The Potential for PE Microplastics to Affect the Removal of Carbamazepine Medical Pollutants from Aqueous Environments by Multiwalled Carbon Nanotubes

Microplastics are ubiquitous in aquatic environments and interact with other kinds of pollutants, which affects the migration, transformation, and fate of those other pollutants. In this study, we employ carbamazepine (CBZ) as the contaminant to study the influence of polyethylene (PE) microplastics...

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Main Authors: Xiaoyu Sheng, Junkai Wang, Wei Zhang, Qiting Zuo
Format: Article
Language:English
Published: MDPI AG 2021-06-01
Series:Toxics
Subjects:
Online Access:https://www.mdpi.com/2305-6304/9/6/139
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author Xiaoyu Sheng
Junkai Wang
Wei Zhang
Qiting Zuo
author_facet Xiaoyu Sheng
Junkai Wang
Wei Zhang
Qiting Zuo
author_sort Xiaoyu Sheng
collection DOAJ
description Microplastics are ubiquitous in aquatic environments and interact with other kinds of pollutants, which affects the migration, transformation, and fate of those other pollutants. In this study, we employ carbamazepine (CBZ) as the contaminant to study the influence of polyethylene (PE) microplastics on the adsorption of CBZ pollutants by multiwalled carbon nanotubes (MCNTs) in aqueous solution. The adsorption capacity of CBZ by MCNTs in the presence of PE microplastics was obviously lower than that by MCNTs alone. The influencing factors, including the dose of microplastics, pH, and CBZ solution concentration, on the adsorption of CBZ by MCNTs and MCNTs−PE were thoroughly investigated. The adsorption rate of CBZ by MCNTs decreased from 97.4% to 90.6% as the PE microplastics dose increased from 2 g/L to 20 g/L. This decrease occurred because the MCNTs were coated on the surface of the PE microplastics, which further decreased the effective adsorption area of the MCNTs. This research provides a framework for revealing the effect of microplastics on the adsorption of pollutants by carbon materials in aqueous environments.
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spelling doaj.art-b7b8ff42446d4b748374d0d0d90aa0502023-11-21T23:52:21ZengMDPI AGToxics2305-63042021-06-019613910.3390/toxics9060139The Potential for PE Microplastics to Affect the Removal of Carbamazepine Medical Pollutants from Aqueous Environments by Multiwalled Carbon NanotubesXiaoyu Sheng0Junkai Wang1Wei Zhang2Qiting Zuo3School of Ecology and Environment, Zhengzhou University, 100 Kexue Avenue, Zhengzhou 450001, ChinaSchool of Ecology and Environment, Zhengzhou University, 100 Kexue Avenue, Zhengzhou 450001, ChinaSchool of Ecology and Environment, Zhengzhou University, 100 Kexue Avenue, Zhengzhou 450001, ChinaYellow River Institute for Ecological Protection & Regional Coordinated Development, Zhengzhou University, Zhengzhou 450001, ChinaMicroplastics are ubiquitous in aquatic environments and interact with other kinds of pollutants, which affects the migration, transformation, and fate of those other pollutants. In this study, we employ carbamazepine (CBZ) as the contaminant to study the influence of polyethylene (PE) microplastics on the adsorption of CBZ pollutants by multiwalled carbon nanotubes (MCNTs) in aqueous solution. The adsorption capacity of CBZ by MCNTs in the presence of PE microplastics was obviously lower than that by MCNTs alone. The influencing factors, including the dose of microplastics, pH, and CBZ solution concentration, on the adsorption of CBZ by MCNTs and MCNTs−PE were thoroughly investigated. The adsorption rate of CBZ by MCNTs decreased from 97.4% to 90.6% as the PE microplastics dose increased from 2 g/L to 20 g/L. This decrease occurred because the MCNTs were coated on the surface of the PE microplastics, which further decreased the effective adsorption area of the MCNTs. This research provides a framework for revealing the effect of microplastics on the adsorption of pollutants by carbon materials in aqueous environments.https://www.mdpi.com/2305-6304/9/6/139PE microplasticsmultiwalled carbon nanotubescarbamazepineadsorptionMCNTs−coated PE microplastics
spellingShingle Xiaoyu Sheng
Junkai Wang
Wei Zhang
Qiting Zuo
The Potential for PE Microplastics to Affect the Removal of Carbamazepine Medical Pollutants from Aqueous Environments by Multiwalled Carbon Nanotubes
Toxics
PE microplastics
multiwalled carbon nanotubes
carbamazepine
adsorption
MCNTs−coated PE microplastics
title The Potential for PE Microplastics to Affect the Removal of Carbamazepine Medical Pollutants from Aqueous Environments by Multiwalled Carbon Nanotubes
title_full The Potential for PE Microplastics to Affect the Removal of Carbamazepine Medical Pollutants from Aqueous Environments by Multiwalled Carbon Nanotubes
title_fullStr The Potential for PE Microplastics to Affect the Removal of Carbamazepine Medical Pollutants from Aqueous Environments by Multiwalled Carbon Nanotubes
title_full_unstemmed The Potential for PE Microplastics to Affect the Removal of Carbamazepine Medical Pollutants from Aqueous Environments by Multiwalled Carbon Nanotubes
title_short The Potential for PE Microplastics to Affect the Removal of Carbamazepine Medical Pollutants from Aqueous Environments by Multiwalled Carbon Nanotubes
title_sort potential for pe microplastics to affect the removal of carbamazepine medical pollutants from aqueous environments by multiwalled carbon nanotubes
topic PE microplastics
multiwalled carbon nanotubes
carbamazepine
adsorption
MCNTs−coated PE microplastics
url https://www.mdpi.com/2305-6304/9/6/139
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