Improvement of low-temperature damping performance by the control of three-dimensional network structure formed by renewable oil in modified waterborne polyurethane

Waterborne polyurethane (WPUs) were synthesized with polytetramethylene ether glycol (PTMG), isophorone diisocyanate (IPDI) as the primary raw material, castor oil (CO) and dimethylolpropionic acid (DMPA) as the crosslinker and hydrophilic chain-extender, respectively. Three-dimensional networks wer...

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Main Authors: Jiuhang Shan, Long Jiang, Linhui Wang, He Zhao, Xiaodan Ding, Chao Zhou
Format: Article
Language:English
Published: Elsevier 2021-06-01
Series:Results in Materials
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2590048X21000042
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author Jiuhang Shan
Long Jiang
Linhui Wang
He Zhao
Xiaodan Ding
Chao Zhou
author_facet Jiuhang Shan
Long Jiang
Linhui Wang
He Zhao
Xiaodan Ding
Chao Zhou
author_sort Jiuhang Shan
collection DOAJ
description Waterborne polyurethane (WPUs) were synthesized with polytetramethylene ether glycol (PTMG), isophorone diisocyanate (IPDI) as the primary raw material, castor oil (CO) and dimethylolpropionic acid (DMPA) as the crosslinker and hydrophilic chain-extender, respectively. Three-dimensional networks were constructed in the molecular chain of the polymer by the introduction of castor oil. With the increase of CO contents, the WPUs prepared with more flexible segments and more points of intersection supporting the three-dimensional structure provided by castor oil have films with weak resistance to water, better elasticity, lower effective damping temperature, and better thermal resistance. Different homogeneity of the network structure was obtained, it was found that with the gradual unification of the structure, the tensile properties of the film were improved by about 25%, and the lowest effective damping temperature moved to −43.25 ​°C. The WPU films could be used as a material for low-temperature damping applications.
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spelling doaj.art-ad60e0a4b4144644ae7ce375dd1cf9c52022-12-22T04:03:47ZengElsevierResults in Materials2590-048X2021-06-0110100171Improvement of low-temperature damping performance by the control of three-dimensional network structure formed by renewable oil in modified waterborne polyurethaneJiuhang Shan0Long Jiang1Linhui Wang2He Zhao3Xiaodan Ding4Chao Zhou5Changchun University of Technology, Changchun, Jilin Province, PR ChinaChangchun University of Technology, Changchun, Jilin Province, PR ChinaChangchun University of Technology, Changchun, Jilin Province, PR ChinaChangchun University of Technology, Changchun, Jilin Province, PR ChinaChangchun University of Technology, Changchun, Jilin Province, PR ChinaCorresponding author.; Changchun University of Technology, Changchun, Jilin Province, PR ChinaWaterborne polyurethane (WPUs) were synthesized with polytetramethylene ether glycol (PTMG), isophorone diisocyanate (IPDI) as the primary raw material, castor oil (CO) and dimethylolpropionic acid (DMPA) as the crosslinker and hydrophilic chain-extender, respectively. Three-dimensional networks were constructed in the molecular chain of the polymer by the introduction of castor oil. With the increase of CO contents, the WPUs prepared with more flexible segments and more points of intersection supporting the three-dimensional structure provided by castor oil have films with weak resistance to water, better elasticity, lower effective damping temperature, and better thermal resistance. Different homogeneity of the network structure was obtained, it was found that with the gradual unification of the structure, the tensile properties of the film were improved by about 25%, and the lowest effective damping temperature moved to −43.25 ​°C. The WPU films could be used as a material for low-temperature damping applications.http://www.sciencedirect.com/science/article/pii/S2590048X21000042Waterborne polyurethaneCastor oil3D cross-linked networkLow temperature damping coating
spellingShingle Jiuhang Shan
Long Jiang
Linhui Wang
He Zhao
Xiaodan Ding
Chao Zhou
Improvement of low-temperature damping performance by the control of three-dimensional network structure formed by renewable oil in modified waterborne polyurethane
Results in Materials
Waterborne polyurethane
Castor oil
3D cross-linked network
Low temperature damping coating
title Improvement of low-temperature damping performance by the control of three-dimensional network structure formed by renewable oil in modified waterborne polyurethane
title_full Improvement of low-temperature damping performance by the control of three-dimensional network structure formed by renewable oil in modified waterborne polyurethane
title_fullStr Improvement of low-temperature damping performance by the control of three-dimensional network structure formed by renewable oil in modified waterborne polyurethane
title_full_unstemmed Improvement of low-temperature damping performance by the control of three-dimensional network structure formed by renewable oil in modified waterborne polyurethane
title_short Improvement of low-temperature damping performance by the control of three-dimensional network structure formed by renewable oil in modified waterborne polyurethane
title_sort improvement of low temperature damping performance by the control of three dimensional network structure formed by renewable oil in modified waterborne polyurethane
topic Waterborne polyurethane
Castor oil
3D cross-linked network
Low temperature damping coating
url http://www.sciencedirect.com/science/article/pii/S2590048X21000042
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AT longjiang improvementoflowtemperaturedampingperformancebythecontrolofthreedimensionalnetworkstructureformedbyrenewableoilinmodifiedwaterbornepolyurethane
AT linhuiwang improvementoflowtemperaturedampingperformancebythecontrolofthreedimensionalnetworkstructureformedbyrenewableoilinmodifiedwaterbornepolyurethane
AT hezhao improvementoflowtemperaturedampingperformancebythecontrolofthreedimensionalnetworkstructureformedbyrenewableoilinmodifiedwaterbornepolyurethane
AT xiaodanding improvementoflowtemperaturedampingperformancebythecontrolofthreedimensionalnetworkstructureformedbyrenewableoilinmodifiedwaterbornepolyurethane
AT chaozhou improvementoflowtemperaturedampingperformancebythecontrolofthreedimensionalnetworkstructureformedbyrenewableoilinmodifiedwaterbornepolyurethane