Hydrogels as Durable Anti-Icing Coatings Inhibit and Delay Ice Nucleation

The accumulation of ice on surfaces brings dangerous and costly problems to our daily life. Thus, it would be desirable to design anti-icing coatings for various surfaces. We report a durable anti-icing coating based on mussel-inspired chemistry, which is enabled via fabricating a liquid water layer...

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Main Authors: Beili Huang, Shanshan Jiang, Yunhe Diao, Xuying Liu, Wentao Liu, Jinzhou Chen, Huige Yang
Format: Article
Language:English
Published: MDPI AG 2020-07-01
Series:Molecules
Subjects:
Online Access:https://www.mdpi.com/1420-3049/25/15/3378
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author Beili Huang
Shanshan Jiang
Yunhe Diao
Xuying Liu
Wentao Liu
Jinzhou Chen
Huige Yang
author_facet Beili Huang
Shanshan Jiang
Yunhe Diao
Xuying Liu
Wentao Liu
Jinzhou Chen
Huige Yang
author_sort Beili Huang
collection DOAJ
description The accumulation of ice on surfaces brings dangerous and costly problems to our daily life. Thus, it would be desirable to design anti-icing coatings for various surfaces. We report a durable anti-icing coating based on mussel-inspired chemistry, which is enabled via fabricating a liquid water layer, achieved by modifying solid substrates with the highly water absorbing property of sodium alginate. Dopamine, the main component of the mussel adhesive protein, is introduced to anchor the sodium alginate in order to render the coating applicable to all types of solid surfaces. Simultaneously, it serves as the cross-linking agent for sodium alginate; thus, the cross-linking degree of the coatings could be easily varied. The non-freezable and freezable water in the coatings with different cross-link degrees all remain liquid-like at subzero conditions and synergistically fulfill the aim of decreasing the temperature of ice nucleation. These anti-icing coatings display excellent stability even under harsh conditions. Furthermore, these coatings can be applied to almost all types of solid surfaces and have great promise in practical applications.
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spelling doaj.art-bad43a44b1af4292a58bbee1432cac6b2023-11-20T07:57:08ZengMDPI AGMolecules1420-30492020-07-012515337810.3390/molecules25153378Hydrogels as Durable Anti-Icing Coatings Inhibit and Delay Ice NucleationBeili Huang0Shanshan Jiang1Yunhe Diao2Xuying Liu3Wentao Liu4Jinzhou Chen5Huige Yang6School of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, Henan, ChinaSchool of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, Henan, ChinaSchool of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, Henan, ChinaSchool of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, Henan, ChinaSchool of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, Henan, ChinaSchool of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, Henan, ChinaSchool of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, Henan, ChinaThe accumulation of ice on surfaces brings dangerous and costly problems to our daily life. Thus, it would be desirable to design anti-icing coatings for various surfaces. We report a durable anti-icing coating based on mussel-inspired chemistry, which is enabled via fabricating a liquid water layer, achieved by modifying solid substrates with the highly water absorbing property of sodium alginate. Dopamine, the main component of the mussel adhesive protein, is introduced to anchor the sodium alginate in order to render the coating applicable to all types of solid surfaces. Simultaneously, it serves as the cross-linking agent for sodium alginate; thus, the cross-linking degree of the coatings could be easily varied. The non-freezable and freezable water in the coatings with different cross-link degrees all remain liquid-like at subzero conditions and synergistically fulfill the aim of decreasing the temperature of ice nucleation. These anti-icing coatings display excellent stability even under harsh conditions. Furthermore, these coatings can be applied to almost all types of solid surfaces and have great promise in practical applications.https://www.mdpi.com/1420-3049/25/15/3378anti-icing coatinghydrogelscross-linkingsodium alginate
spellingShingle Beili Huang
Shanshan Jiang
Yunhe Diao
Xuying Liu
Wentao Liu
Jinzhou Chen
Huige Yang
Hydrogels as Durable Anti-Icing Coatings Inhibit and Delay Ice Nucleation
Molecules
anti-icing coating
hydrogels
cross-linking
sodium alginate
title Hydrogels as Durable Anti-Icing Coatings Inhibit and Delay Ice Nucleation
title_full Hydrogels as Durable Anti-Icing Coatings Inhibit and Delay Ice Nucleation
title_fullStr Hydrogels as Durable Anti-Icing Coatings Inhibit and Delay Ice Nucleation
title_full_unstemmed Hydrogels as Durable Anti-Icing Coatings Inhibit and Delay Ice Nucleation
title_short Hydrogels as Durable Anti-Icing Coatings Inhibit and Delay Ice Nucleation
title_sort hydrogels as durable anti icing coatings inhibit and delay ice nucleation
topic anti-icing coating
hydrogels
cross-linking
sodium alginate
url https://www.mdpi.com/1420-3049/25/15/3378
work_keys_str_mv AT beilihuang hydrogelsasdurableantiicingcoatingsinhibitanddelayicenucleation
AT shanshanjiang hydrogelsasdurableantiicingcoatingsinhibitanddelayicenucleation
AT yunhediao hydrogelsasdurableantiicingcoatingsinhibitanddelayicenucleation
AT xuyingliu hydrogelsasdurableantiicingcoatingsinhibitanddelayicenucleation
AT wentaoliu hydrogelsasdurableantiicingcoatingsinhibitanddelayicenucleation
AT jinzhouchen hydrogelsasdurableantiicingcoatingsinhibitanddelayicenucleation
AT huigeyang hydrogelsasdurableantiicingcoatingsinhibitanddelayicenucleation