Observation of exchange bias in nanoscale AuFe alloy film

We report on observation of the exchange bias effect in AuFe co-sputtered alloy films in the as-deposited state and following swift heavy ion irradiation. The Mössbauer spectrum for the as-deposited film shows a broad paramagnetic doublet together with a small contribution from hyperfine magnetic se...

Full description

Bibliographic Details
Main Authors: Compesh Pannu, Santanu Ghosh, Pankaj Srivastava, K Bharuth-Ram, V R Reddy, Ajay Gupta, Debdulal Kabiraj, D K Avasthi
Format: Article
Language:English
Published: IOP Publishing 2020-01-01
Series:Materials Research Express
Subjects:
Online Access:https://doi.org/10.1088/2053-1591/aba061
_version_ 1797746290231083008
author Compesh Pannu
Santanu Ghosh
Pankaj Srivastava
K Bharuth-Ram
V R Reddy
Ajay Gupta
Debdulal Kabiraj
D K Avasthi
author_facet Compesh Pannu
Santanu Ghosh
Pankaj Srivastava
K Bharuth-Ram
V R Reddy
Ajay Gupta
Debdulal Kabiraj
D K Avasthi
author_sort Compesh Pannu
collection DOAJ
description We report on observation of the exchange bias effect in AuFe co-sputtered alloy films in the as-deposited state and following swift heavy ion irradiation. The Mössbauer spectrum for the as-deposited film shows a broad paramagnetic doublet together with a small contribution from hyperfine magnetic sextets. The magnetization behavior exhibits a spontaneous exchange bias effect at room temperature without application of an external triggering field. The magnitude of exchange bias in the as-deposited sample increases with decreasing temperature, at first gradually down to about 50 K and then more rapidly down to 5 K. Irradiation of AuFe film with 100 MeV Au ^9+ ions transforms the Mössbauer spectrum into a broad magnetic sextet, with asymmetric broadening characteristic of the formation of α-Fe magnetic nanoclusters surrounded by shells of reduced Fe concentration. At room temperature the exchange bias field is in the same sense as that for the as-deposited sample, but decreases with temperature until it reverse its sign at below about 50 K. In both the as-deposited and irradiated samples a well-defined uniaxial magnetic anisotropy, consequent on a stress induced texturing of the Fe precipitate distribution, is observed.
first_indexed 2024-03-12T15:34:42Z
format Article
id doaj.art-b8dc54c036244da8bd178de42aa8b65d
institution Directory Open Access Journal
issn 2053-1591
language English
last_indexed 2024-03-12T15:34:42Z
publishDate 2020-01-01
publisher IOP Publishing
record_format Article
series Materials Research Express
spelling doaj.art-b8dc54c036244da8bd178de42aa8b65d2023-08-09T16:17:15ZengIOP PublishingMaterials Research Express2053-15912020-01-017707610210.1088/2053-1591/aba061Observation of exchange bias in nanoscale AuFe alloy filmCompesh Pannu0https://orcid.org/0000-0002-3783-555XSantanu Ghosh1https://orcid.org/0000-0002-5518-5837Pankaj Srivastava2https://orcid.org/0000-0001-8063-6209K Bharuth-Ram3V R Reddy4Ajay Gupta5https://orcid.org/0000-0002-4430-6875Debdulal Kabiraj6D K Avasthi7Nanostech Laboratory, Department of Physics, Indian Institute of Technology Delhi , New Delhi–110016, IndiaNanostech Laboratory, Department of Physics, Indian Institute of Technology Delhi , New Delhi–110016, IndiaNanostech Laboratory, Department of Physics, Indian Institute of Technology Delhi , New Delhi–110016, IndiaPhysics Department, Durban University of Technology , Durban–4000, South Africa; School of Chemistry and Physics, University of KwaZulu-Natal , Durban–4041, South AfricaUGC-DAE Consortium for Scientific Research, University Campus , Khandwa Road, Indore–452 017, IndiaAmity Centre for Spintronics Materials, Amity University , Noida, Uttar Pardesh–201313, IndiaInter University Accelerator Centre, New Delhi–110067, IndiaAmity Centre for Advance Research and Innovation, Amity University , Noida, Uttar Pardesh–201313, India; Amity Centre of Accelerator based Fundamental and Applied Research, Amity University , Noida–201313, Uttar Pardesh, IndiaWe report on observation of the exchange bias effect in AuFe co-sputtered alloy films in the as-deposited state and following swift heavy ion irradiation. The Mössbauer spectrum for the as-deposited film shows a broad paramagnetic doublet together with a small contribution from hyperfine magnetic sextets. The magnetization behavior exhibits a spontaneous exchange bias effect at room temperature without application of an external triggering field. The magnitude of exchange bias in the as-deposited sample increases with decreasing temperature, at first gradually down to about 50 K and then more rapidly down to 5 K. Irradiation of AuFe film with 100 MeV Au ^9+ ions transforms the Mössbauer spectrum into a broad magnetic sextet, with asymmetric broadening characteristic of the formation of α-Fe magnetic nanoclusters surrounded by shells of reduced Fe concentration. At room temperature the exchange bias field is in the same sense as that for the as-deposited sample, but decreases with temperature until it reverse its sign at below about 50 K. In both the as-deposited and irradiated samples a well-defined uniaxial magnetic anisotropy, consequent on a stress induced texturing of the Fe precipitate distribution, is observed.https://doi.org/10.1088/2053-1591/aba061magnetizationexchange biasion beam irradiationswift heavy ionsalloys
spellingShingle Compesh Pannu
Santanu Ghosh
Pankaj Srivastava
K Bharuth-Ram
V R Reddy
Ajay Gupta
Debdulal Kabiraj
D K Avasthi
Observation of exchange bias in nanoscale AuFe alloy film
Materials Research Express
magnetization
exchange bias
ion beam irradiation
swift heavy ions
alloys
title Observation of exchange bias in nanoscale AuFe alloy film
title_full Observation of exchange bias in nanoscale AuFe alloy film
title_fullStr Observation of exchange bias in nanoscale AuFe alloy film
title_full_unstemmed Observation of exchange bias in nanoscale AuFe alloy film
title_short Observation of exchange bias in nanoscale AuFe alloy film
title_sort observation of exchange bias in nanoscale aufe alloy film
topic magnetization
exchange bias
ion beam irradiation
swift heavy ions
alloys
url https://doi.org/10.1088/2053-1591/aba061
work_keys_str_mv AT compeshpannu observationofexchangebiasinnanoscaleaufealloyfilm
AT santanughosh observationofexchangebiasinnanoscaleaufealloyfilm
AT pankajsrivastava observationofexchangebiasinnanoscaleaufealloyfilm
AT kbharuthram observationofexchangebiasinnanoscaleaufealloyfilm
AT vrreddy observationofexchangebiasinnanoscaleaufealloyfilm
AT ajaygupta observationofexchangebiasinnanoscaleaufealloyfilm
AT debdulalkabiraj observationofexchangebiasinnanoscaleaufealloyfilm
AT dkavasthi observationofexchangebiasinnanoscaleaufealloyfilm