A proposed numerical method for absolute efficiency calibration of α-spectrometers and its application for activity calculation

In this work, an absolute method to calibrate an α-spectrometer is proposed taking into account the Source-to-Detector, and lateral distances due to eccentric source distribution. An analytical formula to calibrate an α-spectrometer is derived and the Simpson's integration method was utilized t...

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Main Authors: K.M. El-Kourghly, W. El-Gammal, Mohamed M. Damoom, Abdulsalam M. Alhawsawi, M. Abdelati, H.I. Khedr, R. Abouzaid
Format: Article
Language:English
Published: Elsevier 2024-04-01
Series:Heliyon
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2405844024045298
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author K.M. El-Kourghly
W. El-Gammal
Mohamed M. Damoom
Abdulsalam M. Alhawsawi
M. Abdelati
H.I. Khedr
R. Abouzaid
author_facet K.M. El-Kourghly
W. El-Gammal
Mohamed M. Damoom
Abdulsalam M. Alhawsawi
M. Abdelati
H.I. Khedr
R. Abouzaid
author_sort K.M. El-Kourghly
collection DOAJ
description In this work, an absolute method to calibrate an α-spectrometer is proposed taking into account the Source-to-Detector, and lateral distances due to eccentric source distribution. An analytical formula to calibrate an α-spectrometer is derived and the Simpson's integration method was utilized to solve these equations in its integral form numerically using a written C computer code. The general Monte Carlo N-particle code, MCNP as well as experimental measurements for some standard α-emitters are used to benchmark the proposed method. An agreement was found between the efficiency results calculated by MC and the proposed method with a maximum relative difference of about 0.5%. While, experimental measurement of α-emitters activity employing the proposed method differs by about 1.65% from the certified values. Accounting for the man made error allows to accurately quantify the assayed sample. Therefore, the inaccuracy in the efficiency results due to non-accurate inputs pertained to the source, and detector radii, Source–Detector distances, and eccentric source distribution are investigated in the Source-to-Detector distance range of (4 to 44 mm). The results show that a difference of ±1% in the detector radius, and Source-to-Detector distance than the normal values yields a relative difference of about ±2%, while a difference of ±50% in the source radius or source lateral distance from detector symmetry axis could only yields inaccuracy of less than ±3% in the efficiency results.
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spelling doaj.art-aff0327b60354c47962997b3fcbe1d6a2024-03-29T05:50:41ZengElsevierHeliyon2405-84402024-04-01107e28498A proposed numerical method for absolute efficiency calibration of α-spectrometers and its application for activity calculationK.M. El-Kourghly0W. El-Gammal1Mohamed M. Damoom2Abdulsalam M. Alhawsawi3M. Abdelati4H.I. Khedr5R. Abouzaid6Nuclear Safeguards and Physical Protection Department, Egyptian Atomic Energy Authority (EAEA), Cairo, Egypt; Corresponding author.Nuclear Safeguards and Physical Protection Department, Egyptian Atomic Energy Authority (EAEA), Cairo, EgyptNuclear Engineering Department, King Abdulaziz University, Jeddah, 21589, Saudi Arabia; Center for Training & Radiation Protection, King Abdulaziz University, Jeddah, 21589, Saudi Arabia; Corresponding author.Nuclear Engineering Department, King Abdulaziz University, Jeddah, 21589, Saudi Arabia; Center for Training & Radiation Protection, King Abdulaziz University, Jeddah, 21589, Saudi ArabiaNuclear Safeguards and Physical Protection Department, Egyptian Atomic Energy Authority (EAEA), Cairo, EgyptNuclear Safeguards and Physical Protection Department, Egyptian Atomic Energy Authority (EAEA), Cairo, EgyptFuel Cycle Safety Department, Egyptian Atomic Energy Authority (EAEA), Cairo, EgyptIn this work, an absolute method to calibrate an α-spectrometer is proposed taking into account the Source-to-Detector, and lateral distances due to eccentric source distribution. An analytical formula to calibrate an α-spectrometer is derived and the Simpson's integration method was utilized to solve these equations in its integral form numerically using a written C computer code. The general Monte Carlo N-particle code, MCNP as well as experimental measurements for some standard α-emitters are used to benchmark the proposed method. An agreement was found between the efficiency results calculated by MC and the proposed method with a maximum relative difference of about 0.5%. While, experimental measurement of α-emitters activity employing the proposed method differs by about 1.65% from the certified values. Accounting for the man made error allows to accurately quantify the assayed sample. Therefore, the inaccuracy in the efficiency results due to non-accurate inputs pertained to the source, and detector radii, Source–Detector distances, and eccentric source distribution are investigated in the Source-to-Detector distance range of (4 to 44 mm). The results show that a difference of ±1% in the detector radius, and Source-to-Detector distance than the normal values yields a relative difference of about ±2%, while a difference of ±50% in the source radius or source lateral distance from detector symmetry axis could only yields inaccuracy of less than ±3% in the efficiency results.http://www.sciencedirect.com/science/article/pii/S2405844024045298Alpha spectrometersAbsolute methodAnalytical-numericalMCNPSolid angle
spellingShingle K.M. El-Kourghly
W. El-Gammal
Mohamed M. Damoom
Abdulsalam M. Alhawsawi
M. Abdelati
H.I. Khedr
R. Abouzaid
A proposed numerical method for absolute efficiency calibration of α-spectrometers and its application for activity calculation
Heliyon
Alpha spectrometers
Absolute method
Analytical-numerical
MCNP
Solid angle
title A proposed numerical method for absolute efficiency calibration of α-spectrometers and its application for activity calculation
title_full A proposed numerical method for absolute efficiency calibration of α-spectrometers and its application for activity calculation
title_fullStr A proposed numerical method for absolute efficiency calibration of α-spectrometers and its application for activity calculation
title_full_unstemmed A proposed numerical method for absolute efficiency calibration of α-spectrometers and its application for activity calculation
title_short A proposed numerical method for absolute efficiency calibration of α-spectrometers and its application for activity calculation
title_sort proposed numerical method for absolute efficiency calibration of α spectrometers and its application for activity calculation
topic Alpha spectrometers
Absolute method
Analytical-numerical
MCNP
Solid angle
url http://www.sciencedirect.com/science/article/pii/S2405844024045298
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