Witnessing entangled two-photon absorption via quantum interferometry

Recent investigations have suggested that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of entangled two-photon absorption (eTPA), there is still a h...

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Bibliographic Details
Main Authors: Áulide Martínez-Tapia, Samuel Corona-Aquino, Freiman Triana-Arango, Chenglong You, Rui-Bo Jin, Omar S. Magaña-Loaiza, Shi-Hai Dong, Alfred B. U’Ren, Roberto de J. León-Montiel
Format: Article
Language:English
Published: AIP Publishing LLC 2023-03-01
Series:APL Photonics
Online Access:http://dx.doi.org/10.1063/5.0128249
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Summary:Recent investigations have suggested that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of entangled two-photon absorption (eTPA), there is still a heated debate on whether eTPA has truly been observed. This interesting debate has arisen mainly because it has recently been argued that single-photon-loss mechanisms, such as scattering or hot-band absorption, may mimic the expected entangled-photon linear absorption behavior. In this work, we focus on transmission measurements of eTPA and explore three different two-photon quantum interferometers in the context of assessing eTPA. We demonstrate that the so-called N00N-state configuration is the only one among those considered insensitive to linear (single-photon) losses. Remarkably, our results show that N00N states may become a potentially powerful tool for quantum spectroscopy, placing them as a strong candidate for the certification of eTPA in an arbitrary sample.
ISSN:2378-0967