a nationwide monitoring network across china
url http://www.atmos-chem-phys.net/15/12345/2015/acp-15-12345-2015.pdf
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