Tunneling noise and defects in exfoliated hexagonal boron nitride
Hexagonal boron nitride (hBN) has become a mainstay as an insulating barrier in stackable nanoelectronics because of its large bandgap and chemical stability. At mono- and bilayer thicknesses, hBN can function as a tunnel barrier for electronic spectroscopy measurements. Noise spectroscopy is of par...
Main Authors: | , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
AIP Publishing LLC
2019-10-01
|
Series: | AIP Advances |
Online Access: | http://dx.doi.org/10.1063/1.5126129 |
_version_ | 1828858165961162752 |
---|---|
author | Xuanhan Zhao Panpan Zhou Liyang Chen Kenji Watanabe Takashi Taniguchi Douglas Natelson |
author_facet | Xuanhan Zhao Panpan Zhou Liyang Chen Kenji Watanabe Takashi Taniguchi Douglas Natelson |
author_sort | Xuanhan Zhao |
collection | DOAJ |
description | Hexagonal boron nitride (hBN) has become a mainstay as an insulating barrier in stackable nanoelectronics because of its large bandgap and chemical stability. At mono- and bilayer thicknesses, hBN can function as a tunnel barrier for electronic spectroscopy measurements. Noise spectroscopy is of particular interest, as noise can be a sensitive probe for electronic correlations not detectable by first-moment current measurements. In addition to the expected Johnson-Nyquist thermal noise and nonequilibrium shot noise, low frequency (<100 kHz) noise measurements in Au/hBN/Au tunneling structures as a function of temperature and bias reveal the presence of thermally excited dynamic defects, as manifested through a flicker noise contribution at high bias that freezes out as temperature is decreased. In contrast, broad-band high frequency (∼250MHz – 580MHz) measurements on the same device show shot noise with no flicker noise contribution. The presence of the flicker noise through multiple fabrication approaches and processing treatments suggests that the fluctuators are in the hBN layer itself. Device-to-device variation and the approximate 1/f dependence of the flicker noise constrain the fluctuator density to on the order of a few per square micron. |
first_indexed | 2024-12-13T01:52:27Z |
format | Article |
id | doaj.art-b0de5e98c6084272b3622e9b8aa25eda |
institution | Directory Open Access Journal |
issn | 2158-3226 |
language | English |
last_indexed | 2024-12-13T01:52:27Z |
publishDate | 2019-10-01 |
publisher | AIP Publishing LLC |
record_format | Article |
series | AIP Advances |
spelling | doaj.art-b0de5e98c6084272b3622e9b8aa25eda2022-12-22T00:03:29ZengAIP Publishing LLCAIP Advances2158-32262019-10-01910105218105218-610.1063/1.5126129078910ADVTunneling noise and defects in exfoliated hexagonal boron nitrideXuanhan Zhao0Panpan Zhou1Liyang Chen2Kenji Watanabe3Takashi Taniguchi4Douglas Natelson5Department of Physics and Astronomy, Rice, University, Houston, Texas 77005, USADepartment of Physics and Astronomy, Rice, University, Houston, Texas 77005, USAApplied Physics Program, Smalley-Curl Institute, Rice University, 6100 Main Street, Houston, Texas 77005, USANational Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044, JapanNational Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044, JapanDepartment of Physics and Astronomy, Rice, University, Houston, Texas 77005, USAHexagonal boron nitride (hBN) has become a mainstay as an insulating barrier in stackable nanoelectronics because of its large bandgap and chemical stability. At mono- and bilayer thicknesses, hBN can function as a tunnel barrier for electronic spectroscopy measurements. Noise spectroscopy is of particular interest, as noise can be a sensitive probe for electronic correlations not detectable by first-moment current measurements. In addition to the expected Johnson-Nyquist thermal noise and nonequilibrium shot noise, low frequency (<100 kHz) noise measurements in Au/hBN/Au tunneling structures as a function of temperature and bias reveal the presence of thermally excited dynamic defects, as manifested through a flicker noise contribution at high bias that freezes out as temperature is decreased. In contrast, broad-band high frequency (∼250MHz – 580MHz) measurements on the same device show shot noise with no flicker noise contribution. The presence of the flicker noise through multiple fabrication approaches and processing treatments suggests that the fluctuators are in the hBN layer itself. Device-to-device variation and the approximate 1/f dependence of the flicker noise constrain the fluctuator density to on the order of a few per square micron.http://dx.doi.org/10.1063/1.5126129 |
spellingShingle | Xuanhan Zhao Panpan Zhou Liyang Chen Kenji Watanabe Takashi Taniguchi Douglas Natelson Tunneling noise and defects in exfoliated hexagonal boron nitride AIP Advances |
title | Tunneling noise and defects in exfoliated hexagonal boron nitride |
title_full | Tunneling noise and defects in exfoliated hexagonal boron nitride |
title_fullStr | Tunneling noise and defects in exfoliated hexagonal boron nitride |
title_full_unstemmed | Tunneling noise and defects in exfoliated hexagonal boron nitride |
title_short | Tunneling noise and defects in exfoliated hexagonal boron nitride |
title_sort | tunneling noise and defects in exfoliated hexagonal boron nitride |
url | http://dx.doi.org/10.1063/1.5126129 |
work_keys_str_mv | AT xuanhanzhao tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride AT panpanzhou tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride AT liyangchen tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride AT kenjiwatanabe tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride AT takashitaniguchi tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride AT douglasnatelson tunnelingnoiseanddefectsinexfoliatedhexagonalboronnitride |