Mechanically Robust and Flexible GO/PI Hybrid Aerogels as Highly Efficient Oil Absorbents

Herein, mechanically robust and flexible graphene oxide/polyimide (GO/PI) hybrid aerogels (GIAs) were fabricated by a facile method, in which the mixed suspensions of the water-soluble polyimide precursor and graphene oxide (GO) sheets were freeze-dried, which was followed by a routine thermal imida...

Full description

Bibliographic Details
Main Authors: Li Zhang, Yuting Wang, Ruidong Wang, Penggang Yin, Juntao Wu
Format: Article
Language:English
Published: MDPI AG 2022-11-01
Series:Polymers
Subjects:
Online Access:https://www.mdpi.com/2073-4360/14/22/4903
_version_ 1797464174077411328
author Li Zhang
Yuting Wang
Ruidong Wang
Penggang Yin
Juntao Wu
author_facet Li Zhang
Yuting Wang
Ruidong Wang
Penggang Yin
Juntao Wu
author_sort Li Zhang
collection DOAJ
description Herein, mechanically robust and flexible graphene oxide/polyimide (GO/PI) hybrid aerogels (GIAs) were fabricated by a facile method, in which the mixed suspensions of the water-soluble polyimide precursor and graphene oxide (GO) sheets were freeze-dried, which was followed by a routine thermal imidation process. The porous GIAs obtained not only exhibit excellent elasticity and extremely low density values (from 33.3 to 38.9 mg.cm<sup>−3</sup>), but they also possess a superior compressive strength (121.7 KPa). The GIAs could support a weight of up to 31,250 times of its own weight, and such a weight-carrying capacity is much higher than that of other typical carbon-based aerogels. Having such a porous structure, and high strength and toughness properties make GIAs ideal candidates for oil spill cleanup materials. The oil/organic solvents’ absorption capacity ranges from 14.6 to 85, which is higher than that of most other aerogels (sponges). With their broad temperature tolerance and acidic stability, the unique multifunctional GIAs are expected to further extend their application range into extreme environments.
first_indexed 2024-03-09T18:03:15Z
format Article
id doaj.art-af509c49a09344668670762d574934d9
institution Directory Open Access Journal
issn 2073-4360
language English
last_indexed 2024-03-09T18:03:15Z
publishDate 2022-11-01
publisher MDPI AG
record_format Article
series Polymers
spelling doaj.art-af509c49a09344668670762d574934d92023-11-24T09:42:53ZengMDPI AGPolymers2073-43602022-11-011422490310.3390/polym14224903Mechanically Robust and Flexible GO/PI Hybrid Aerogels as Highly Efficient Oil AbsorbentsLi Zhang0Yuting Wang1Ruidong Wang2Penggang Yin3Juntao Wu4Key Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, ChinaKey Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, ChinaKey Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, ChinaKey Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, ChinaKey Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, ChinaHerein, mechanically robust and flexible graphene oxide/polyimide (GO/PI) hybrid aerogels (GIAs) were fabricated by a facile method, in which the mixed suspensions of the water-soluble polyimide precursor and graphene oxide (GO) sheets were freeze-dried, which was followed by a routine thermal imidation process. The porous GIAs obtained not only exhibit excellent elasticity and extremely low density values (from 33.3 to 38.9 mg.cm<sup>−3</sup>), but they also possess a superior compressive strength (121.7 KPa). The GIAs could support a weight of up to 31,250 times of its own weight, and such a weight-carrying capacity is much higher than that of other typical carbon-based aerogels. Having such a porous structure, and high strength and toughness properties make GIAs ideal candidates for oil spill cleanup materials. The oil/organic solvents’ absorption capacity ranges from 14.6 to 85, which is higher than that of most other aerogels (sponges). With their broad temperature tolerance and acidic stability, the unique multifunctional GIAs are expected to further extend their application range into extreme environments.https://www.mdpi.com/2073-4360/14/22/4903GIAscompressive strengthabsorption capacity
spellingShingle Li Zhang
Yuting Wang
Ruidong Wang
Penggang Yin
Juntao Wu
Mechanically Robust and Flexible GO/PI Hybrid Aerogels as Highly Efficient Oil Absorbents
Polymers
GIAs
compressive strength
absorption capacity
title Mechanically Robust and Flexible GO/PI Hybrid Aerogels as Highly Efficient Oil Absorbents
title_full Mechanically Robust and Flexible GO/PI Hybrid Aerogels as Highly Efficient Oil Absorbents
title_fullStr Mechanically Robust and Flexible GO/PI Hybrid Aerogels as Highly Efficient Oil Absorbents
title_full_unstemmed Mechanically Robust and Flexible GO/PI Hybrid Aerogels as Highly Efficient Oil Absorbents
title_short Mechanically Robust and Flexible GO/PI Hybrid Aerogels as Highly Efficient Oil Absorbents
title_sort mechanically robust and flexible go pi hybrid aerogels as highly efficient oil absorbents
topic GIAs
compressive strength
absorption capacity
url https://www.mdpi.com/2073-4360/14/22/4903
work_keys_str_mv AT lizhang mechanicallyrobustandflexiblegopihybridaerogelsashighlyefficientoilabsorbents
AT yutingwang mechanicallyrobustandflexiblegopihybridaerogelsashighlyefficientoilabsorbents
AT ruidongwang mechanicallyrobustandflexiblegopihybridaerogelsashighlyefficientoilabsorbents
AT penggangyin mechanicallyrobustandflexiblegopihybridaerogelsashighlyefficientoilabsorbents
AT juntaowu mechanicallyrobustandflexiblegopihybridaerogelsashighlyefficientoilabsorbents