Spin photogalvanic effect in two-dimensional collinear antiferromagnets

Abstract Recent discovered two-dimensional (2D) antiferromagnetic (AFM) van der Waals quantum materials have attracted increasing interest due to the emergent exotic physical phenomena. The spintronic properties utilizing the intrinsic AFM state in 2D antiferromagnets, however, have been rarely foun...

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Main Authors: Rui-Chun Xiao, Ding-Fu Shao, Yu-Hang Li, Hua Jiang
Format: Article
Language:English
Published: Nature Portfolio 2021-04-01
Series:npj Quantum Materials
Online Access:https://doi.org/10.1038/s41535-021-00334-5
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author Rui-Chun Xiao
Ding-Fu Shao
Yu-Hang Li
Hua Jiang
author_facet Rui-Chun Xiao
Ding-Fu Shao
Yu-Hang Li
Hua Jiang
author_sort Rui-Chun Xiao
collection DOAJ
description Abstract Recent discovered two-dimensional (2D) antiferromagnetic (AFM) van der Waals quantum materials have attracted increasing interest due to the emergent exotic physical phenomena. The spintronic properties utilizing the intrinsic AFM state in 2D antiferromagnets, however, have been rarely found. Here we show that the spin photogalvanic effect (SPGE), which has been predicted in three-dimensional (3D) antiferromagnets, can intrinsically emerge in 2D antiferromagnets for promising spintronic applications. Based on the symmetry analysis of possible AFM orders in the honeycomb lattice, we conclude suitable 2D AFM candidate materials for realizing the SPGE. We choose two experimentally synthesized 2D collinear AFM materials, monolayer MnPS3, and bilayer CrCl3, as representative materials to perform first-principles calculations, and find that they support sizable SPGE. The SPGE in collinear 2D AFM materials can be utilized to generate pure spin current in a contactless and ultra-fast way.
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spelling doaj.art-bca022a8451243f097d8527ffcfdae2c2022-12-21T22:55:13ZengNature Portfolionpj Quantum Materials2397-46482021-04-01611610.1038/s41535-021-00334-5Spin photogalvanic effect in two-dimensional collinear antiferromagnetsRui-Chun Xiao0Ding-Fu Shao1Yu-Hang Li2Hua Jiang3Institute of Physical Science and Information Technology, Anhui UniversityDepartment of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of NebraskaDepartment of Electrical and Computer Engineering, University of CaliforniaSchool of Physical Science and Technology, Soochow UniversityAbstract Recent discovered two-dimensional (2D) antiferromagnetic (AFM) van der Waals quantum materials have attracted increasing interest due to the emergent exotic physical phenomena. The spintronic properties utilizing the intrinsic AFM state in 2D antiferromagnets, however, have been rarely found. Here we show that the spin photogalvanic effect (SPGE), which has been predicted in three-dimensional (3D) antiferromagnets, can intrinsically emerge in 2D antiferromagnets for promising spintronic applications. Based on the symmetry analysis of possible AFM orders in the honeycomb lattice, we conclude suitable 2D AFM candidate materials for realizing the SPGE. We choose two experimentally synthesized 2D collinear AFM materials, monolayer MnPS3, and bilayer CrCl3, as representative materials to perform first-principles calculations, and find that they support sizable SPGE. The SPGE in collinear 2D AFM materials can be utilized to generate pure spin current in a contactless and ultra-fast way.https://doi.org/10.1038/s41535-021-00334-5
spellingShingle Rui-Chun Xiao
Ding-Fu Shao
Yu-Hang Li
Hua Jiang
Spin photogalvanic effect in two-dimensional collinear antiferromagnets
npj Quantum Materials
title Spin photogalvanic effect in two-dimensional collinear antiferromagnets
title_full Spin photogalvanic effect in two-dimensional collinear antiferromagnets
title_fullStr Spin photogalvanic effect in two-dimensional collinear antiferromagnets
title_full_unstemmed Spin photogalvanic effect in two-dimensional collinear antiferromagnets
title_short Spin photogalvanic effect in two-dimensional collinear antiferromagnets
title_sort spin photogalvanic effect in two dimensional collinear antiferromagnets
url https://doi.org/10.1038/s41535-021-00334-5
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AT yuhangli spinphotogalvaniceffectintwodimensionalcollinearantiferromagnets
AT huajiang spinphotogalvaniceffectintwodimensionalcollinearantiferromagnets