Selective electrochemical oxidative coupling of methane mediated by Sr2Fe1.5Mo0.5O6-δ and its chemical stability

Catalytic conversion of methane to ethene is limited by poor conversion, selectivity, and catalyst stability. Here a solid oxide electrolysis process is reported as a promising method for selective, partial oxidation of methane with low overpotentials.

Bibliographic Details
Main Authors: Kannan P. Ramaiyan, Luke H. Denoyer, Angelica Benavidez, Fernando H. Garzon
Format: Article
Language:English
Published: Nature Portfolio 2021-09-01
Series:Communications Chemistry
Online Access:https://doi.org/10.1038/s42004-021-00568-1
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author Kannan P. Ramaiyan
Luke H. Denoyer
Angelica Benavidez
Fernando H. Garzon
author_facet Kannan P. Ramaiyan
Luke H. Denoyer
Angelica Benavidez
Fernando H. Garzon
author_sort Kannan P. Ramaiyan
collection DOAJ
description Catalytic conversion of methane to ethene is limited by poor conversion, selectivity, and catalyst stability. Here a solid oxide electrolysis process is reported as a promising method for selective, partial oxidation of methane with low overpotentials.
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spelling doaj.art-b3d2b7dd28b54bb4b8f5d13cb944b9de2022-12-21T23:37:30ZengNature PortfolioCommunications Chemistry2399-36692021-09-01411910.1038/s42004-021-00568-1Selective electrochemical oxidative coupling of methane mediated by Sr2Fe1.5Mo0.5O6-δ and its chemical stabilityKannan P. Ramaiyan0Luke H. Denoyer1Angelica Benavidez2Fernando H. Garzon3Center for Micro-Engineered Materials, Department of Chemical and Biological Engineering, University of New MexicoCenter for Micro-Engineered Materials, Department of Chemical and Biological Engineering, University of New MexicoCenter for Micro-Engineered Materials, Department of Chemical and Biological Engineering, University of New MexicoCenter for Micro-Engineered Materials, Department of Chemical and Biological Engineering, University of New MexicoCatalytic conversion of methane to ethene is limited by poor conversion, selectivity, and catalyst stability. Here a solid oxide electrolysis process is reported as a promising method for selective, partial oxidation of methane with low overpotentials.https://doi.org/10.1038/s42004-021-00568-1
spellingShingle Kannan P. Ramaiyan
Luke H. Denoyer
Angelica Benavidez
Fernando H. Garzon
Selective electrochemical oxidative coupling of methane mediated by Sr2Fe1.5Mo0.5O6-δ and its chemical stability
Communications Chemistry
title Selective electrochemical oxidative coupling of methane mediated by Sr2Fe1.5Mo0.5O6-δ and its chemical stability
title_full Selective electrochemical oxidative coupling of methane mediated by Sr2Fe1.5Mo0.5O6-δ and its chemical stability
title_fullStr Selective electrochemical oxidative coupling of methane mediated by Sr2Fe1.5Mo0.5O6-δ and its chemical stability
title_full_unstemmed Selective electrochemical oxidative coupling of methane mediated by Sr2Fe1.5Mo0.5O6-δ and its chemical stability
title_short Selective electrochemical oxidative coupling of methane mediated by Sr2Fe1.5Mo0.5O6-δ and its chemical stability
title_sort selective electrochemical oxidative coupling of methane mediated by sr2fe1 5mo0 5o6 δ and its chemical stability
url https://doi.org/10.1038/s42004-021-00568-1
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AT lukehdenoyer selectiveelectrochemicaloxidativecouplingofmethanemediatedbysr2fe15mo05o6danditschemicalstability
AT angelicabenavidez selectiveelectrochemicaloxidativecouplingofmethanemediatedbysr2fe15mo05o6danditschemicalstability
AT fernandohgarzon selectiveelectrochemicaloxidativecouplingofmethanemediatedbysr2fe15mo05o6danditschemicalstability