Observation of secondary ice production in clouds at low temperatures

<p>Ice particles play an important role in precipitation formation and radiation balance. Therefore, an accurate description of ice initiation in the atmosphere is of great importance for weather prediction models and climate simulations. Despite the abundance of ice crystals in the atmosphere...

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Main Authors: A. Korolev, P. J. DeMott, I. Heckman, M. Wolde, E. Williams, D. J. Smalley, M. F. Donovan
Format: Article
Language:English
Published: Copernicus Publications 2022-10-01
Series:Atmospheric Chemistry and Physics
Online Access:https://acp.copernicus.org/articles/22/13103/2022/acp-22-13103-2022.pdf
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author A. Korolev
P. J. DeMott
I. Heckman
M. Wolde
E. Williams
D. J. Smalley
M. F. Donovan
author_facet A. Korolev
P. J. DeMott
I. Heckman
M. Wolde
E. Williams
D. J. Smalley
M. F. Donovan
author_sort A. Korolev
collection DOAJ
description <p>Ice particles play an important role in precipitation formation and radiation balance. Therefore, an accurate description of ice initiation in the atmosphere is of great importance for weather prediction models and climate simulations. Despite the abundance of ice crystals in the atmosphere, the mechanisms for their formation remain not well understood. There are two major sets of mechanisms of ice initiation in the atmosphere: primary nucleation and secondary ice production. Secondary ice production occurs in the presence of preexisting ice, which results in an enhancement of the concentration of ice particles. Until recently, secondary ice production was mainly attributed to the rime-splintering mechanism, known as the Hallett–Mossop process, which is active in a relatively narrow temperature range from <span class="inline-formula">−3</span> to <span class="inline-formula">−8</span> <span class="inline-formula"><sup>∘</sup></span>C. The existence of the Hallett–Mossop process was well supported by in situ observations. The present study provides an explicit in situ observation of secondary ice production at temperatures as low as <span class="inline-formula">−27</span> <span class="inline-formula"><sup>∘</sup></span>C, which is well outside the range of the Hallett–Mossop process. This observation expands our knowledge of the temperature range of initiation of secondary ice in clouds. The obtained results are intended to stimulate laboratory and theoretical studies to develop physically based parameterizations for weather prediction and climate models.</p>
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spelling doaj.art-bad4970dfad641bd89daf21449deff262022-12-22T02:33:41ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242022-10-0122131031311310.5194/acp-22-13103-2022Observation of secondary ice production in clouds at low temperaturesA. Korolev0P. J. DeMott1I. Heckman2M. Wolde3E. Williams4D. J. Smalley5M. F. Donovan6Meteorological Research Division, Environment and Climate Change Canada, Toronto, ON, CanadaDepartment of Atmospheric Science, Colorado State University, Fort Collins, CO, USAMeteorological Research Division, Environment and Climate Change Canada, Toronto, ON, CanadaAerospace Research Centre, National Research Council Canada, Ottawa, ON, CanadaDepartment of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USALincoln Laboratory, Massachusetts Institute of Technology, Lexington, MA, USALincoln Laboratory, Massachusetts Institute of Technology, Lexington, MA, USA<p>Ice particles play an important role in precipitation formation and radiation balance. Therefore, an accurate description of ice initiation in the atmosphere is of great importance for weather prediction models and climate simulations. Despite the abundance of ice crystals in the atmosphere, the mechanisms for their formation remain not well understood. There are two major sets of mechanisms of ice initiation in the atmosphere: primary nucleation and secondary ice production. Secondary ice production occurs in the presence of preexisting ice, which results in an enhancement of the concentration of ice particles. Until recently, secondary ice production was mainly attributed to the rime-splintering mechanism, known as the Hallett–Mossop process, which is active in a relatively narrow temperature range from <span class="inline-formula">−3</span> to <span class="inline-formula">−8</span> <span class="inline-formula"><sup>∘</sup></span>C. The existence of the Hallett–Mossop process was well supported by in situ observations. The present study provides an explicit in situ observation of secondary ice production at temperatures as low as <span class="inline-formula">−27</span> <span class="inline-formula"><sup>∘</sup></span>C, which is well outside the range of the Hallett–Mossop process. This observation expands our knowledge of the temperature range of initiation of secondary ice in clouds. The obtained results are intended to stimulate laboratory and theoretical studies to develop physically based parameterizations for weather prediction and climate models.</p>https://acp.copernicus.org/articles/22/13103/2022/acp-22-13103-2022.pdf
spellingShingle A. Korolev
P. J. DeMott
I. Heckman
M. Wolde
E. Williams
D. J. Smalley
M. F. Donovan
Observation of secondary ice production in clouds at low temperatures
Atmospheric Chemistry and Physics
title Observation of secondary ice production in clouds at low temperatures
title_full Observation of secondary ice production in clouds at low temperatures
title_fullStr Observation of secondary ice production in clouds at low temperatures
title_full_unstemmed Observation of secondary ice production in clouds at low temperatures
title_short Observation of secondary ice production in clouds at low temperatures
title_sort observation of secondary ice production in clouds at low temperatures
url https://acp.copernicus.org/articles/22/13103/2022/acp-22-13103-2022.pdf
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