Multi-Electron Ionization and Coulomb Explosion of the IBr Molecule in the Near-Infrared Femtosecond Laser Field

The DC-sliced ion velocity map imaging approach was used to analyze the multi-electron ionization and subsequent Coulomb explosion of an IBr molecule exposed to a near-infrared femtosecond laser field. The existence of the molecular ions up to IBr<sup>7+</sup> was observed in the experim...

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Main Authors: Botong Liu, Zhipeng Li, Zhenrong Sun, Yan Yang
Format: Article
Language:English
Published: MDPI AG 2023-12-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/13/24/13185
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author Botong Liu
Zhipeng Li
Zhenrong Sun
Yan Yang
author_facet Botong Liu
Zhipeng Li
Zhenrong Sun
Yan Yang
author_sort Botong Liu
collection DOAJ
description The DC-sliced ion velocity map imaging approach was used to analyze the multi-electron ionization and subsequent Coulomb explosion of an IBr molecule exposed to a near-infrared femtosecond laser field. The existence of the molecular ions up to IBr<sup>7+</sup> was observed in the experiment, and a series of Coulomb explosion channels are assigned. According to the “ladder-path” ionization model, the multi-electron ionization paths of IBr molecules are determined. We find that the charge transfer process does not occur during ionization, and the presence of higher charge states can be explained by considering the higher-order ionization process.
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spelling doaj.art-b67085d17a7d40638c351b1c27928f812023-12-22T13:51:46ZengMDPI AGApplied Sciences2076-34172023-12-0113241318510.3390/app132413185Multi-Electron Ionization and Coulomb Explosion of the IBr Molecule in the Near-Infrared Femtosecond Laser FieldBotong Liu0Zhipeng Li1Zhenrong Sun2Yan Yang3School of Information Engineering, Yancheng Institute of Technology, Yancheng 224051, ChinaState Key Laboratory of Precision Spectroscopy, School of Physics and Electronic Science, East China Normal University, Shanghai 200062, ChinaState Key Laboratory of Precision Spectroscopy, School of Physics and Electronic Science, East China Normal University, Shanghai 200062, ChinaState Key Laboratory of Precision Spectroscopy, School of Physics and Electronic Science, East China Normal University, Shanghai 200062, ChinaThe DC-sliced ion velocity map imaging approach was used to analyze the multi-electron ionization and subsequent Coulomb explosion of an IBr molecule exposed to a near-infrared femtosecond laser field. The existence of the molecular ions up to IBr<sup>7+</sup> was observed in the experiment, and a series of Coulomb explosion channels are assigned. According to the “ladder-path” ionization model, the multi-electron ionization paths of IBr molecules are determined. We find that the charge transfer process does not occur during ionization, and the presence of higher charge states can be explained by considering the higher-order ionization process.https://www.mdpi.com/2076-3417/13/24/13185multi-electron ionizationCoulomb explosionfemtosecond laser field
spellingShingle Botong Liu
Zhipeng Li
Zhenrong Sun
Yan Yang
Multi-Electron Ionization and Coulomb Explosion of the IBr Molecule in the Near-Infrared Femtosecond Laser Field
Applied Sciences
multi-electron ionization
Coulomb explosion
femtosecond laser field
title Multi-Electron Ionization and Coulomb Explosion of the IBr Molecule in the Near-Infrared Femtosecond Laser Field
title_full Multi-Electron Ionization and Coulomb Explosion of the IBr Molecule in the Near-Infrared Femtosecond Laser Field
title_fullStr Multi-Electron Ionization and Coulomb Explosion of the IBr Molecule in the Near-Infrared Femtosecond Laser Field
title_full_unstemmed Multi-Electron Ionization and Coulomb Explosion of the IBr Molecule in the Near-Infrared Femtosecond Laser Field
title_short Multi-Electron Ionization and Coulomb Explosion of the IBr Molecule in the Near-Infrared Femtosecond Laser Field
title_sort multi electron ionization and coulomb explosion of the ibr molecule in the near infrared femtosecond laser field
topic multi-electron ionization
Coulomb explosion
femtosecond laser field
url https://www.mdpi.com/2076-3417/13/24/13185
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AT zhenrongsun multielectronionizationandcoulombexplosionoftheibrmoleculeinthenearinfraredfemtosecondlaserfield
AT yanyang multielectronionizationandcoulombexplosionoftheibrmoleculeinthenearinfraredfemtosecondlaserfield