Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics

We present detuning-dependent spectral and decay-rate measurements to study the difference between the spectral and dynamical properties of single quantum dots embedded in micropillar and photonic crystal cavities. For the micropillar cavity, the dynamics is well described by the dissipative Jaynes–...

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Main Authors: K H Madsen, P Lodahl
Format: Article
Language:English
Published: IOP Publishing 2013-01-01
Series:New Journal of Physics
Online Access:https://doi.org/10.1088/1367-2630/15/2/025013
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author K H Madsen
P Lodahl
author_facet K H Madsen
P Lodahl
author_sort K H Madsen
collection DOAJ
description We present detuning-dependent spectral and decay-rate measurements to study the difference between the spectral and dynamical properties of single quantum dots embedded in micropillar and photonic crystal cavities. For the micropillar cavity, the dynamics is well described by the dissipative Jaynes–Cummings model, whereas systematic deviations are observed for the emission spectra. The discrepancy for the spectra is attributed to the coupling of other exciton lines to the cavity and interference of different propagation paths toward the detector of the fields emitted by the quantum dot. In contrast, quantitative information about the system can readily be extracted from the dynamical measurements. In the case of photonic crystal cavities, we observe an anti-crossing in the spectra when detuning a single quantum dot through resonance, which is the spectral signature of a strong coupling. However, time-resolved measurements reveal that the actual coupling strength is significantly smaller than anticipated from the spectral measurements and that the quantum dot is rather weakly coupled to the cavity. We suggest that the observed Rabi splitting is due to cavity feeding by other quantum dots and/or multi-exciton complexes giving rise to collective emission effects.
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spelling doaj.art-b03034f5f412408b8beb704ab9221ff72023-08-08T11:06:00ZengIOP PublishingNew Journal of Physics1367-26302013-01-0115202501310.1088/1367-2630/15/2/025013Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamicsK H Madsen0P Lodahl1DTU Fotonik, Department of Photonics Engineering, Technical University of Denmark , Ørsteds Plads 343, DK-2800 Kongens Lyngby, Denmark; Niels Bohr Institute, University of Copenhagen , Blegdamsvej 17, DK-2100 Copenhagen, DenmarkNiels Bohr Institute, University of Copenhagen , Blegdamsvej 17, DK-2100 Copenhagen, DenmarkWe present detuning-dependent spectral and decay-rate measurements to study the difference between the spectral and dynamical properties of single quantum dots embedded in micropillar and photonic crystal cavities. For the micropillar cavity, the dynamics is well described by the dissipative Jaynes–Cummings model, whereas systematic deviations are observed for the emission spectra. The discrepancy for the spectra is attributed to the coupling of other exciton lines to the cavity and interference of different propagation paths toward the detector of the fields emitted by the quantum dot. In contrast, quantitative information about the system can readily be extracted from the dynamical measurements. In the case of photonic crystal cavities, we observe an anti-crossing in the spectra when detuning a single quantum dot through resonance, which is the spectral signature of a strong coupling. However, time-resolved measurements reveal that the actual coupling strength is significantly smaller than anticipated from the spectral measurements and that the quantum dot is rather weakly coupled to the cavity. We suggest that the observed Rabi splitting is due to cavity feeding by other quantum dots and/or multi-exciton complexes giving rise to collective emission effects.https://doi.org/10.1088/1367-2630/15/2/025013
spellingShingle K H Madsen
P Lodahl
Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics
New Journal of Physics
title Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics
title_full Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics
title_fullStr Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics
title_full_unstemmed Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics
title_short Quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics
title_sort quantitative analysis of quantum dot dynamics and emission spectra in cavity quantum electrodynamics
url https://doi.org/10.1088/1367-2630/15/2/025013
work_keys_str_mv AT khmadsen quantitativeanalysisofquantumdotdynamicsandemissionspectraincavityquantumelectrodynamics
AT plodahl quantitativeanalysisofquantumdotdynamicsandemissionspectraincavityquantumelectrodynamics