Tunable Photoresponse in a Two-Dimensional Superconducting Heterostructure

The photo-induced superconducting phase transition is widely used in probing the physical properties of correlated electronic systems and to realize broadband photodetection with extremely high responsivity. However, such photoresponse is usually insensitive to electrostatic doping due to the high c...

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Những tác giả chính: Zijie Ji, Ruan Zhang, Shuangxing Zhu, Feifan Gu, Yunmin Jin, Binghe Xie, Jiaxin Wu, Xinghan Cai
Định dạng: Bài viết
Ngôn ngữ:English
Được phát hành: MDPI AG 2023-01-01
Loạt:Nanomaterials
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Truy cập trực tuyến:https://www.mdpi.com/2079-4991/13/3/421
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author Zijie Ji
Ruan Zhang
Shuangxing Zhu
Feifan Gu
Yunmin Jin
Binghe Xie
Jiaxin Wu
Xinghan Cai
author_facet Zijie Ji
Ruan Zhang
Shuangxing Zhu
Feifan Gu
Yunmin Jin
Binghe Xie
Jiaxin Wu
Xinghan Cai
author_sort Zijie Ji
collection DOAJ
description The photo-induced superconducting phase transition is widely used in probing the physical properties of correlated electronic systems and to realize broadband photodetection with extremely high responsivity. However, such photoresponse is usually insensitive to electrostatic doping due to the high carrier density of the superconductor, restricting its applications in tunable optoelectronic devices. In this work, we demonstrate the gate voltage modulation to the photoresponsivity in a two-dimensional NbSe<sub>2</sub>-graphene heterojunction. The superconducting critical current of the NbSe<sub>2</sub> relies on the gate-dependent hot carrier generation in graphene via the Joule heating effect, leading to the observed shift of both the magnitude and peak position of the photoresponsivity spectra as the gate voltage changes. This heating effect is further confirmed by the temperature and laser-power-dependent characterization of the photoresponse. In addition, we investigate the spatially-resolved photocurrent, finding that the superconductivity is inhomogeneous across the junction area. Our results provide a new platform for designing tunable superconducting photodetector and indicate that the photoresponse could be a powerful tool in studying the local electronic properties and phase transitions in low-dimensional superconducting systems.
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spelling doaj.art-b667673609d841c6a35d974854516cc82023-11-16T17:34:28ZengMDPI AGNanomaterials2079-49912023-01-0113342110.3390/nano13030421Tunable Photoresponse in a Two-Dimensional Superconducting HeterostructureZijie Ji0Ruan Zhang1Shuangxing Zhu2Feifan Gu3Yunmin Jin4Binghe Xie5Jiaxin Wu6Xinghan Cai7National Key Laboratory of Science and Technology on Micro/Nano Fabrication, Shanghai Jiao Tong University, Shanghai 200240, ChinaNational Key Laboratory of Science and Technology on Micro/Nano Fabrication, Shanghai Jiao Tong University, Shanghai 200240, ChinaNational Key Laboratory of Science and Technology on Micro/Nano Fabrication, Shanghai Jiao Tong University, Shanghai 200240, ChinaNational Key Laboratory of Science and Technology on Micro/Nano Fabrication, Shanghai Jiao Tong University, Shanghai 200240, ChinaNational Key Laboratory of Science and Technology on Micro/Nano Fabrication, Shanghai Jiao Tong University, Shanghai 200240, ChinaNational Key Laboratory of Science and Technology on Micro/Nano Fabrication, Shanghai Jiao Tong University, Shanghai 200240, ChinaNational Key Laboratory of Science and Technology on Micro/Nano Fabrication, Shanghai Jiao Tong University, Shanghai 200240, ChinaNational Key Laboratory of Science and Technology on Micro/Nano Fabrication, Shanghai Jiao Tong University, Shanghai 200240, ChinaThe photo-induced superconducting phase transition is widely used in probing the physical properties of correlated electronic systems and to realize broadband photodetection with extremely high responsivity. However, such photoresponse is usually insensitive to electrostatic doping due to the high carrier density of the superconductor, restricting its applications in tunable optoelectronic devices. In this work, we demonstrate the gate voltage modulation to the photoresponsivity in a two-dimensional NbSe<sub>2</sub>-graphene heterojunction. The superconducting critical current of the NbSe<sub>2</sub> relies on the gate-dependent hot carrier generation in graphene via the Joule heating effect, leading to the observed shift of both the magnitude and peak position of the photoresponsivity spectra as the gate voltage changes. This heating effect is further confirmed by the temperature and laser-power-dependent characterization of the photoresponse. In addition, we investigate the spatially-resolved photocurrent, finding that the superconductivity is inhomogeneous across the junction area. Our results provide a new platform for designing tunable superconducting photodetector and indicate that the photoresponse could be a powerful tool in studying the local electronic properties and phase transitions in low-dimensional superconducting systems.https://www.mdpi.com/2079-4991/13/3/421niobium diselenidevan der Waals heterostructuresuperconducting photodetectorgate modulation
spellingShingle Zijie Ji
Ruan Zhang
Shuangxing Zhu
Feifan Gu
Yunmin Jin
Binghe Xie
Jiaxin Wu
Xinghan Cai
Tunable Photoresponse in a Two-Dimensional Superconducting Heterostructure
Nanomaterials
niobium diselenide
van der Waals heterostructure
superconducting photodetector
gate modulation
title Tunable Photoresponse in a Two-Dimensional Superconducting Heterostructure
title_full Tunable Photoresponse in a Two-Dimensional Superconducting Heterostructure
title_fullStr Tunable Photoresponse in a Two-Dimensional Superconducting Heterostructure
title_full_unstemmed Tunable Photoresponse in a Two-Dimensional Superconducting Heterostructure
title_short Tunable Photoresponse in a Two-Dimensional Superconducting Heterostructure
title_sort tunable photoresponse in a two dimensional superconducting heterostructure
topic niobium diselenide
van der Waals heterostructure
superconducting photodetector
gate modulation
url https://www.mdpi.com/2079-4991/13/3/421
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AT feifangu tunablephotoresponseinatwodimensionalsuperconductingheterostructure
AT yunminjin tunablephotoresponseinatwodimensionalsuperconductingheterostructure
AT binghexie tunablephotoresponseinatwodimensionalsuperconductingheterostructure
AT jiaxinwu tunablephotoresponseinatwodimensionalsuperconductingheterostructure
AT xinghancai tunablephotoresponseinatwodimensionalsuperconductingheterostructure