Carbon balance of China constrained by CONTRAIL aircraft CO<sub>2</sub> measurements

Terrestrial carbon dioxide (CO<sub>2</sub>) flux estimates in China using atmospheric inversion method are beset with considerable uncertainties because very few atmospheric CO<sub>2</sub> concentration measurements are available. In order to improve these estimates, nested a...

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Main Authors: F. Jiang, H. M. Wang, J. M. Chen, T. Machida, L. X. Zhou, W. M. Ju, H. Matsueda, Y. Sawa
Format: Article
Language:English
Published: Copernicus Publications 2014-09-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/14/10133/2014/acp-14-10133-2014.pdf
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author F. Jiang
H. M. Wang
J. M. Chen
T. Machida
L. X. Zhou
W. M. Ju
H. Matsueda
Y. Sawa
author_facet F. Jiang
H. M. Wang
J. M. Chen
T. Machida
L. X. Zhou
W. M. Ju
H. Matsueda
Y. Sawa
author_sort F. Jiang
collection DOAJ
description Terrestrial carbon dioxide (CO<sub>2</sub>) flux estimates in China using atmospheric inversion method are beset with considerable uncertainties because very few atmospheric CO<sub>2</sub> concentration measurements are available. In order to improve these estimates, nested atmospheric CO<sub>2</sub> inversion during 2002–2008 is performed in this study using passenger aircraft-based CO<sub>2</sub> measurements over Eurasia from the Comprehensive Observation Network for Trace gases by Airliner (CONTRAIL) project. The inversion system includes 43 regions with a focus on China, and is based on the Bayesian synthesis approach and the TM5 transport model. The terrestrial ecosystem carbon flux modeled by the Boreal Ecosystems Productivity Simulator (BEPS) model and the ocean exchange simulated by the OPA-PISCES-T model are considered as the prior fluxes. The impacts of CONTRAIL CO<sub>2</sub> data on inverted China terrestrial carbon fluxes are quantified, the improvement of the inverted fluxes after adding CONTRAIL CO<sub>2</sub> data are rationed against climate factors and evaluated by comparing the simulated atmospheric CO<sub>2</sub> concentrations with three independent surface CO<sub>2</sub> measurements in China. Results show that with the addition of CONTRAIL CO<sub>2</sub> data, the inverted carbon sink in China increases while those in South and Southeast Asia decrease. Meanwhile, the posterior uncertainties over these regions are all reduced (2–12%). CONTRAIL CO<sub>2</sub> data also have a large effect on the inter-annual variation of carbon sinks in China, leading to a better correlation between the carbon sink and the annual mean climate factors. Evaluations against the CO<sub>2</sub> measurements at three sites in China also show that the CONTRAIL CO<sub>2</sub> measurements may have improved the inversion results.
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spelling doaj.art-a68e7660ad654c058fef6cb892f1e4062022-12-22T00:14:58ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242014-09-011418101331014410.5194/acp-14-10133-2014Carbon balance of China constrained by CONTRAIL aircraft CO<sub>2</sub> measurementsF. Jiang0H. M. Wang1J. M. Chen2T. Machida3L. X. Zhou4W. M. Ju5H. Matsueda6Y. Sawa7Jiangsu Provincial Key Laboratory of Geographic Information Science and Technology, Nanjing University, Nanjing, ChinaJiangsu Provincial Key Laboratory of Geographic Information Science and Technology, Nanjing University, Nanjing, ChinaJiangsu Provincial Key Laboratory of Geographic Information Science and Technology, Nanjing University, Nanjing, ChinaNational Institute for Environmental Studies, Tsukuba, JapanChinese Academy of Meteorological Sciences, China Meteorological Administration, Beijing, ChinaJiangsu Provincial Key Laboratory of Geographic Information Science and Technology, Nanjing University, Nanjing, ChinaGeochemical Research Department, Meteorological Research Institute, Tsukuba, JapanGeochemical Research Department, Meteorological Research Institute, Tsukuba, JapanTerrestrial carbon dioxide (CO<sub>2</sub>) flux estimates in China using atmospheric inversion method are beset with considerable uncertainties because very few atmospheric CO<sub>2</sub> concentration measurements are available. In order to improve these estimates, nested atmospheric CO<sub>2</sub> inversion during 2002–2008 is performed in this study using passenger aircraft-based CO<sub>2</sub> measurements over Eurasia from the Comprehensive Observation Network for Trace gases by Airliner (CONTRAIL) project. The inversion system includes 43 regions with a focus on China, and is based on the Bayesian synthesis approach and the TM5 transport model. The terrestrial ecosystem carbon flux modeled by the Boreal Ecosystems Productivity Simulator (BEPS) model and the ocean exchange simulated by the OPA-PISCES-T model are considered as the prior fluxes. The impacts of CONTRAIL CO<sub>2</sub> data on inverted China terrestrial carbon fluxes are quantified, the improvement of the inverted fluxes after adding CONTRAIL CO<sub>2</sub> data are rationed against climate factors and evaluated by comparing the simulated atmospheric CO<sub>2</sub> concentrations with three independent surface CO<sub>2</sub> measurements in China. Results show that with the addition of CONTRAIL CO<sub>2</sub> data, the inverted carbon sink in China increases while those in South and Southeast Asia decrease. Meanwhile, the posterior uncertainties over these regions are all reduced (2–12%). CONTRAIL CO<sub>2</sub> data also have a large effect on the inter-annual variation of carbon sinks in China, leading to a better correlation between the carbon sink and the annual mean climate factors. Evaluations against the CO<sub>2</sub> measurements at three sites in China also show that the CONTRAIL CO<sub>2</sub> measurements may have improved the inversion results.http://www.atmos-chem-phys.net/14/10133/2014/acp-14-10133-2014.pdf
spellingShingle F. Jiang
H. M. Wang
J. M. Chen
T. Machida
L. X. Zhou
W. M. Ju
H. Matsueda
Y. Sawa
Carbon balance of China constrained by CONTRAIL aircraft CO<sub>2</sub> measurements
Atmospheric Chemistry and Physics
title Carbon balance of China constrained by CONTRAIL aircraft CO<sub>2</sub> measurements
title_full Carbon balance of China constrained by CONTRAIL aircraft CO<sub>2</sub> measurements
title_fullStr Carbon balance of China constrained by CONTRAIL aircraft CO<sub>2</sub> measurements
title_full_unstemmed Carbon balance of China constrained by CONTRAIL aircraft CO<sub>2</sub> measurements
title_short Carbon balance of China constrained by CONTRAIL aircraft CO<sub>2</sub> measurements
title_sort carbon balance of china constrained by contrail aircraft co sub 2 sub measurements
url http://www.atmos-chem-phys.net/14/10133/2014/acp-14-10133-2014.pdf
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