Critical behavior and magnetic entropy change of skyrmion host Co7Zn8Mn5

The magnetic properties of a β-Mn-type alloy Co _7 Zn _8 Mn _5 , which is a chiral magnet hosting skyrmion phase, are comprehensively investigated, exhibiting a ferromagnetic transition around 184 K and a spin freezing near 20 K. The generated Rhodes–Wolfarth ratio equals 1.10, which indicates a wea...

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Bibliographic Details
Main Authors: Xiaojun Yang, Junxiao Pan, Xiangyu He, Shijiang Liu, Hong Jia, Leiming Cao, Mao Yang
Format: Article
Language:English
Published: IOP Publishing 2022-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/ac8b62
Description
Summary:The magnetic properties of a β-Mn-type alloy Co _7 Zn _8 Mn _5 , which is a chiral magnet hosting skyrmion phase, are comprehensively investigated, exhibiting a ferromagnetic transition around 184 K and a spin freezing near 20 K. The generated Rhodes–Wolfarth ratio equals 1.10, which indicates a weak itinerant character of the ferromagnetism in Co _7 Zn _8 Mn _5 . The spin dynamics of the spin freezing agrees with the universal scaling law of critical slowing down with τ _0 = 1.7 × 10 ^−5 s, T _g = 20.2 K, and zν = 3.92. Critical exponents β = 0.423(1) and γ = 1.366(4) are deduced by the modified Arrott plot, whereas δ = 4.22(2) is obtained by a critical isotherm analysis. The validity of the deduced critical exponents is verified by the Widom scaling relation and the scaling hypothesis. The boundary between the first-order and the second-order phase transition is evaluated by a scaling analysis. The magnetic interaction, obtained by a renormalization group theory, decays with distance r as J ( r ) ≈ r ^−4.9 , lying between the mean-field model and the 3D Heisenberg model. The analyses on critical behavior could shed new light on the origin of ferromagnetism and topological Hall effect. Moreover, the magnetic entropy change −Δ S _M exhibits a maximal value around T _C , and the peak position gradually raises with an increasing fields, eliminating the mean-field model. The $-{\Delta}{S}_{\mathrm{M}}^{\mathrm{max}}\enspace $ features a power-law behavior with n > 2/3, excluding any universal standard models of ferromagnetism. The −Δ S _M ( T , H ) plots can be scaled into a universal curve, further verifying the reliability and accuracy of the yielded critical exponents.
ISSN:1367-2630