Direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observations

We used more than five years of continuous aerosol measurements to estimate the direct radiative feedback parameter associated with the formation of biogenic secondary organic aerosol (BSOA) at a remote continental site at the edge of the boreal forest zone in Northern Finland. Our upper-limit estim...

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Main Authors: Heikki Lihavainen, Eija Asmi, Veijo Aaltonen, Ulla Makkonen, Veli-Matti Kerminen
Format: Article
Language:English
Published: IOP Publishing 2015-01-01
Series:Environmental Research Letters
Subjects:
Online Access:https://doi.org/10.1088/1748-9326/10/10/104005
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author Heikki Lihavainen
Eija Asmi
Veijo Aaltonen
Ulla Makkonen
Veli-Matti Kerminen
author_facet Heikki Lihavainen
Eija Asmi
Veijo Aaltonen
Ulla Makkonen
Veli-Matti Kerminen
author_sort Heikki Lihavainen
collection DOAJ
description We used more than five years of continuous aerosol measurements to estimate the direct radiative feedback parameter associated with the formation of biogenic secondary organic aerosol (BSOA) at a remote continental site at the edge of the boreal forest zone in Northern Finland. Our upper-limit estimate for this feedback parameter during the summer period (ambient temperatures above 10 °C) was −97 ± 66 mW m ^−2 K ^−1 (mean ± STD) when using measurements of the aerosol optical depth ( f _AOD ) and −63 ± 40 mW m ^−2 K ^−1 when using measurements of the ‘dry’ aerosol scattering coefficient at the ground level ( f _σ ). Here STD represents the variability in f caused by the observed variability in the quantities used to derive the value of f . Compared with our measurement site, the magnitude of the direct radiative feedback associated with BSOA is expected to be larger in warmer continental regions with more abundant biogenic emissions, and even larger in regions where biogenic emissions are mixed with anthropogenic pollution.
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spelling doaj.art-b5b71d0d365a44e0a7bc98b5992cbef22023-08-09T14:16:34ZengIOP PublishingEnvironmental Research Letters1748-93262015-01-01101010400510.1088/1748-9326/10/10/104005Direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observationsHeikki Lihavainen0Eija Asmi1Veijo Aaltonen2Ulla Makkonen3Veli-Matti Kerminen4Finnish Meteorological Institute, Helsinki, FinlandFinnish Meteorological Institute, Helsinki, FinlandFinnish Meteorological Institute, Helsinki, FinlandFinnish Meteorological Institute, Helsinki, FinlandFinnish Meteorological Institute, Helsinki, Finland; Department of Physics, University of Helsinki , FinlandWe used more than five years of continuous aerosol measurements to estimate the direct radiative feedback parameter associated with the formation of biogenic secondary organic aerosol (BSOA) at a remote continental site at the edge of the boreal forest zone in Northern Finland. Our upper-limit estimate for this feedback parameter during the summer period (ambient temperatures above 10 °C) was −97 ± 66 mW m ^−2 K ^−1 (mean ± STD) when using measurements of the aerosol optical depth ( f _AOD ) and −63 ± 40 mW m ^−2 K ^−1 when using measurements of the ‘dry’ aerosol scattering coefficient at the ground level ( f _σ ). Here STD represents the variability in f caused by the observed variability in the quantities used to derive the value of f . Compared with our measurement site, the magnitude of the direct radiative feedback associated with BSOA is expected to be larger in warmer continental regions with more abundant biogenic emissions, and even larger in regions where biogenic emissions are mixed with anthropogenic pollution.https://doi.org/10.1088/1748-9326/10/10/104005aerosolfeedbackbiogenic
spellingShingle Heikki Lihavainen
Eija Asmi
Veijo Aaltonen
Ulla Makkonen
Veli-Matti Kerminen
Direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observations
Environmental Research Letters
aerosol
feedback
biogenic
title Direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observations
title_full Direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observations
title_fullStr Direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observations
title_full_unstemmed Direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observations
title_short Direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observations
title_sort direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observations
topic aerosol
feedback
biogenic
url https://doi.org/10.1088/1748-9326/10/10/104005
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