Femtosecond Pulse Laser Near-Field Ablation of Ag Nanorods

Ag nanorods (Ag NRs) with a mean aspect ratio of 3.9 were prepared through a wet-chemical method, and the absorption spectra for various aspect ratios were obtained. The morphology transformation of Ag NRs irradiated with a femtosecond pulse laser was investigated through transmission electron micro...

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Main Authors: Dezhi Zhu, Jianfeng Yan
Format: Article
Language:English
Published: MDPI AG 2019-01-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/9/3/363
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author Dezhi Zhu
Jianfeng Yan
author_facet Dezhi Zhu
Jianfeng Yan
author_sort Dezhi Zhu
collection DOAJ
description Ag nanorods (Ag NRs) with a mean aspect ratio of 3.9 were prepared through a wet-chemical method, and the absorption spectra for various aspect ratios were obtained. The morphology transformation of Ag NRs irradiated with a femtosecond pulse laser was investigated through transmission electron microscopy (TEM). The near-field ablation was dependent on the laser polarization and wavelength. Laser-induced high electric field intensity was observed at the ends, middle, and junctions of the Ag NRs under various ablation conditions. Through simulation, the evolution mechanism was analyzed in detail. The effect of laser polarization angle on plasmonic junction welding was also investigated. By controlling the electronic field distribution, several nanostructures were obtained: bone-shaped NRs, T-shaped NRs, dimers, trimers, curved NRs, and nanodots. This study suggests a potentially useful approach for the reshaping, cutting, and welding of nanostructures.
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spelling doaj.art-ac5a3a5efced4c79a93bbc927a45b4a02022-12-21T18:51:48ZengMDPI AGApplied Sciences2076-34172019-01-019336310.3390/app9030363app9030363Femtosecond Pulse Laser Near-Field Ablation of Ag NanorodsDezhi Zhu0Jianfeng Yan1Department of Mechanical Engineering, Tsinghua University, Beijing 100084, ChinaDepartment of Mechanical Engineering, Tsinghua University, Beijing 100084, ChinaAg nanorods (Ag NRs) with a mean aspect ratio of 3.9 were prepared through a wet-chemical method, and the absorption spectra for various aspect ratios were obtained. The morphology transformation of Ag NRs irradiated with a femtosecond pulse laser was investigated through transmission electron microscopy (TEM). The near-field ablation was dependent on the laser polarization and wavelength. Laser-induced high electric field intensity was observed at the ends, middle, and junctions of the Ag NRs under various ablation conditions. Through simulation, the evolution mechanism was analyzed in detail. The effect of laser polarization angle on plasmonic junction welding was also investigated. By controlling the electronic field distribution, several nanostructures were obtained: bone-shaped NRs, T-shaped NRs, dimers, trimers, curved NRs, and nanodots. This study suggests a potentially useful approach for the reshaping, cutting, and welding of nanostructures.https://www.mdpi.com/2076-3417/9/3/363Ag nanorodsfemtosecond pulse lasernear-field ablationpolarization
spellingShingle Dezhi Zhu
Jianfeng Yan
Femtosecond Pulse Laser Near-Field Ablation of Ag Nanorods
Applied Sciences
Ag nanorods
femtosecond pulse laser
near-field ablation
polarization
title Femtosecond Pulse Laser Near-Field Ablation of Ag Nanorods
title_full Femtosecond Pulse Laser Near-Field Ablation of Ag Nanorods
title_fullStr Femtosecond Pulse Laser Near-Field Ablation of Ag Nanorods
title_full_unstemmed Femtosecond Pulse Laser Near-Field Ablation of Ag Nanorods
title_short Femtosecond Pulse Laser Near-Field Ablation of Ag Nanorods
title_sort femtosecond pulse laser near field ablation of ag nanorods
topic Ag nanorods
femtosecond pulse laser
near-field ablation
polarization
url https://www.mdpi.com/2076-3417/9/3/363
work_keys_str_mv AT dezhizhu femtosecondpulselasernearfieldablationofagnanorods
AT jianfengyan femtosecondpulselasernearfieldablationofagnanorods