Investigation of Nonlinear Optical Processes in Mercury Sulfide Quantum Dots
The authors report the third-harmonic generation, nonlinear refraction, and nonlinear absorption in HgS quantum dot (QD) suspensions and films using the nanosecond and femtosecond pulses. High conversion efficiency (7 × 10<sup>−4</sup>) towards the third harmonic (TH) of the 900–1700 nm,...
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MDPI AG
2022-04-01
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author | Vyacheslav V. Kim Ivan A. Shuklov Alaa A. Mardini Arturs Bundulis Andrey I. Zvyagin Rawda Kholany Anna A. Lizunova Jurgis Grube Anatolijs Sarakovskis Oleg V. Ovchinnikov Rashid A. Ganeev |
author_facet | Vyacheslav V. Kim Ivan A. Shuklov Alaa A. Mardini Arturs Bundulis Andrey I. Zvyagin Rawda Kholany Anna A. Lizunova Jurgis Grube Anatolijs Sarakovskis Oleg V. Ovchinnikov Rashid A. Ganeev |
author_sort | Vyacheslav V. Kim |
collection | DOAJ |
description | The authors report the third-harmonic generation, nonlinear refraction, and nonlinear absorption in HgS quantum dot (QD) suspensions and films using the nanosecond and femtosecond pulses. High conversion efficiency (7 × 10<sup>−4</sup>) towards the third harmonic (TH) of the 900–1700 nm, 150 fs laser in the thin (70 nm) films containing HgS QDs deposited on the glass substrates is obtained. The authors analyze spectral dependencies of the TH, nonlinear refractive indices, and nonlinear absorption coefficients of QDs in the 500–1700 nm range and discuss the relation between the TH process and the low-order nonlinear optical properties of these quantum dots. |
first_indexed | 2024-03-09T13:13:29Z |
format | Article |
id | doaj.art-a892247143e84f478ca4fa49e5efdbc4 |
institution | Directory Open Access Journal |
issn | 2079-4991 |
language | English |
last_indexed | 2024-03-09T13:13:29Z |
publishDate | 2022-04-01 |
publisher | MDPI AG |
record_format | Article |
series | Nanomaterials |
spelling | doaj.art-a892247143e84f478ca4fa49e5efdbc42023-11-30T21:39:14ZengMDPI AGNanomaterials2079-49912022-04-01128126410.3390/nano12081264Investigation of Nonlinear Optical Processes in Mercury Sulfide Quantum DotsVyacheslav V. Kim0Ivan A. Shuklov1Alaa A. Mardini2Arturs Bundulis3Andrey I. Zvyagin4Rawda Kholany5Anna A. Lizunova6Jurgis Grube7Anatolijs Sarakovskis8Oleg V. Ovchinnikov9Rashid A. Ganeev10Laboratory of Nonlinear Optics, University of Latvia, Jelgavas 3, LV-1004 Riga, LatviaMoscow Institute of Physics and Technology, National Research University, 141701 Dolgoprudny, RussiaMoscow Institute of Physics and Technology, National Research University, 141701 Dolgoprudny, RussiaInstitute of Solid State Physics, University of Latvia, Kengaraga 8, LV-1063 Riga, LatviaDepartment of Physics, Voronezh State University, 394006 Voronezh, RussiaMoscow Institute of Physics and Technology, National Research University, 141701 Dolgoprudny, RussiaMoscow Institute of Physics and Technology, National Research University, 141701 Dolgoprudny, RussiaInstitute of Solid State Physics, University of Latvia, Kengaraga 8, LV-1063 Riga, LatviaInstitute of Solid State Physics, University of Latvia, Kengaraga 8, LV-1063 Riga, LatviaDepartment of Physics, Voronezh State University, 394006 Voronezh, RussiaLaboratory of Nonlinear Optics, University of Latvia, Jelgavas 3, LV-1004 Riga, LatviaThe authors report the third-harmonic generation, nonlinear refraction, and nonlinear absorption in HgS quantum dot (QD) suspensions and films using the nanosecond and femtosecond pulses. High conversion efficiency (7 × 10<sup>−4</sup>) towards the third harmonic (TH) of the 900–1700 nm, 150 fs laser in the thin (70 nm) films containing HgS QDs deposited on the glass substrates is obtained. The authors analyze spectral dependencies of the TH, nonlinear refractive indices, and nonlinear absorption coefficients of QDs in the 500–1700 nm range and discuss the relation between the TH process and the low-order nonlinear optical properties of these quantum dots.https://www.mdpi.com/2079-4991/12/8/1264quantum dotsmercury sulfidethird-harmonic generationnonlinear refractionnonlinear absorption |
spellingShingle | Vyacheslav V. Kim Ivan A. Shuklov Alaa A. Mardini Arturs Bundulis Andrey I. Zvyagin Rawda Kholany Anna A. Lizunova Jurgis Grube Anatolijs Sarakovskis Oleg V. Ovchinnikov Rashid A. Ganeev Investigation of Nonlinear Optical Processes in Mercury Sulfide Quantum Dots Nanomaterials quantum dots mercury sulfide third-harmonic generation nonlinear refraction nonlinear absorption |
title | Investigation of Nonlinear Optical Processes in Mercury Sulfide Quantum Dots |
title_full | Investigation of Nonlinear Optical Processes in Mercury Sulfide Quantum Dots |
title_fullStr | Investigation of Nonlinear Optical Processes in Mercury Sulfide Quantum Dots |
title_full_unstemmed | Investigation of Nonlinear Optical Processes in Mercury Sulfide Quantum Dots |
title_short | Investigation of Nonlinear Optical Processes in Mercury Sulfide Quantum Dots |
title_sort | investigation of nonlinear optical processes in mercury sulfide quantum dots |
topic | quantum dots mercury sulfide third-harmonic generation nonlinear refraction nonlinear absorption |
url | https://www.mdpi.com/2079-4991/12/8/1264 |
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