Self‐Charging Persistent Mechanoluminescence with Mechanics Storage and Visualization Activities
Abstract Persistent mechanoluminescence (ML) with long lifetime is highly required to break the limits of the transient emitting behavior under mechanics stimuli. However, the existing materials with persistent ML are completely trap‐controlled, and a pre‐irradiation is required, which severely hind...
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Format: | Article |
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Wiley
2022-10-01
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Series: | Advanced Science |
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Online Access: | https://doi.org/10.1002/advs.202203249 |
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author | Yongqing Bai Xiuping Guo Birong Tian Yongmin Liang Dengfeng Peng Zhaofeng Wang |
author_facet | Yongqing Bai Xiuping Guo Birong Tian Yongmin Liang Dengfeng Peng Zhaofeng Wang |
author_sort | Yongqing Bai |
collection | DOAJ |
description | Abstract Persistent mechanoluminescence (ML) with long lifetime is highly required to break the limits of the transient emitting behavior under mechanics stimuli. However, the existing materials with persistent ML are completely trap‐controlled, and a pre‐irradiation is required, which severely hinders the practical applications. In this work, a novel type of ML, self‐charging persistent ML, is created by compositing the Sr3Al2O5Cl2:Dy3+ (SAOCD) powders into flexible polydimethylsiloxane (PDMS) matrix. With no need for any pre‐irradiation, the as‐fabricated SAOCD/PDMS elastomer could exhibit intense and persistent ML under mechanics stimuli directly, which greatly facilitates its applications in mechanics lighting, displaying, imaging, and visualization. By investigating the matrix effects as well as the thermoluminescence, cathodoluminescence, and triboelectricity properties, the interfacial triboelectrification‐induced electron bombardment processes are demonstrated to be responsible for the self‐charged energy in SAOCD under mechanics stimuli. Based on the unique self‐charging processes, the SAOCD/PDMS further exhibits mechanics storage and visualized reading activities, which brings novel ideas and approaches to deal with the mechanics‐related problems in the fields of mechanical engineering, bioengineering, and artificial intelligence. |
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id | doaj.art-baf1ce5f8f6f4e36b98c0b17494335e7 |
institution | Directory Open Access Journal |
issn | 2198-3844 |
language | English |
last_indexed | 2024-04-11T10:28:18Z |
publishDate | 2022-10-01 |
publisher | Wiley |
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series | Advanced Science |
spelling | doaj.art-baf1ce5f8f6f4e36b98c0b17494335e72022-12-22T04:29:29ZengWileyAdvanced Science2198-38442022-10-01928n/an/a10.1002/advs.202203249Self‐Charging Persistent Mechanoluminescence with Mechanics Storage and Visualization ActivitiesYongqing Bai0Xiuping Guo1Birong Tian2Yongmin Liang3Dengfeng Peng4Zhaofeng Wang5State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical Physics Chinese Academy of Sciences Lanzhou 730000 ChinaState Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical Physics Chinese Academy of Sciences Lanzhou 730000 ChinaState Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical Physics Chinese Academy of Sciences Lanzhou 730000 ChinaState Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical Engineering Lanzhou University Lanzhou Gansu 730000 ChinaKey Laboratory of Optoelectronic Devices and Systems of the Ministry of Education and Guangdong Province College of Physics and Optoelectronic Engineering Shenzhen University Shenzhen 518060 ChinaState Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical Physics Chinese Academy of Sciences Lanzhou 730000 ChinaAbstract Persistent mechanoluminescence (ML) with long lifetime is highly required to break the limits of the transient emitting behavior under mechanics stimuli. However, the existing materials with persistent ML are completely trap‐controlled, and a pre‐irradiation is required, which severely hinders the practical applications. In this work, a novel type of ML, self‐charging persistent ML, is created by compositing the Sr3Al2O5Cl2:Dy3+ (SAOCD) powders into flexible polydimethylsiloxane (PDMS) matrix. With no need for any pre‐irradiation, the as‐fabricated SAOCD/PDMS elastomer could exhibit intense and persistent ML under mechanics stimuli directly, which greatly facilitates its applications in mechanics lighting, displaying, imaging, and visualization. By investigating the matrix effects as well as the thermoluminescence, cathodoluminescence, and triboelectricity properties, the interfacial triboelectrification‐induced electron bombardment processes are demonstrated to be responsible for the self‐charged energy in SAOCD under mechanics stimuli. Based on the unique self‐charging processes, the SAOCD/PDMS further exhibits mechanics storage and visualized reading activities, which brings novel ideas and approaches to deal with the mechanics‐related problems in the fields of mechanical engineering, bioengineering, and artificial intelligence.https://doi.org/10.1002/advs.202203249mechanics storagemechanics visualizationpersistent mechanoluminescenceself‐charging materials |
spellingShingle | Yongqing Bai Xiuping Guo Birong Tian Yongmin Liang Dengfeng Peng Zhaofeng Wang Self‐Charging Persistent Mechanoluminescence with Mechanics Storage and Visualization Activities Advanced Science mechanics storage mechanics visualization persistent mechanoluminescence self‐charging materials |
title | Self‐Charging Persistent Mechanoluminescence with Mechanics Storage and Visualization Activities |
title_full | Self‐Charging Persistent Mechanoluminescence with Mechanics Storage and Visualization Activities |
title_fullStr | Self‐Charging Persistent Mechanoluminescence with Mechanics Storage and Visualization Activities |
title_full_unstemmed | Self‐Charging Persistent Mechanoluminescence with Mechanics Storage and Visualization Activities |
title_short | Self‐Charging Persistent Mechanoluminescence with Mechanics Storage and Visualization Activities |
title_sort | self charging persistent mechanoluminescence with mechanics storage and visualization activities |
topic | mechanics storage mechanics visualization persistent mechanoluminescence self‐charging materials |
url | https://doi.org/10.1002/advs.202203249 |
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