Isolated copper single sites for high-performance electroreduction of carbon monoxide to multicarbon products

Electrochemical carbon monoxide reduction is a promising strategy to yield valuable multicarbon products but low selectivities and Faradaic efficiencies are common. Here the authors show single atom copper catalyst supported on MXene with high CO reduction performance and stability.

Bibliographic Details
Main Authors: Haihong Bao, Yuan Qiu, Xianyun Peng, Jia-ao Wang, Yuying Mi, Shunzheng Zhao, Xijun Liu, Yifan Liu, Rui Cao, Longchao Zhuo, Junqiang Ren, Jiaqiang Sun, Jun Luo, Xuping Sun
Format: Article
Language:English
Published: Nature Portfolio 2021-01-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-020-20336-4
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author Haihong Bao
Yuan Qiu
Xianyun Peng
Jia-ao Wang
Yuying Mi
Shunzheng Zhao
Xijun Liu
Yifan Liu
Rui Cao
Longchao Zhuo
Junqiang Ren
Jiaqiang Sun
Jun Luo
Xuping Sun
author_facet Haihong Bao
Yuan Qiu
Xianyun Peng
Jia-ao Wang
Yuying Mi
Shunzheng Zhao
Xijun Liu
Yifan Liu
Rui Cao
Longchao Zhuo
Junqiang Ren
Jiaqiang Sun
Jun Luo
Xuping Sun
author_sort Haihong Bao
collection DOAJ
description Electrochemical carbon monoxide reduction is a promising strategy to yield valuable multicarbon products but low selectivities and Faradaic efficiencies are common. Here the authors show single atom copper catalyst supported on MXene with high CO reduction performance and stability.
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spelling doaj.art-b45a761d38ec4c42894c07f2b99721e52022-12-21T18:35:40ZengNature PortfolioNature Communications2041-17232021-01-011211910.1038/s41467-020-20336-4Isolated copper single sites for high-performance electroreduction of carbon monoxide to multicarbon productsHaihong Bao0Yuan Qiu1Xianyun Peng2Jia-ao Wang3Yuying Mi4Shunzheng Zhao5Xijun Liu6Yifan Liu7Rui Cao8Longchao Zhuo9Junqiang Ren10Jiaqiang Sun11Jun Luo12Xuping Sun13Institute for New Energy Materials & Low-Carbon Technologies and Tianjin Key Lab of Photoelectric Materials & Devices, School of Materials Science and Engineering, Tianjin University of TechnologyInstitute for New Energy Materials & Low-Carbon Technologies and Tianjin Key Lab of Photoelectric Materials & Devices, School of Materials Science and Engineering, Tianjin University of TechnologyInstitute for New Energy Materials & Low-Carbon Technologies and Tianjin Key Lab of Photoelectric Materials & Devices, School of Materials Science and Engineering, Tianjin University of TechnologySchool of Material Science and Engineering, University of JinanInstitute for New Energy Materials & Low-Carbon Technologies and Tianjin Key Lab of Photoelectric Materials & Devices, School of Materials Science and Engineering, Tianjin University of TechnologyDepartment of Environmental Engineering, University of Science and Technology BeijingInstitute for New Energy Materials & Low-Carbon Technologies and Tianjin Key Lab of Photoelectric Materials & Devices, School of Materials Science and Engineering, Tianjin University of TechnologyCollege of Physics and Optoelectronic Engineering, Shenzhen UniversityStanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratorySchool of Materials Science and Engineering, Xi’an University of TechnologyState Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals, Lanzhou University of TechnologyState Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of SciencesInstitute for New Energy Materials & Low-Carbon Technologies and Tianjin Key Lab of Photoelectric Materials & Devices, School of Materials Science and Engineering, Tianjin University of TechnologyInstitute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of ChinaElectrochemical carbon monoxide reduction is a promising strategy to yield valuable multicarbon products but low selectivities and Faradaic efficiencies are common. Here the authors show single atom copper catalyst supported on MXene with high CO reduction performance and stability.https://doi.org/10.1038/s41467-020-20336-4
spellingShingle Haihong Bao
Yuan Qiu
Xianyun Peng
Jia-ao Wang
Yuying Mi
Shunzheng Zhao
Xijun Liu
Yifan Liu
Rui Cao
Longchao Zhuo
Junqiang Ren
Jiaqiang Sun
Jun Luo
Xuping Sun
Isolated copper single sites for high-performance electroreduction of carbon monoxide to multicarbon products
Nature Communications
title Isolated copper single sites for high-performance electroreduction of carbon monoxide to multicarbon products
title_full Isolated copper single sites for high-performance electroreduction of carbon monoxide to multicarbon products
title_fullStr Isolated copper single sites for high-performance electroreduction of carbon monoxide to multicarbon products
title_full_unstemmed Isolated copper single sites for high-performance electroreduction of carbon monoxide to multicarbon products
title_short Isolated copper single sites for high-performance electroreduction of carbon monoxide to multicarbon products
title_sort isolated copper single sites for high performance electroreduction of carbon monoxide to multicarbon products
url https://doi.org/10.1038/s41467-020-20336-4
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