Optimization of N_{2}^{+} lasing through population depletion in the X^{2}Σ_{g}^{+} state using elliptically modulated ultrashort intense laser fields

We generate unidirectional coherent radiations at 391 and 428 nm corresponding to the B^{2}Σ_{u}^{+}-X^{2}Σ_{g}^{+} (0,0) and (0,1) emission of N_{2}^{+} by irradiating neutral N_{2} with an elliptically modulated near-IR ultrashort laser field generated using a quarter-wave plate (QWP) with the dif...

Full description

Bibliographic Details
Main Authors: Yao Fu, Erik Lötstedt, Helong Li, Siqi Wang, Danwen Yao, Toshiaki Ando, Atsushi Iwasaki, Farhad H. M. Faisal, Kaoru Yamanouchi, Huailiang Xu
Format: Article
Language:English
Published: American Physical Society 2020-01-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.2.012007
_version_ 1797211622865895424
author Yao Fu
Erik Lötstedt
Helong Li
Siqi Wang
Danwen Yao
Toshiaki Ando
Atsushi Iwasaki
Farhad H. M. Faisal
Kaoru Yamanouchi
Huailiang Xu
author_facet Yao Fu
Erik Lötstedt
Helong Li
Siqi Wang
Danwen Yao
Toshiaki Ando
Atsushi Iwasaki
Farhad H. M. Faisal
Kaoru Yamanouchi
Huailiang Xu
author_sort Yao Fu
collection DOAJ
description We generate unidirectional coherent radiations at 391 and 428 nm corresponding to the B^{2}Σ_{u}^{+}-X^{2}Σ_{g}^{+} (0,0) and (0,1) emission of N_{2}^{+} by irradiating neutral N_{2} with an elliptically modulated near-IR ultrashort laser field generated using a quarter-wave plate (QWP) with the different orders, and reveal that the lasing intensity at 391 nm becomes maximum at a specific orientation of the fast axis of QWP with respect to the polarization direction of the input laser field. We reproduce this observation by numerical calculations and show that the lasing intensity can be optimized by adjusting the temporal separation between the two polarization components of the elliptically modulated laser pulse and their relative amplitudes so that the inverted population between the B^{2}Σ_{u}^{+} and X^{2}Σ_{g}^{+} states can be achieved efficiently and the population in the X^{2}Σ_{g}^{+}(v^{″}=0) level is further depleted in the latter part of the laser pulse by the A^{2}Π_{u}-X^{2}Σ_{g}^{+} transition.
first_indexed 2024-04-24T10:29:25Z
format Article
id doaj.art-aee76215315042fe80cb0324b0173779
institution Directory Open Access Journal
issn 2643-1564
language English
last_indexed 2024-04-24T10:29:25Z
publishDate 2020-01-01
publisher American Physical Society
record_format Article
series Physical Review Research
spelling doaj.art-aee76215315042fe80cb0324b01737792024-04-12T16:48:32ZengAmerican Physical SocietyPhysical Review Research2643-15642020-01-012101200710.1103/PhysRevResearch.2.012007Optimization of N_{2}^{+} lasing through population depletion in the X^{2}Σ_{g}^{+} state using elliptically modulated ultrashort intense laser fieldsYao FuErik LötstedtHelong LiSiqi WangDanwen YaoToshiaki AndoAtsushi IwasakiFarhad H. M. FaisalKaoru YamanouchiHuailiang XuWe generate unidirectional coherent radiations at 391 and 428 nm corresponding to the B^{2}Σ_{u}^{+}-X^{2}Σ_{g}^{+} (0,0) and (0,1) emission of N_{2}^{+} by irradiating neutral N_{2} with an elliptically modulated near-IR ultrashort laser field generated using a quarter-wave plate (QWP) with the different orders, and reveal that the lasing intensity at 391 nm becomes maximum at a specific orientation of the fast axis of QWP with respect to the polarization direction of the input laser field. We reproduce this observation by numerical calculations and show that the lasing intensity can be optimized by adjusting the temporal separation between the two polarization components of the elliptically modulated laser pulse and their relative amplitudes so that the inverted population between the B^{2}Σ_{u}^{+} and X^{2}Σ_{g}^{+} states can be achieved efficiently and the population in the X^{2}Σ_{g}^{+}(v^{″}=0) level is further depleted in the latter part of the laser pulse by the A^{2}Π_{u}-X^{2}Σ_{g}^{+} transition.http://doi.org/10.1103/PhysRevResearch.2.012007
spellingShingle Yao Fu
Erik Lötstedt
Helong Li
Siqi Wang
Danwen Yao
Toshiaki Ando
Atsushi Iwasaki
Farhad H. M. Faisal
Kaoru Yamanouchi
Huailiang Xu
Optimization of N_{2}^{+} lasing through population depletion in the X^{2}Σ_{g}^{+} state using elliptically modulated ultrashort intense laser fields
Physical Review Research
title Optimization of N_{2}^{+} lasing through population depletion in the X^{2}Σ_{g}^{+} state using elliptically modulated ultrashort intense laser fields
title_full Optimization of N_{2}^{+} lasing through population depletion in the X^{2}Σ_{g}^{+} state using elliptically modulated ultrashort intense laser fields
title_fullStr Optimization of N_{2}^{+} lasing through population depletion in the X^{2}Σ_{g}^{+} state using elliptically modulated ultrashort intense laser fields
title_full_unstemmed Optimization of N_{2}^{+} lasing through population depletion in the X^{2}Σ_{g}^{+} state using elliptically modulated ultrashort intense laser fields
title_short Optimization of N_{2}^{+} lasing through population depletion in the X^{2}Σ_{g}^{+} state using elliptically modulated ultrashort intense laser fields
title_sort optimization of n 2 lasing through population depletion in the x 2 σ g state using elliptically modulated ultrashort intense laser fields
url http://doi.org/10.1103/PhysRevResearch.2.012007
work_keys_str_mv AT yaofu optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields
AT eriklotstedt optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields
AT helongli optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields
AT siqiwang optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields
AT danwenyao optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields
AT toshiakiando optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields
AT atsushiiwasaki optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields
AT farhadhmfaisal optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields
AT kaoruyamanouchi optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields
AT huailiangxu optimizationofn2lasingthroughpopulationdepletioninthex2sgstateusingellipticallymodulatedultrashortintenselaserfields