On AC-Field-Induced Nonlinear Electroosmosis next to the Sharp Corner-Field-Singularity of Leaky Dielectric Blocks and Its Application in on-Chip Micro-Mixing

Induced-charge electroosmosis has attracted lots of attention from the microfluidic community over the past decade. Most previous researches on this subject focused on induced-charge electroosmosis (ICEO) vortex streaming actuated on ideally polarizable surfaces immersed in electrolyte solutions. St...

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Main Authors: Yukun Ren, Weiyu Liu, Ye Tao, Meng Hui, Qisheng Wu
Format: Article
Language:English
Published: MDPI AG 2018-02-01
Series:Micromachines
Subjects:
Online Access:http://www.mdpi.com/2072-666X/9/3/102
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author Yukun Ren
Weiyu Liu
Ye Tao
Meng Hui
Qisheng Wu
author_facet Yukun Ren
Weiyu Liu
Ye Tao
Meng Hui
Qisheng Wu
author_sort Yukun Ren
collection DOAJ
description Induced-charge electroosmosis has attracted lots of attention from the microfluidic community over the past decade. Most previous researches on this subject focused on induced-charge electroosmosis (ICEO) vortex streaming actuated on ideally polarizable surfaces immersed in electrolyte solutions. Starting from this point, we conduct herein a linear asymptotic analysis on nonlinear electroosmotic flow next to leaky dielectric blocks of arbitrary electrical conductivity and dielectric permittivity in harmonic AC electric fields, and theoretically demonstrate that observable ICEO fluid motion can be generated at high field frequencies in the vicinity of nearly insulating semiconductors, a very low electrical conductivity, of which can evidently increase the double-layer relaxation frequency (inversely proportional to the solid permittivity) to be much higher than the typical reciprocal RC time constant for induced double-layer charging on ideally polarizable surfaces. A computational model is developed to study the feasibility of this high-frequency vortex flow field of ICEO for sample mixing in microfluidics, in which the usage of AC voltage signal at high field frequencies may be beneficial to suppress electrochemical reactions to some extent. The influence of various parameters for developing an efficient mixer is investigated, and an integrated arrangement of semiconductor block array is suggested for achieving a reliable mixing performance at relatively high sample fluxes. Our physical demonstration with high-frequency ICEO next to leaky dielectric blocks using a simple channel structure offers valuable insights into the design of high-throughput micromixers for a variety of lab-on-a-chip applications.
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spelling doaj.art-b7f760c4e4bc4a88b650c1c5fa22264c2022-12-21T23:22:41ZengMDPI AGMicromachines2072-666X2018-02-019310210.3390/mi9030102mi9030102On AC-Field-Induced Nonlinear Electroosmosis next to the Sharp Corner-Field-Singularity of Leaky Dielectric Blocks and Its Application in on-Chip Micro-MixingYukun Ren0Weiyu Liu1Ye Tao2Meng Hui3Qisheng Wu4State Key Laboratory of Robotics and System, Harbin Institute of Technology, West Da-zhi Street 92, Harbin 150001, ChinaSchool of Electronics and Control Engineering, Chang’an University, Middle-Section of Nan’er Huan Road, Xi’an 710064, ChinaState Key Laboratory of Robotics and System, Harbin Institute of Technology, West Da-zhi Street 92, Harbin 150001, ChinaSchool of Electronics and Control Engineering, Chang’an University, Middle-Section of Nan’er Huan Road, Xi’an 710064, ChinaSchool of Electronics and Control Engineering, Chang’an University, Middle-Section of Nan’er Huan Road, Xi’an 710064, ChinaInduced-charge electroosmosis has attracted lots of attention from the microfluidic community over the past decade. Most previous researches on this subject focused on induced-charge electroosmosis (ICEO) vortex streaming actuated on ideally polarizable surfaces immersed in electrolyte solutions. Starting from this point, we conduct herein a linear asymptotic analysis on nonlinear electroosmotic flow next to leaky dielectric blocks of arbitrary electrical conductivity and dielectric permittivity in harmonic AC electric fields, and theoretically demonstrate that observable ICEO fluid motion can be generated at high field frequencies in the vicinity of nearly insulating semiconductors, a very low electrical conductivity, of which can evidently increase the double-layer relaxation frequency (inversely proportional to the solid permittivity) to be much higher than the typical reciprocal RC time constant for induced double-layer charging on ideally polarizable surfaces. A computational model is developed to study the feasibility of this high-frequency vortex flow field of ICEO for sample mixing in microfluidics, in which the usage of AC voltage signal at high field frequencies may be beneficial to suppress electrochemical reactions to some extent. The influence of various parameters for developing an efficient mixer is investigated, and an integrated arrangement of semiconductor block array is suggested for achieving a reliable mixing performance at relatively high sample fluxes. Our physical demonstration with high-frequency ICEO next to leaky dielectric blocks using a simple channel structure offers valuable insights into the design of high-throughput micromixers for a variety of lab-on-a-chip applications.http://www.mdpi.com/2072-666X/9/3/102micromixerinduced-charge electroosmosisleaky dielectric blockdebye screeningelectrochemical ion relaxationsharp corner-field-singularity
spellingShingle Yukun Ren
Weiyu Liu
Ye Tao
Meng Hui
Qisheng Wu
On AC-Field-Induced Nonlinear Electroosmosis next to the Sharp Corner-Field-Singularity of Leaky Dielectric Blocks and Its Application in on-Chip Micro-Mixing
Micromachines
micromixer
induced-charge electroosmosis
leaky dielectric block
debye screening
electrochemical ion relaxation
sharp corner-field-singularity
title On AC-Field-Induced Nonlinear Electroosmosis next to the Sharp Corner-Field-Singularity of Leaky Dielectric Blocks and Its Application in on-Chip Micro-Mixing
title_full On AC-Field-Induced Nonlinear Electroosmosis next to the Sharp Corner-Field-Singularity of Leaky Dielectric Blocks and Its Application in on-Chip Micro-Mixing
title_fullStr On AC-Field-Induced Nonlinear Electroosmosis next to the Sharp Corner-Field-Singularity of Leaky Dielectric Blocks and Its Application in on-Chip Micro-Mixing
title_full_unstemmed On AC-Field-Induced Nonlinear Electroosmosis next to the Sharp Corner-Field-Singularity of Leaky Dielectric Blocks and Its Application in on-Chip Micro-Mixing
title_short On AC-Field-Induced Nonlinear Electroosmosis next to the Sharp Corner-Field-Singularity of Leaky Dielectric Blocks and Its Application in on-Chip Micro-Mixing
title_sort on ac field induced nonlinear electroosmosis next to the sharp corner field singularity of leaky dielectric blocks and its application in on chip micro mixing
topic micromixer
induced-charge electroosmosis
leaky dielectric block
debye screening
electrochemical ion relaxation
sharp corner-field-singularity
url http://www.mdpi.com/2072-666X/9/3/102
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