Tunneling noise and defects in exfoliated hexagonal boron nitride

Hexagonal boron nitride (hBN) has become a mainstay as an insulating barrier in stackable nanoelectronics because of its large bandgap and chemical stability. At mono- and bilayer thicknesses, hBN can function as a tunnel barrier for electronic spectroscopy measurements. Noise spectroscopy is of par...

Full description

Bibliographic Details
Main Authors: Xuanhan Zhao, Panpan Zhou, Liyang Chen, Kenji Watanabe, Takashi Taniguchi, Douglas Natelson
Format: Article
Language:English
Published: AIP Publishing LLC 2019-10-01
Series:AIP Advances
Online Access:http://dx.doi.org/10.1063/1.5126129
_version_ 1828858165961162752
author Xuanhan Zhao
Panpan Zhou
Liyang Chen
Kenji Watanabe
Takashi Taniguchi
Douglas Natelson
author_facet Xuanhan Zhao
Panpan Zhou
Liyang Chen
Kenji Watanabe
Takashi Taniguchi
Douglas Natelson
author_sort Xuanhan Zhao
collection DOAJ
description Hexagonal boron nitride (hBN) has become a mainstay as an insulating barrier in stackable nanoelectronics because of its large bandgap and chemical stability. At mono- and bilayer thicknesses, hBN can function as a tunnel barrier for electronic spectroscopy measurements. Noise spectroscopy is of particular interest, as noise can be a sensitive probe for electronic correlations not detectable by first-moment current measurements. In addition to the expected Johnson-Nyquist thermal noise and nonequilibrium shot noise, low frequency (<100 kHz) noise measurements in Au/hBN/Au tunneling structures as a function of temperature and bias reveal the presence of thermally excited dynamic defects, as manifested through a flicker noise contribution at high bias that freezes out as temperature is decreased. In contrast, broad-band high frequency (∼250MHz – 580MHz) measurements on the same device show shot noise with no flicker noise contribution. The presence of the flicker noise through multiple fabrication approaches and processing treatments suggests that the fluctuators are in the hBN layer itself. Device-to-device variation and the approximate 1/f dependence of the flicker noise constrain the fluctuator density to on the order of a few per square micron.
first_indexed 2024-12-13T01:52:27Z
format Article
id doaj.art-b0de5e98c6084272b3622e9b8aa25eda
institution Directory Open Access Journal
issn 2158-3226
language English
last_indexed 2024-12-13T01:52:27Z
publishDate 2019-10-01
publisher AIP Publishing LLC
record_format Article
series AIP Advances
spelling doaj.art-b0de5e98c6084272b3622e9b8aa25eda2022-12-22T00:03:29ZengAIP Publishing LLCAIP Advances2158-32262019-10-01910105218105218-610.1063/1.5126129078910ADVTunneling noise and defects in exfoliated hexagonal boron nitrideXuanhan Zhao0Panpan Zhou1Liyang Chen2Kenji Watanabe3Takashi Taniguchi4Douglas Natelson5Department of Physics and Astronomy, Rice, University, Houston, Texas 77005, USADepartment of Physics and Astronomy, Rice, University, Houston, Texas 77005, USAApplied Physics Program, Smalley-Curl Institute, Rice University, 6100 Main Street, Houston, Texas 77005, USANational Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044, JapanNational Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044, JapanDepartment of Physics and Astronomy, Rice, University, Houston, Texas 77005, USAHexagonal boron nitride (hBN) has become a mainstay as an insulating barrier in stackable nanoelectronics because of its large bandgap and chemical stability. At mono- and bilayer thicknesses, hBN can function as a tunnel barrier for electronic spectroscopy measurements. Noise spectroscopy is of particular interest, as noise can be a sensitive probe for electronic correlations not detectable by first-moment current measurements. In addition to the expected Johnson-Nyquist thermal noise and nonequilibrium shot noise, low frequency (<100 kHz) noise measurements in Au/hBN/Au tunneling structures as a function of temperature and bias reveal the presence of thermally excited dynamic defects, as manifested through a flicker noise contribution at high bias that freezes out as temperature is decreased. In contrast, broad-band high frequency (∼250MHz – 580MHz) measurements on the same device show shot noise with no flicker noise contribution. The presence of the flicker noise through multiple fabrication approaches and processing treatments suggests that the fluctuators are in the hBN layer itself. Device-to-device variation and the approximate 1/f dependence of the flicker noise constrain the fluctuator density to on the order of a few per square micron.http://dx.doi.org/10.1063/1.5126129
spellingShingle Xuanhan Zhao
Panpan Zhou
Liyang Chen
Kenji Watanabe
Takashi Taniguchi
Douglas Natelson
Tunneling noise and defects in exfoliated hexagonal boron nitride
AIP Advances
title Tunneling noise and defects in exfoliated hexagonal boron nitride
title_full Tunneling noise and defects in exfoliated hexagonal boron nitride
title_fullStr Tunneling noise and defects in exfoliated hexagonal boron nitride
title_full_unstemmed Tunneling noise and defects in exfoliated hexagonal boron nitride
title_short Tunneling noise and defects in exfoliated hexagonal boron nitride
title_sort tunneling noise and defects in exfoliated hexagonal boron nitride
url http://dx.doi.org/10.1063/1.5126129
work_keys_str_mv AT xuanhanzhao tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride
AT panpanzhou tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride
AT liyangchen tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride
AT kenjiwatanabe tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride
AT takashitaniguchi tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride
AT douglasnatelson tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride