One step upcycling CO2 from flue gas into CO using natural stone in an integrated CO2 capture and utilisation system
Natural marble was successfully applied in integrated CO2 capture and utilisation for selectively producing valuable CO. The cheap and easy-accessible marble dust is proven to have a high capacity of CO2 capture (9.4 mmol g−1) and be active in converting the captured CO2 into CO (> 85% CO2 conver...
| Main Authors: | , , , , |
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| Format: | Article |
| Language: | English |
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Elsevier
2022-12-01
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| Series: | Carbon Capture Science & Technology |
| Subjects: | |
| Online Access: | http://www.sciencedirect.com/science/article/pii/S2772656822000495 |
| _version_ | 1811295548517384192 |
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| author | Shuzhuang Sun Yuanyuan Wang Xiaotong Zhao Chen Zhang Chunfei Wu |
| author_facet | Shuzhuang Sun Yuanyuan Wang Xiaotong Zhao Chen Zhang Chunfei Wu |
| author_sort | Shuzhuang Sun |
| collection | DOAJ |
| description | Natural marble was successfully applied in integrated CO2 capture and utilisation for selectively producing valuable CO. The cheap and easy-accessible marble dust is proven to have a high capacity of CO2 capture (9.4 mmol g−1) and be active in converting the captured CO2 into CO (> 85% CO2 conversion at 650 °C) with almost 100% CO selectivity. Furthermore, the stone material exhibits impressive cycle stability (0.036 mmol g−1 decrease per cycle). This report demonstrates that carbon emission control and CO2 utilisation can be realised over a straightforward process using cheap and robust materials, representing an attractive technology for cost-effective low-carbon technology development. |
| first_indexed | 2024-04-13T05:35:10Z |
| format | Article |
| id | doaj.art-b8d76de936d8447bbb700d25fee1e286 |
| institution | Directory Open Access Journal |
| issn | 2772-6568 |
| language | English |
| last_indexed | 2024-04-13T05:35:10Z |
| publishDate | 2022-12-01 |
| publisher | Elsevier |
| record_format | Article |
| series | Carbon Capture Science & Technology |
| spelling | doaj.art-b8d76de936d8447bbb700d25fee1e2862022-12-22T03:00:19ZengElsevierCarbon Capture Science & Technology2772-65682022-12-015100078One step upcycling CO2 from flue gas into CO using natural stone in an integrated CO2 capture and utilisation systemShuzhuang Sun0Yuanyuan Wang1Xiaotong Zhao2Chen Zhang3Chunfei Wu4School of Chemistry and Chemical Engineering, Queen's University Belfast, Belfast BT7 1NN, UKSchool of Chemistry and Chemical Engineering, Queen's University Belfast, Belfast BT7 1NN, UKSchool of Chemistry and Chemical Engineering, Queen's University Belfast, Belfast BT7 1NN, UKSchool of Chemistry and Chemical Engineering, Queen's University Belfast, Belfast BT7 1NN, UKCorresponding author.; School of Chemistry and Chemical Engineering, Queen's University Belfast, Belfast BT7 1NN, UKNatural marble was successfully applied in integrated CO2 capture and utilisation for selectively producing valuable CO. The cheap and easy-accessible marble dust is proven to have a high capacity of CO2 capture (9.4 mmol g−1) and be active in converting the captured CO2 into CO (> 85% CO2 conversion at 650 °C) with almost 100% CO selectivity. Furthermore, the stone material exhibits impressive cycle stability (0.036 mmol g−1 decrease per cycle). This report demonstrates that carbon emission control and CO2 utilisation can be realised over a straightforward process using cheap and robust materials, representing an attractive technology for cost-effective low-carbon technology development.http://www.sciencedirect.com/science/article/pii/S2772656822000495Carbon captureIntegrated CO2 capture and utilisationCO2 conversionReverse water gas shift reaction |
| spellingShingle | Shuzhuang Sun Yuanyuan Wang Xiaotong Zhao Chen Zhang Chunfei Wu One step upcycling CO2 from flue gas into CO using natural stone in an integrated CO2 capture and utilisation system Carbon Capture Science & Technology Carbon capture Integrated CO2 capture and utilisation CO2 conversion Reverse water gas shift reaction |
| title | One step upcycling CO2 from flue gas into CO using natural stone in an integrated CO2 capture and utilisation system |
| title_full | One step upcycling CO2 from flue gas into CO using natural stone in an integrated CO2 capture and utilisation system |
| title_fullStr | One step upcycling CO2 from flue gas into CO using natural stone in an integrated CO2 capture and utilisation system |
| title_full_unstemmed | One step upcycling CO2 from flue gas into CO using natural stone in an integrated CO2 capture and utilisation system |
| title_short | One step upcycling CO2 from flue gas into CO using natural stone in an integrated CO2 capture and utilisation system |
| title_sort | one step upcycling co2 from flue gas into co using natural stone in an integrated co2 capture and utilisation system |
| topic | Carbon capture Integrated CO2 capture and utilisation CO2 conversion Reverse water gas shift reaction |
| url | http://www.sciencedirect.com/science/article/pii/S2772656822000495 |
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