Material design and prospect of dual-functional materials for integrated carbon dioxide capture and conversion
Large amounts of CO2 were discharged into the atmosphere, resulting in a severe greenhouse effect and inducing ecological environmental problems that threaten human survival. Integrated carbon dioxide capture and conversion (ICCC) with Dual Functional Materials (DFMs) was a promising process to capt...
| Main Authors: | , , , , , , , |
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| Format: | Article |
| Language: | English |
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Elsevier
2024-09-01
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| Series: | Carbon Capture Science & Technology |
| Subjects: | |
| Online Access: | http://www.sciencedirect.com/science/article/pii/S2772656824000198 |
| _version_ | 1797267132548907008 |
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| author | Bowen Lu Yu Fan Xinyu Zhi Ziqiang Han Fan Wu Xiaoshan Li Cong Luo Liqi Zhang |
| author_facet | Bowen Lu Yu Fan Xinyu Zhi Ziqiang Han Fan Wu Xiaoshan Li Cong Luo Liqi Zhang |
| author_sort | Bowen Lu |
| collection | DOAJ |
| description | Large amounts of CO2 were discharged into the atmosphere, resulting in a severe greenhouse effect and inducing ecological environmental problems that threaten human survival. Integrated carbon dioxide capture and conversion (ICCC) with Dual Functional Materials (DFMs) was a promising process to capture CO2 emission in flue gas and convert it into value-added chemicals, reducing energy consumption and economic cost. The catalytic component of DFMs enhances hydrogen source activation and promotes carbonate hydrogenation to produce high value-added chemicals. The hydrogenation process achieved the regeneration of dual-functional materials, which is the key to realizing the ICCC process. This research focuses on DFMs development with different hydrogen sources (hydrogen or light alkanes) for the ICCC process in recent years. In addition, the reaction mechanism and catalytic components modification were discussed to improve the in-situ conversion activity of the ICCC process. Finally, future prospects were anticipated to guide the development and application scenarios of DFMs in the ICCC process. |
| first_indexed | 2024-04-25T01:11:44Z |
| format | Article |
| id | doaj.art-b356c09132ad47e5821f20942ce885b4 |
| institution | Directory Open Access Journal |
| issn | 2772-6568 |
| language | English |
| last_indexed | 2024-04-25T01:11:44Z |
| publishDate | 2024-09-01 |
| publisher | Elsevier |
| record_format | Article |
| series | Carbon Capture Science & Technology |
| spelling | doaj.art-b356c09132ad47e5821f20942ce885b42024-03-10T05:13:33ZengElsevierCarbon Capture Science & Technology2772-65682024-09-0112100207Material design and prospect of dual-functional materials for integrated carbon dioxide capture and conversionBowen Lu0Yu Fan1Xinyu Zhi2Ziqiang Han3Fan Wu4Xiaoshan Li5Cong Luo6Liqi Zhang7State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei Province, People's Republic of ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei Province, People's Republic of ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei Province, People's Republic of ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei Province, People's Republic of ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei Province, People's Republic of ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei Province, People's Republic of ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei Province, People's Republic of ChinaCorresponding author.; State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, Hubei Province, People's Republic of ChinaLarge amounts of CO2 were discharged into the atmosphere, resulting in a severe greenhouse effect and inducing ecological environmental problems that threaten human survival. Integrated carbon dioxide capture and conversion (ICCC) with Dual Functional Materials (DFMs) was a promising process to capture CO2 emission in flue gas and convert it into value-added chemicals, reducing energy consumption and economic cost. The catalytic component of DFMs enhances hydrogen source activation and promotes carbonate hydrogenation to produce high value-added chemicals. The hydrogenation process achieved the regeneration of dual-functional materials, which is the key to realizing the ICCC process. This research focuses on DFMs development with different hydrogen sources (hydrogen or light alkanes) for the ICCC process in recent years. In addition, the reaction mechanism and catalytic components modification were discussed to improve the in-situ conversion activity of the ICCC process. Finally, future prospects were anticipated to guide the development and application scenarios of DFMs in the ICCC process.http://www.sciencedirect.com/science/article/pii/S2772656824000198Hydrogen sourceDual functional materials, CO2 captureIn-situ CO2 conversion |
| spellingShingle | Bowen Lu Yu Fan Xinyu Zhi Ziqiang Han Fan Wu Xiaoshan Li Cong Luo Liqi Zhang Material design and prospect of dual-functional materials for integrated carbon dioxide capture and conversion Carbon Capture Science & Technology Hydrogen source Dual functional materials, CO2 capture In-situ CO2 conversion |
| title | Material design and prospect of dual-functional materials for integrated carbon dioxide capture and conversion |
| title_full | Material design and prospect of dual-functional materials for integrated carbon dioxide capture and conversion |
| title_fullStr | Material design and prospect of dual-functional materials for integrated carbon dioxide capture and conversion |
| title_full_unstemmed | Material design and prospect of dual-functional materials for integrated carbon dioxide capture and conversion |
| title_short | Material design and prospect of dual-functional materials for integrated carbon dioxide capture and conversion |
| title_sort | material design and prospect of dual functional materials for integrated carbon dioxide capture and conversion |
| topic | Hydrogen source Dual functional materials, CO2 capture In-situ CO2 conversion |
| url | http://www.sciencedirect.com/science/article/pii/S2772656824000198 |
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