Emissions of non-methane volatile organic compounds from combustion of domestic fuels in Delhi, India
<p>Twenty-nine different fuel types used in residential dwellings in northern India were collected from across Delhi (76 samples in total). Emission factors of a wide range of non-methane volatile organic compounds (NMVOCs) (192 compounds in total) were measured during controlled burning exper...
Main Authors: | , , , , , , , , , , , , , , , , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Copernicus Publications
2021-02-01
|
Series: | Atmospheric Chemistry and Physics |
Online Access: | https://acp.copernicus.org/articles/21/2383/2021/acp-21-2383-2021.pdf |
_version_ | 1818923146610212864 |
---|---|
author | G. J. Stewart W. J. F. Acton W. J. F. Acton B. S. Nelson A. R. Vaughan J. R. Hopkins J. R. Hopkins R. Arya R. Arya A. Mondal A. Mondal R. Jangirh R. Jangirh S. Ahlawat S. Ahlawat L. Yadav L. Yadav S. K. Sharma S. K. Sharma R. E. Dunmore S. S. M. Yunus C. N. Hewitt E. Nemitz N. Mullinger R. Gadi L. K. Sahu N. Tripathi A. R. Rickard A. R. Rickard J. D. Lee J. D. Lee T. K. Mandal T. K. Mandal J. F. Hamilton |
author_facet | G. J. Stewart W. J. F. Acton W. J. F. Acton B. S. Nelson A. R. Vaughan J. R. Hopkins J. R. Hopkins R. Arya R. Arya A. Mondal A. Mondal R. Jangirh R. Jangirh S. Ahlawat S. Ahlawat L. Yadav L. Yadav S. K. Sharma S. K. Sharma R. E. Dunmore S. S. M. Yunus C. N. Hewitt E. Nemitz N. Mullinger R. Gadi L. K. Sahu N. Tripathi A. R. Rickard A. R. Rickard J. D. Lee J. D. Lee T. K. Mandal T. K. Mandal J. F. Hamilton |
author_sort | G. J. Stewart |
collection | DOAJ |
description | <p>Twenty-nine different fuel types used in residential dwellings in northern India were
collected from across Delhi (76 samples in total). Emission factors of a
wide range of non-methane volatile organic compounds (NMVOCs) (192 compounds
in total) were measured during controlled burning experiments using
dual-channel gas chromatography with flame ionisation detection (DC-GC-FID),
two-dimensional gas chromatography (GC <span class="inline-formula">×</span> GC-FID),
proton-transfer-reaction time-of-flight mass spectrometry (PTR-ToF-MS) and
solid-phase extraction two-dimensional gas chromatography with
time-of-flight mass spectrometry (SPE-GC <span class="inline-formula">×</span> GC–ToF-MS). On average, 94 %
speciation of total measured NMVOC emissions was achieved across
all fuel types. The largest contributors to emissions from most fuel types
were small non-aromatic oxygenated species, phenolics and furanics. The
emission factors (in g kg<span class="inline-formula"><sup>−1</sup></span>) for total gas-phase NMVOCs were fuelwood (18.7, 4.3–96.7), cow dung cake (62.0, 35.3–83.0), crop residue (37.9, 8.9–73.8), charcoal (5.4, 2.4–7.9), sawdust (72.4, 28.6–115.5), municipal solid waste (87.3, 56.6–119.1) and liquefied petroleum gas (5.7, 1.9–9.8).</p>
<p>The emission factors measured in this study allow for better
characterisation, evaluation and understanding of the air quality impacts of residential solid-fuel combustion in India.</p> |
first_indexed | 2024-12-20T02:04:48Z |
format | Article |
id | doaj.art-b4819481fd544590a71131cde677d3db |
institution | Directory Open Access Journal |
issn | 1680-7316 1680-7324 |
language | English |
last_indexed | 2024-12-20T02:04:48Z |
publishDate | 2021-02-01 |
publisher | Copernicus Publications |
record_format | Article |
series | Atmospheric Chemistry and Physics |
spelling | doaj.art-b4819481fd544590a71131cde677d3db2022-12-21T19:57:13ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242021-02-01212383240610.5194/acp-21-2383-2021Emissions of non-methane volatile organic compounds from combustion of domestic fuels in Delhi, IndiaG. J. Stewart0W. J. F. Acton1W. J. F. Acton2B. S. Nelson3A. R. Vaughan4J. R. Hopkins5J. R. Hopkins6R. Arya7R. Arya8A. Mondal9A. Mondal10R. Jangirh11R. Jangirh12S. Ahlawat13S. Ahlawat14L. Yadav15L. Yadav16S. K. Sharma17S. K. Sharma18R. E. Dunmore19S. S. M. Yunus20C. N. Hewitt21E. Nemitz22N. Mullinger23R. Gadi24L. K. Sahu25N. Tripathi26A. R. Rickard27A. R. Rickard28J. D. Lee29J. D. Lee30T. K. Mandal31T. K. Mandal32J. F. Hamilton33Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UKLancaster Environment Centre, Lancaster University, Lancaster LA1 4YQ, UKnow at: School of Geography, Earth and Environmental Sciences, University of Birmingham, B15 2TT, Birmingham, UKWolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UKWolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UKWolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UKNational Centre for Atmospheric Science, University of York, York, YO10 5DD, UKCSIR-National Physical Laboratory, Dr. K.S. Krishnan Marg, New Delhi, Delhi 110012, IndiaAcademy of Scientific & Innovative Research, Ghaziabad, Uttar Pradesh 201 002, IndiaCSIR-National Physical Laboratory, Dr. K.S. Krishnan Marg, New Delhi, Delhi 110012, IndiaAcademy of Scientific & Innovative Research, Ghaziabad, Uttar Pradesh 201 002, IndiaCSIR-National Physical Laboratory, Dr. K.S. Krishnan Marg, New Delhi, Delhi 110012, IndiaAcademy of Scientific & Innovative Research, Ghaziabad, Uttar Pradesh 201 002, IndiaCSIR-National Physical Laboratory, Dr. K.S. Krishnan Marg, New Delhi, Delhi 110012, IndiaAcademy of Scientific & Innovative Research, Ghaziabad, Uttar Pradesh 201 002, IndiaCSIR-National Physical Laboratory, Dr. K.S. Krishnan Marg, New Delhi, Delhi 110012, IndiaAcademy of Scientific & Innovative Research, Ghaziabad, Uttar Pradesh 201 002, IndiaCSIR-National Physical Laboratory, Dr. K.S. Krishnan Marg, New Delhi, Delhi 110012, IndiaAcademy of Scientific & Innovative Research, Ghaziabad, Uttar Pradesh 201 002, IndiaWolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UKSchool of Water, Energy and Environment, Cranfield University, Cranfield, MK43 0AL, UKLancaster Environment Centre, Lancaster University, Lancaster LA1 4YQ, UKUK Centre for Ecology and Hydrology, Bush Estate, Penicuik, EH26 0QB, UKUK Centre for Ecology and Hydrology, Bush Estate, Penicuik, EH26 0QB, UKIndira Gandhi Delhi Technical University for Women, Kashmiri Gate, New Delhi, Delhi 110006, IndiaPhysical Research Laboratory (PRL), Ahmedabad 380009, IndiaPhysical Research Laboratory (PRL), Ahmedabad 380009, IndiaWolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UKNational Centre for Atmospheric Science, University of York, York, YO10 5DD, UKWolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UKNational Centre for Atmospheric Science, University of York, York, YO10 5DD, UKCSIR-National Physical Laboratory, Dr. K.S. Krishnan Marg, New Delhi, Delhi 110012, IndiaAcademy of Scientific & Innovative Research, Ghaziabad, Uttar Pradesh 201 002, IndiaWolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, YO10 5DD, UK<p>Twenty-nine different fuel types used in residential dwellings in northern India were collected from across Delhi (76 samples in total). Emission factors of a wide range of non-methane volatile organic compounds (NMVOCs) (192 compounds in total) were measured during controlled burning experiments using dual-channel gas chromatography with flame ionisation detection (DC-GC-FID), two-dimensional gas chromatography (GC <span class="inline-formula">×</span> GC-FID), proton-transfer-reaction time-of-flight mass spectrometry (PTR-ToF-MS) and solid-phase extraction two-dimensional gas chromatography with time-of-flight mass spectrometry (SPE-GC <span class="inline-formula">×</span> GC–ToF-MS). On average, 94 % speciation of total measured NMVOC emissions was achieved across all fuel types. The largest contributors to emissions from most fuel types were small non-aromatic oxygenated species, phenolics and furanics. The emission factors (in g kg<span class="inline-formula"><sup>−1</sup></span>) for total gas-phase NMVOCs were fuelwood (18.7, 4.3–96.7), cow dung cake (62.0, 35.3–83.0), crop residue (37.9, 8.9–73.8), charcoal (5.4, 2.4–7.9), sawdust (72.4, 28.6–115.5), municipal solid waste (87.3, 56.6–119.1) and liquefied petroleum gas (5.7, 1.9–9.8).</p> <p>The emission factors measured in this study allow for better characterisation, evaluation and understanding of the air quality impacts of residential solid-fuel combustion in India.</p>https://acp.copernicus.org/articles/21/2383/2021/acp-21-2383-2021.pdf |
spellingShingle | G. J. Stewart W. J. F. Acton W. J. F. Acton B. S. Nelson A. R. Vaughan J. R. Hopkins J. R. Hopkins R. Arya R. Arya A. Mondal A. Mondal R. Jangirh R. Jangirh S. Ahlawat S. Ahlawat L. Yadav L. Yadav S. K. Sharma S. K. Sharma R. E. Dunmore S. S. M. Yunus C. N. Hewitt E. Nemitz N. Mullinger R. Gadi L. K. Sahu N. Tripathi A. R. Rickard A. R. Rickard J. D. Lee J. D. Lee T. K. Mandal T. K. Mandal J. F. Hamilton Emissions of non-methane volatile organic compounds from combustion of domestic fuels in Delhi, India Atmospheric Chemistry and Physics |
title | Emissions of non-methane volatile organic compounds from combustion of domestic fuels in Delhi, India |
title_full | Emissions of non-methane volatile organic compounds from combustion of domestic fuels in Delhi, India |
title_fullStr | Emissions of non-methane volatile organic compounds from combustion of domestic fuels in Delhi, India |
title_full_unstemmed | Emissions of non-methane volatile organic compounds from combustion of domestic fuels in Delhi, India |
title_short | Emissions of non-methane volatile organic compounds from combustion of domestic fuels in Delhi, India |
title_sort | emissions of non methane volatile organic compounds from combustion of domestic fuels in delhi india |
url | https://acp.copernicus.org/articles/21/2383/2021/acp-21-2383-2021.pdf |
work_keys_str_mv | AT gjstewart emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT wjfacton emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT wjfacton emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT bsnelson emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT arvaughan emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT jrhopkins emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT jrhopkins emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT rarya emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT rarya emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT amondal emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT amondal emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT rjangirh emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT rjangirh emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT sahlawat emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT sahlawat emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT lyadav emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT lyadav emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT sksharma emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT sksharma emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT redunmore emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT ssmyunus emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT cnhewitt emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT enemitz emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT nmullinger emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT rgadi emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT lksahu emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT ntripathi emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT arrickard emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT arrickard emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT jdlee emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT jdlee emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT tkmandal emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT tkmandal emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia AT jfhamilton emissionsofnonmethanevolatileorganiccompoundsfromcombustionofdomesticfuelsindelhiindia |