Thermal-healing of lattice defects for high-energy single-crystalline battery cathodes

The lattice strain and defects in layered oxides is critical to the intercalation chemistry and battery performance. Here, the authors demonstrate a thermal-healing of lattice defects in single-crystalline cathodes caused by the thermal-induced release of lattice strain and the structure ordering.

Bibliographic Details
Main Authors: Shaofeng Li, Guannan Qian, Xiaomei He, Xiaojing Huang, Sang-Jun Lee, Zhisen Jiang, Yang Yang, Wei-Na Wang, Dechao Meng, Chang Yu, Jun-Sik Lee, Yong S. Chu, Zi-Feng Ma, Piero Pianetta, Jieshan Qiu, Linsen Li, Kejie Zhao, Yijin Liu
Format: Article
Language:English
Published: Nature Portfolio 2022-02-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-022-28325-5
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author Shaofeng Li
Guannan Qian
Xiaomei He
Xiaojing Huang
Sang-Jun Lee
Zhisen Jiang
Yang Yang
Wei-Na Wang
Dechao Meng
Chang Yu
Jun-Sik Lee
Yong S. Chu
Zi-Feng Ma
Piero Pianetta
Jieshan Qiu
Linsen Li
Kejie Zhao
Yijin Liu
author_facet Shaofeng Li
Guannan Qian
Xiaomei He
Xiaojing Huang
Sang-Jun Lee
Zhisen Jiang
Yang Yang
Wei-Na Wang
Dechao Meng
Chang Yu
Jun-Sik Lee
Yong S. Chu
Zi-Feng Ma
Piero Pianetta
Jieshan Qiu
Linsen Li
Kejie Zhao
Yijin Liu
author_sort Shaofeng Li
collection DOAJ
description The lattice strain and defects in layered oxides is critical to the intercalation chemistry and battery performance. Here, the authors demonstrate a thermal-healing of lattice defects in single-crystalline cathodes caused by the thermal-induced release of lattice strain and the structure ordering.
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spelling doaj.art-afca7adc5df044dca43cebe2db1213812022-12-22T04:10:56ZengNature PortfolioNature Communications2041-17232022-02-0113111010.1038/s41467-022-28325-5Thermal-healing of lattice defects for high-energy single-crystalline battery cathodesShaofeng Li0Guannan Qian1Xiaomei He2Xiaojing Huang3Sang-Jun Lee4Zhisen Jiang5Yang Yang6Wei-Na Wang7Dechao Meng8Chang Yu9Jun-Sik Lee10Yong S. Chu11Zi-Feng Ma12Piero Pianetta13Jieshan Qiu14Linsen Li15Kejie Zhao16Yijin Liu17Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratoryStanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratorySchool of Mechanical Engineering, Purdue UniversityNational Synchrotron Light Source II, Brookhaven National LaboratoryStanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratoryStanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratoryNational Synchrotron Light Source II, Brookhaven National LaboratoryDepartment of Chemical Engineering, School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, Shanghai Jiao Tong UniversityDepartment of Chemical Engineering, School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, Shanghai Jiao Tong UniversityState Key Lab of Fine Chemicals, School of Chemical Engineering, Liaoning Key Lab for Energy Materials and Chemical Engineering, Dalian University of TechnologyStanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratoryNational Synchrotron Light Source II, Brookhaven National LaboratoryDepartment of Chemical Engineering, School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, Shanghai Jiao Tong UniversityStanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratoryState Key Lab of Fine Chemicals, School of Chemical Engineering, Liaoning Key Lab for Energy Materials and Chemical Engineering, Dalian University of TechnologyDepartment of Chemical Engineering, School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, Shanghai Jiao Tong UniversitySchool of Mechanical Engineering, Purdue UniversityStanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratoryThe lattice strain and defects in layered oxides is critical to the intercalation chemistry and battery performance. Here, the authors demonstrate a thermal-healing of lattice defects in single-crystalline cathodes caused by the thermal-induced release of lattice strain and the structure ordering.https://doi.org/10.1038/s41467-022-28325-5
spellingShingle Shaofeng Li
Guannan Qian
Xiaomei He
Xiaojing Huang
Sang-Jun Lee
Zhisen Jiang
Yang Yang
Wei-Na Wang
Dechao Meng
Chang Yu
Jun-Sik Lee
Yong S. Chu
Zi-Feng Ma
Piero Pianetta
Jieshan Qiu
Linsen Li
Kejie Zhao
Yijin Liu
Thermal-healing of lattice defects for high-energy single-crystalline battery cathodes
Nature Communications
title Thermal-healing of lattice defects for high-energy single-crystalline battery cathodes
title_full Thermal-healing of lattice defects for high-energy single-crystalline battery cathodes
title_fullStr Thermal-healing of lattice defects for high-energy single-crystalline battery cathodes
title_full_unstemmed Thermal-healing of lattice defects for high-energy single-crystalline battery cathodes
title_short Thermal-healing of lattice defects for high-energy single-crystalline battery cathodes
title_sort thermal healing of lattice defects for high energy single crystalline battery cathodes
url https://doi.org/10.1038/s41467-022-28325-5
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