Simulation and Experimental Study of Ion Concentration Polarization Induced Electroconvective Vortex and Particle Movement

Ion concentration polarization (ICP) has been widely applied in microfluidic systems in pre-concentration, particle separation, and desalination applications. General ICP microfluidic systems have three components (i.e., source, ion-exchange, and buffer), which allow selective ion transport. Recentl...

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Main Authors: Junghyo Yoon, Youngkyu Cho, Jaehoon Kim, Hyunho Kim, Kyuhwan Na, Jeong Hoon Lee, Seok Chung
Format: Article
Language:English
Published: MDPI AG 2021-07-01
Series:Micromachines
Subjects:
Online Access:https://www.mdpi.com/2072-666X/12/8/903
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author Junghyo Yoon
Youngkyu Cho
Jaehoon Kim
Hyunho Kim
Kyuhwan Na
Jeong Hoon Lee
Seok Chung
author_facet Junghyo Yoon
Youngkyu Cho
Jaehoon Kim
Hyunho Kim
Kyuhwan Na
Jeong Hoon Lee
Seok Chung
author_sort Junghyo Yoon
collection DOAJ
description Ion concentration polarization (ICP) has been widely applied in microfluidic systems in pre-concentration, particle separation, and desalination applications. General ICP microfluidic systems have three components (i.e., source, ion-exchange, and buffer), which allow selective ion transport. Recently developed trials to eliminate one of the three components to simplify the system have suffered from decreased performance by the accumulation of unwanted ions. In this paper, we presented a new ICP microfluidic system with only an ion-exchange membrane-coated channel. Numerical investigation on hydrodynamic flow and electric fields with a series of coupled governing equations enabled a strong correlation to experimental investigations on electroconvective vortices and the trajectory of charged particles. This study has significant implications for the development and optimization of ICP microfluidic and electrochemical systems for biomarker concentration and separation to improve sensing reliability and detection limits in analytic chemistry.
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spelling doaj.art-a90118c22485468083686a53e04516e52023-11-22T08:43:48ZengMDPI AGMicromachines2072-666X2021-07-0112890310.3390/mi12080903Simulation and Experimental Study of Ion Concentration Polarization Induced Electroconvective Vortex and Particle MovementJunghyo Yoon0Youngkyu Cho1Jaehoon Kim2Hyunho Kim3Kyuhwan Na4Jeong Hoon Lee5Seok Chung6School of Mechanical Engineering, Korea University, 145 Anam-ro, Seoungbuk-gu, Seoul 02841, KoreaDepartment of IT Convergence, Korea University, 145 Anam-ro, Seoungbuk-gu, Seoul 02841, KoreaSchool of Mechanical Engineering, Korea University, 145 Anam-ro, Seoungbuk-gu, Seoul 02841, KoreaSchool of Mechanical Engineering, Korea University, 145 Anam-ro, Seoungbuk-gu, Seoul 02841, KoreaSchool of Mechanical Engineering, Korea University, 145 Anam-ro, Seoungbuk-gu, Seoul 02841, KoreaDepartment of Electrical Engineering, Kwangwoon University, 20 Kwangwoon-ro, Nowon-gu, Seoul 01897, KoreaSchool of Mechanical Engineering, Korea University, 145 Anam-ro, Seoungbuk-gu, Seoul 02841, KoreaIon concentration polarization (ICP) has been widely applied in microfluidic systems in pre-concentration, particle separation, and desalination applications. General ICP microfluidic systems have three components (i.e., source, ion-exchange, and buffer), which allow selective ion transport. Recently developed trials to eliminate one of the three components to simplify the system have suffered from decreased performance by the accumulation of unwanted ions. In this paper, we presented a new ICP microfluidic system with only an ion-exchange membrane-coated channel. Numerical investigation on hydrodynamic flow and electric fields with a series of coupled governing equations enabled a strong correlation to experimental investigations on electroconvective vortices and the trajectory of charged particles. This study has significant implications for the development and optimization of ICP microfluidic and electrochemical systems for biomarker concentration and separation to improve sensing reliability and detection limits in analytic chemistry.https://www.mdpi.com/2072-666X/12/8/903ion concentration polarizationelectroconvective vortexmanipulationion-permselective material
spellingShingle Junghyo Yoon
Youngkyu Cho
Jaehoon Kim
Hyunho Kim
Kyuhwan Na
Jeong Hoon Lee
Seok Chung
Simulation and Experimental Study of Ion Concentration Polarization Induced Electroconvective Vortex and Particle Movement
Micromachines
ion concentration polarization
electroconvective vortex
manipulation
ion-permselective material
title Simulation and Experimental Study of Ion Concentration Polarization Induced Electroconvective Vortex and Particle Movement
title_full Simulation and Experimental Study of Ion Concentration Polarization Induced Electroconvective Vortex and Particle Movement
title_fullStr Simulation and Experimental Study of Ion Concentration Polarization Induced Electroconvective Vortex and Particle Movement
title_full_unstemmed Simulation and Experimental Study of Ion Concentration Polarization Induced Electroconvective Vortex and Particle Movement
title_short Simulation and Experimental Study of Ion Concentration Polarization Induced Electroconvective Vortex and Particle Movement
title_sort simulation and experimental study of ion concentration polarization induced electroconvective vortex and particle movement
topic ion concentration polarization
electroconvective vortex
manipulation
ion-permselective material
url https://www.mdpi.com/2072-666X/12/8/903
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