Modeling of Laboratory Steam Methane Reforming and CO<sub>2</sub> Methanation Reactors
To support the interpretation of the experimental results obtained from two laboratory-scale reactors, one working in the steam methane reforming (SMR) mode, and the other in the CO<sub>2</sub> hydrogenation (MCO2) mode, a steady-state pseudo-homogeneous 1D non-isothermal packed-bed reac...
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2020-05-01
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Online Access: | https://www.mdpi.com/1996-1073/13/10/2624 |
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author | Paola Costamagna Federico Pugliese Tullio Cavattoni Guido Busca Gabriella Garbarino |
author_facet | Paola Costamagna Federico Pugliese Tullio Cavattoni Guido Busca Gabriella Garbarino |
author_sort | Paola Costamagna |
collection | DOAJ |
description | To support the interpretation of the experimental results obtained from two laboratory-scale reactors, one working in the steam methane reforming (SMR) mode, and the other in the CO<sub>2</sub> hydrogenation (MCO2) mode, a steady-state pseudo-homogeneous 1D non-isothermal packed-bed reactor model is developed, embedding the classical Xu and Froment local kinetics. The laboratory reactors are operated with three different catalysts, two commercial and one homemade. The simulation model makes it possible to identify and account for thermal effects occurring inside the catalytic zone of the reactor and along the exit line. The model is intended to guide the development of small size SMR and MCO2 reactors in the context of Power-to-X (P2X) studies. |
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format | Article |
id | doaj.art-ae86d20983f54a64a030fd33fcdd1758 |
institution | Directory Open Access Journal |
issn | 1996-1073 |
language | English |
last_indexed | 2024-03-10T19:40:00Z |
publishDate | 2020-05-01 |
publisher | MDPI AG |
record_format | Article |
series | Energies |
spelling | doaj.art-ae86d20983f54a64a030fd33fcdd17582023-11-20T01:20:37ZengMDPI AGEnergies1996-10732020-05-011310262410.3390/en13102624Modeling of Laboratory Steam Methane Reforming and CO<sub>2</sub> Methanation ReactorsPaola Costamagna0Federico Pugliese1Tullio Cavattoni2Guido Busca3Gabriella Garbarino4Department of Chemistry and Industrial Chemistry, University of Genova, via Dodecaneso 31, I-16146 Genova, ItalyDepartment of Civil, Chemical and Environmental Engineering, Chemical Engineering Pole, University of Genova, via Opera Pia 15, I-16145 Genova, ItalyINSTM, UdR Genova, via Dodecaneso 31, I-16146 Genova, ItalyDepartment of Civil, Chemical and Environmental Engineering, Chemical Engineering Pole, University of Genova, via Opera Pia 15, I-16145 Genova, ItalyDepartment of Civil, Chemical and Environmental Engineering, Chemical Engineering Pole, University of Genova, via Opera Pia 15, I-16145 Genova, ItalyTo support the interpretation of the experimental results obtained from two laboratory-scale reactors, one working in the steam methane reforming (SMR) mode, and the other in the CO<sub>2</sub> hydrogenation (MCO2) mode, a steady-state pseudo-homogeneous 1D non-isothermal packed-bed reactor model is developed, embedding the classical Xu and Froment local kinetics. The laboratory reactors are operated with three different catalysts, two commercial and one homemade. The simulation model makes it possible to identify and account for thermal effects occurring inside the catalytic zone of the reactor and along the exit line. The model is intended to guide the development of small size SMR and MCO2 reactors in the context of Power-to-X (P2X) studies.https://www.mdpi.com/1996-1073/13/10/2624chemical reactor modelingCO<sub>2</sub> methanationhydrogenNi-based catalystsPower-to-Xsteam methane reforming |
spellingShingle | Paola Costamagna Federico Pugliese Tullio Cavattoni Guido Busca Gabriella Garbarino Modeling of Laboratory Steam Methane Reforming and CO<sub>2</sub> Methanation Reactors Energies chemical reactor modeling CO<sub>2</sub> methanation hydrogen Ni-based catalysts Power-to-X steam methane reforming |
title | Modeling of Laboratory Steam Methane Reforming and CO<sub>2</sub> Methanation Reactors |
title_full | Modeling of Laboratory Steam Methane Reforming and CO<sub>2</sub> Methanation Reactors |
title_fullStr | Modeling of Laboratory Steam Methane Reforming and CO<sub>2</sub> Methanation Reactors |
title_full_unstemmed | Modeling of Laboratory Steam Methane Reforming and CO<sub>2</sub> Methanation Reactors |
title_short | Modeling of Laboratory Steam Methane Reforming and CO<sub>2</sub> Methanation Reactors |
title_sort | modeling of laboratory steam methane reforming and co sub 2 sub methanation reactors |
topic | chemical reactor modeling CO<sub>2</sub> methanation hydrogen Ni-based catalysts Power-to-X steam methane reforming |
url | https://www.mdpi.com/1996-1073/13/10/2624 |
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