The thermo-mechanical recyclability potential of biodegradable biopolyesters: Perspectives and limits for food packaging application

Up to now, recycling has been opposed to biodegradability, although these two end-of-life options are complementary. If combined in an integrated system, recycling creates an after-use economy, while biodegradability eradicates definitely the issues of environmental spreading of the persistent plast...

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Main Authors: Isabelle Dedieu, Stéphane Peyron, Nathalie Gontard, Chahinez Aouf
Format: Article
Language:English
Published: Elsevier 2022-07-01
Series:Polymer Testing
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S0142941822001453
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author Isabelle Dedieu
Stéphane Peyron
Nathalie Gontard
Chahinez Aouf
author_facet Isabelle Dedieu
Stéphane Peyron
Nathalie Gontard
Chahinez Aouf
author_sort Isabelle Dedieu
collection DOAJ
description Up to now, recycling has been opposed to biodegradability, although these two end-of-life options are complementary. If combined in an integrated system, recycling creates an after-use economy, while biodegradability eradicates definitely the issues of environmental spreading of the persistent plastic wastes. This paper reviews the current state on recyclability of some promising biodegradable polyesters, polylactide acid (PLA), polyhydroxyalkanoates (PHAs), bio-polybutylene succinate (PBS) and polybutylene adipate terephthalate (PBAT), with emphasis on mechanical recycling. The effect of the mechanical reprocessing (multiple extrusion or injection-molding) on the chemical structure and thermomechanical properties of the polymers is reported. In addition, the application of upgrading strategies such as blends and/or composites to improve polyesters recyclability are considered. A further decontamination step is studied in order to achieve food contact aptitude in mechanical recycling for food packaging application. Finally, the challenges that should be faced in the future, to promote the recyclability of biodegradable polyesters are addressed.
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spelling doaj.art-ac3f5a3294794d93ae78d48d85f4c8e02022-12-22T03:26:57ZengElsevierPolymer Testing0142-94182022-07-01111107620The thermo-mechanical recyclability potential of biodegradable biopolyesters: Perspectives and limits for food packaging applicationIsabelle Dedieu0Stéphane Peyron1Nathalie Gontard2Chahinez Aouf3UMR 1208 IATE, INRAE Montpellier, 2 place Pierre Viala, 34060, Montpellier, France; Corresponding author.UMR 1208 IATE, Univ Montpellier, 2 place Pierre Viala, 34060, Montpellier, France; Corresponding author.UMR 1208 IATE, INRAE Montpellier, 2 place Pierre Viala, 34060, Montpellier, FranceUMR 1208 IATE, INRAE Montpellier, 2 place Pierre Viala, 34060, Montpellier, France; Corresponding author. 2 Place Pierre viala, 34060, Montpelluer, France.Up to now, recycling has been opposed to biodegradability, although these two end-of-life options are complementary. If combined in an integrated system, recycling creates an after-use economy, while biodegradability eradicates definitely the issues of environmental spreading of the persistent plastic wastes. This paper reviews the current state on recyclability of some promising biodegradable polyesters, polylactide acid (PLA), polyhydroxyalkanoates (PHAs), bio-polybutylene succinate (PBS) and polybutylene adipate terephthalate (PBAT), with emphasis on mechanical recycling. The effect of the mechanical reprocessing (multiple extrusion or injection-molding) on the chemical structure and thermomechanical properties of the polymers is reported. In addition, the application of upgrading strategies such as blends and/or composites to improve polyesters recyclability are considered. A further decontamination step is studied in order to achieve food contact aptitude in mechanical recycling for food packaging application. Finally, the challenges that should be faced in the future, to promote the recyclability of biodegradable polyesters are addressed.http://www.sciencedirect.com/science/article/pii/S0142941822001453Mechanical recyclingBiodegradable biopolyestersDegradation mechanismsThermomechanical propertiesFood packaging
spellingShingle Isabelle Dedieu
Stéphane Peyron
Nathalie Gontard
Chahinez Aouf
The thermo-mechanical recyclability potential of biodegradable biopolyesters: Perspectives and limits for food packaging application
Polymer Testing
Mechanical recycling
Biodegradable biopolyesters
Degradation mechanisms
Thermomechanical properties
Food packaging
title The thermo-mechanical recyclability potential of biodegradable biopolyesters: Perspectives and limits for food packaging application
title_full The thermo-mechanical recyclability potential of biodegradable biopolyesters: Perspectives and limits for food packaging application
title_fullStr The thermo-mechanical recyclability potential of biodegradable biopolyesters: Perspectives and limits for food packaging application
title_full_unstemmed The thermo-mechanical recyclability potential of biodegradable biopolyesters: Perspectives and limits for food packaging application
title_short The thermo-mechanical recyclability potential of biodegradable biopolyesters: Perspectives and limits for food packaging application
title_sort thermo mechanical recyclability potential of biodegradable biopolyesters perspectives and limits for food packaging application
topic Mechanical recycling
Biodegradable biopolyesters
Degradation mechanisms
Thermomechanical properties
Food packaging
url http://www.sciencedirect.com/science/article/pii/S0142941822001453
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