Indirect methods to control population distribution in a large spin system

We demonstrate how a large spin system ( $S=7/2$ ) with the ground and first excited state separated by a seven-photon transition exhibits nonequilibrium thermodynamic properties and how the population distribution may be manipulated using coupling between energy levels. The first method involves no...

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Main Authors: Lingfei Zhao, Maxim Goryachev, Jeremy Bourhill, Michael E Tobar
Format: Article
Language:English
Published: IOP Publishing 2017-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/aa5fdd
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author Lingfei Zhao
Maxim Goryachev
Jeremy Bourhill
Michael E Tobar
author_facet Lingfei Zhao
Maxim Goryachev
Jeremy Bourhill
Michael E Tobar
author_sort Lingfei Zhao
collection DOAJ
description We demonstrate how a large spin system ( $S=7/2$ ) with the ground and first excited state separated by a seven-photon transition exhibits nonequilibrium thermodynamic properties and how the population distribution may be manipulated using coupling between energy levels. The first method involves non-adiabatic passage through an avoided level crossing controlled with an external DC magnetic field and the resulting Landau–Zener transition. The second method is based on external cavity pumping to a higher energy state hybridised with another state that is two single-photon transitions away from the ground state. The results are confirmed experimentally with a Gd ^3+ impurity ion ensemble in a YVO _4 crystal cooled to 20 mK, which also acts as a microwave photonic whispering gallery mode resonator. Extremely long lifetimes are observed due to the large number of photons required for the transition between the ground and first excited states.
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spelling doaj.art-b3580d1057d84688accc5409d90b93542023-08-08T14:36:10ZengIOP PublishingNew Journal of Physics1367-26302017-01-0119303301610.1088/1367-2630/aa5fddIndirect methods to control population distribution in a large spin systemLingfei Zhao0Maxim Goryachev1https://orcid.org/0000-0002-0257-4054Jeremy Bourhill2Michael E Tobar3Department of Physics, Nanjing University , Nanjing 210093, People's Republic of ChinaARC Centre of Excellence for Engineered Quantum Systems, University of Western Australia , 35 Stirling Highway, Crawley WA 6009, AustraliaARC Centre of Excellence for Engineered Quantum Systems, University of Western Australia , 35 Stirling Highway, Crawley WA 6009, AustraliaARC Centre of Excellence for Engineered Quantum Systems, University of Western Australia , 35 Stirling Highway, Crawley WA 6009, AustraliaWe demonstrate how a large spin system ( $S=7/2$ ) with the ground and first excited state separated by a seven-photon transition exhibits nonequilibrium thermodynamic properties and how the population distribution may be manipulated using coupling between energy levels. The first method involves non-adiabatic passage through an avoided level crossing controlled with an external DC magnetic field and the resulting Landau–Zener transition. The second method is based on external cavity pumping to a higher energy state hybridised with another state that is two single-photon transitions away from the ground state. The results are confirmed experimentally with a Gd ^3+ impurity ion ensemble in a YVO _4 crystal cooled to 20 mK, which also acts as a microwave photonic whispering gallery mode resonator. Extremely long lifetimes are observed due to the large number of photons required for the transition between the ground and first excited states.https://doi.org/10.1088/1367-2630/aa5fddspins in solidslarge spin systemwhispering gallery modeLandau–Zener transition
spellingShingle Lingfei Zhao
Maxim Goryachev
Jeremy Bourhill
Michael E Tobar
Indirect methods to control population distribution in a large spin system
New Journal of Physics
spins in solids
large spin system
whispering gallery mode
Landau–Zener transition
title Indirect methods to control population distribution in a large spin system
title_full Indirect methods to control population distribution in a large spin system
title_fullStr Indirect methods to control population distribution in a large spin system
title_full_unstemmed Indirect methods to control population distribution in a large spin system
title_short Indirect methods to control population distribution in a large spin system
title_sort indirect methods to control population distribution in a large spin system
topic spins in solids
large spin system
whispering gallery mode
Landau–Zener transition
url https://doi.org/10.1088/1367-2630/aa5fdd
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