Readily prepared and processed multifunctional MXene nanocomposite hydrogels for smart electronics

Abstract Booming sophisticated robotics and prosthetics put forward high requirements on soft conductive materials that can bridge electronics and biology, those soft conductive materials should imitate the mechanical properties of biological tissues and build information transmission networks. Unti...

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Main Authors: Jiahui Huang, Xianwu Huang, Peiyi Wu
Format: Article
Language:English
Published: Wiley 2024-04-01
Series:SmartMat
Subjects:
Online Access:https://doi.org/10.1002/smm2.1228
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author Jiahui Huang
Xianwu Huang
Peiyi Wu
author_facet Jiahui Huang
Xianwu Huang
Peiyi Wu
author_sort Jiahui Huang
collection DOAJ
description Abstract Booming sophisticated robotics and prosthetics put forward high requirements on soft conductive materials that can bridge electronics and biology, those soft conductive materials should imitate the mechanical properties of biological tissues and build information transmission networks. Until now, it remains a great challenge to handle the trade‐off among ease of preparation, high conductivity, processability, mechanical adaptability, and external stimuli responsiveness. Herein, a kind of readily prepared and processed multifunctional MXene nanocomposite hydrogel is reported, which is prepared via the fast gelation of cationic monomer initiated by delaminated MXene sheets. The gelation time can be adjusted (several seconds to minutes) based on the MXene loadings. By adjusting the MXene ratio, the resulting nanocomposites are ultrastretchable (>5000%), three‐dimensional (3D) printable, and show outstanding mechanical and electrical self‐healing. As expected, the integration of multifunctional systems onto various substrates (e.g., gloves and masks) is further demonstrated via 3D printing and could achieve diverse sensory capabilities toward strain, pressure, and temperature, showing great prospects as smart flexible electronics.
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spelling doaj.art-b10babc337964c2885bd69469d3888fd2024-04-10T13:32:42ZengWileySmartMat2688-819X2024-04-0152n/an/a10.1002/smm2.1228Readily prepared and processed multifunctional MXene nanocomposite hydrogels for smart electronicsJiahui Huang0Xianwu Huang1Peiyi Wu2State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Chemistry and Chemical Engineering, Center for Advanced Low‐Dimension Materials Donghua University Shanghai ChinaState Key Laboratory of Molecular Engineering of Polymers, Department of Macromolecular Science and Laboratory of Advanced Materials Fudan University Shanghai ChinaState Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Chemistry and Chemical Engineering, Center for Advanced Low‐Dimension Materials Donghua University Shanghai ChinaAbstract Booming sophisticated robotics and prosthetics put forward high requirements on soft conductive materials that can bridge electronics and biology, those soft conductive materials should imitate the mechanical properties of biological tissues and build information transmission networks. Until now, it remains a great challenge to handle the trade‐off among ease of preparation, high conductivity, processability, mechanical adaptability, and external stimuli responsiveness. Herein, a kind of readily prepared and processed multifunctional MXene nanocomposite hydrogel is reported, which is prepared via the fast gelation of cationic monomer initiated by delaminated MXene sheets. The gelation time can be adjusted (several seconds to minutes) based on the MXene loadings. By adjusting the MXene ratio, the resulting nanocomposites are ultrastretchable (>5000%), three‐dimensional (3D) printable, and show outstanding mechanical and electrical self‐healing. As expected, the integration of multifunctional systems onto various substrates (e.g., gloves and masks) is further demonstrated via 3D printing and could achieve diverse sensory capabilities toward strain, pressure, and temperature, showing great prospects as smart flexible electronics.https://doi.org/10.1002/smm2.12283D printableelectronicsMXenepolymeric hydrogelsstretchable and conductive
spellingShingle Jiahui Huang
Xianwu Huang
Peiyi Wu
Readily prepared and processed multifunctional MXene nanocomposite hydrogels for smart electronics
SmartMat
3D printable
electronics
MXene
polymeric hydrogels
stretchable and conductive
title Readily prepared and processed multifunctional MXene nanocomposite hydrogels for smart electronics
title_full Readily prepared and processed multifunctional MXene nanocomposite hydrogels for smart electronics
title_fullStr Readily prepared and processed multifunctional MXene nanocomposite hydrogels for smart electronics
title_full_unstemmed Readily prepared and processed multifunctional MXene nanocomposite hydrogels for smart electronics
title_short Readily prepared and processed multifunctional MXene nanocomposite hydrogels for smart electronics
title_sort readily prepared and processed multifunctional mxene nanocomposite hydrogels for smart electronics
topic 3D printable
electronics
MXene
polymeric hydrogels
stretchable and conductive
url https://doi.org/10.1002/smm2.1228
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