Updated trends of the stratospheric ozone vertical distribution in the 60° S–60° N latitude range based on the LOTUS regression model

<p>This study presents an updated evaluation of stratospheric ozone profile trends in the 60<span class="inline-formula"><sup>∘</sup></span> S–60<span class="inline-formula"><sup>∘</sup></span> N latitude range over the 2000–2...

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Main Authors: S. Godin-Beekmann, N. Azouz, V. F. Sofieva, D. Hubert, I. Petropavlovskikh, P. Effertz, G. Ancellet, D. A. Degenstein, D. Zawada, L. Froidevaux, S. Frith, J. Wild, S. Davis, W. Steinbrecht, T. Leblanc, R. Querel, K. Tourpali, R. Damadeo, E. Maillard Barras, R. Stübi, C. Vigouroux, C. Arosio, G. Nedoluha, I. Boyd, R. Van Malderen, E. Mahieu, D. Smale, R. Sussmann
Format: Article
Language:English
Published: Copernicus Publications 2022-09-01
Series:Atmospheric Chemistry and Physics
Online Access:https://acp.copernicus.org/articles/22/11657/2022/acp-22-11657-2022.pdf
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author S. Godin-Beekmann
N. Azouz
V. F. Sofieva
D. Hubert
I. Petropavlovskikh
P. Effertz
G. Ancellet
D. A. Degenstein
D. Zawada
L. Froidevaux
S. Frith
J. Wild
S. Davis
W. Steinbrecht
T. Leblanc
R. Querel
K. Tourpali
R. Damadeo
E. Maillard Barras
R. Stübi
C. Vigouroux
C. Arosio
G. Nedoluha
I. Boyd
R. Van Malderen
E. Mahieu
D. Smale
R. Sussmann
author_facet S. Godin-Beekmann
N. Azouz
V. F. Sofieva
D. Hubert
I. Petropavlovskikh
P. Effertz
G. Ancellet
D. A. Degenstein
D. Zawada
L. Froidevaux
S. Frith
J. Wild
S. Davis
W. Steinbrecht
T. Leblanc
R. Querel
K. Tourpali
R. Damadeo
E. Maillard Barras
R. Stübi
C. Vigouroux
C. Arosio
G. Nedoluha
I. Boyd
R. Van Malderen
E. Mahieu
D. Smale
R. Sussmann
author_sort S. Godin-Beekmann
collection DOAJ
description <p>This study presents an updated evaluation of stratospheric ozone profile trends in the 60<span class="inline-formula"><sup>∘</sup></span> S–60<span class="inline-formula"><sup>∘</sup></span> N latitude range over the 2000–2020 period using an updated version of the Long-term Ozone Trends and Uncertainties in the Stratosphere (LOTUS) regression model that was used to evaluate such trends up to 2016 for the last WMO Ozone Assessment (2018). In addition to the derivation of detailed trends as a function of latitude and vertical coordinates, the regressions are performed with the datasets averaged over broad latitude bands, i.e. 60–35<span class="inline-formula"><sup>∘</sup></span> S, 20<span class="inline-formula"><sup>∘</sup></span> S–20<span class="inline-formula"><sup>∘</sup></span> N and 35–60<span class="inline-formula"><sup>∘</sup></span> N. The same methodology as in the last assessment is applied to combine trends in these broad latitude bands in order to compare the results with the previous studies. Longitudinally resolved merged satellite records are also considered in order to provide a better comparison with trends retrieved from ground-based records, e.g. lidar, ozonesondes, Umkehr, microwave and Fourier transform infrared (FTIR) spectrometers at selected stations where long-term time series are available. The study includes a comparison with trends derived from the REF-C2 simulations of the Chemistry Climate Model Initiative (CCMI-1). This work confirms past results showing an ozone increase in the upper stratosphere, which is now significant in the three broad latitude bands. The increase is largest in the Northern and Southern Hemisphere midlatitudes, with <span class="inline-formula">∼2.2</span> <span class="inline-formula">±</span> 0.7 % per decade at <span class="inline-formula">∼2.1</span> hPa and <span class="inline-formula">∼2.1</span> <span class="inline-formula">±</span> 0.6 % per decade at <span class="inline-formula">∼3.2</span> hPa respectively compared to <span class="inline-formula">∼1.6</span> <span class="inline-formula">±</span> 0.6 % per decade at <span class="inline-formula">∼2.6</span> hPa in the tropics. New trend signals have emerged from the records, such as a significant decrease in ozone in the tropics around 35 hPa and a non-significant increase in ozone in the southern midlatitudes at about 20 hPa. Non-significant negative ozone trends are derived in the lowermost stratosphere, with the most pronounced trends in the tropics. While a very good agreement is obtained between trends from merged satellite records and the CCMI-1 REF-C2 simulation in the upper stratosphere, observed negative trends in the lower stratosphere are not reproduced by models at southern and, in particular, at northern midlatitudes, where models report an ozone increase. However, the lower-stratospheric trend uncertainties are quite large, for both measured and modelled trends. Finally, 2000–2020 stratospheric ozone trends derived from the ground-based and longitudinally resolved satellite records are in reasonable agreement over the European Alpine and tropical regions, while at the Lauder station in the Southern Hemisphere midlatitudes they show some differences.</p>
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spelling doaj.art-bd187cf485834713ab837ef740cd1fb72022-12-22T04:24:42ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242022-09-0122116571167310.5194/acp-22-11657-2022Updated trends of the stratospheric ozone vertical distribution in the 60°&thinsp;S–60°&thinsp;N latitude range based on the LOTUS regression model S. Godin-Beekmann0N. Azouz1V. F. Sofieva2D. Hubert3I. Petropavlovskikh4P. Effertz5G. Ancellet6D. A. Degenstein7D. Zawada8L. Froidevaux9S. Frith10J. Wild11S. Davis12W. Steinbrecht13T. Leblanc14R. Querel15K. Tourpali16R. Damadeo17E. Maillard Barras18R. Stübi19C. Vigouroux20C. Arosio21G. Nedoluha22I. Boyd23R. Van Malderen24E. Mahieu25D. Smale26R. Sussmann27LATMOS, Sorbonne Université, UVSQ, CNRS, Paris, FranceLATMOS, Sorbonne Université, UVSQ, CNRS, Paris, FranceFinnish Meteorological Institute, Helsinki, FinlandRoyal Belgian Institute for Space Aeronomy (BIRA-IASB), Uccle, BelgiumCooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USACooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USALATMOS, Sorbonne Université, UVSQ, CNRS, Paris, FranceUniversity of Saskatchewan, Saskatun, CanadaUniversity of Saskatchewan, Saskatun, CanadaJet Propulsion Laboratory, California Institute of Technology, Pasadena, CA, USAScience Systems and Applications, Inc & NASA Goddard Space Flight Center, Greenbelt, MA, USAESSIC/UMD & NOAA/NESDIS/STAR, College Park, MD, USANOAA Chemical Sciences Laboratory, Boulder, CO, USADeutsche Wetterdienst, Hohenpeißenberg, GermanyJet Propulsion Laboratory, California Institute of Technology, Wrightwood, CA, USANational Institute of Water and Atmospheric Research (NIWA), Lauder, New ZealandAristotle University of Thessaloniki, Thessaloniki, GreeceNASA Langley Research Center, Hampton, VA, USAFederal Office of Meteorology and Climatology, MeteoSwiss, Payerne, SwitzerlandFederal Office of Meteorology and Climatology, MeteoSwiss, Payerne, SwitzerlandRoyal Belgian Institute for Space Aeronomy (BIRA-IASB), Uccle, BelgiumInstitute of Environmental Physics, Bremen University, Bremen, GermanyRemote Sensing Division, Naval Research Laboratory, Washington, DC, USABryan Scientific Consulting, Charlottesville, VA, USARoyal Meteorological Institute, Uccle, BelgiumInstitute of Astrophysics and Geophysics, University of Liège, Liège, BelgiumNational Institute of Water and Atmospheric Research (NIWA), Lauder, New ZealandKarlsruhe Institute of Technology (KIT), IMK-IFU, Garmisch-Partenkirchen, Germany<p>This study presents an updated evaluation of stratospheric ozone profile trends in the 60<span class="inline-formula"><sup>∘</sup></span> S–60<span class="inline-formula"><sup>∘</sup></span> N latitude range over the 2000–2020 period using an updated version of the Long-term Ozone Trends and Uncertainties in the Stratosphere (LOTUS) regression model that was used to evaluate such trends up to 2016 for the last WMO Ozone Assessment (2018). In addition to the derivation of detailed trends as a function of latitude and vertical coordinates, the regressions are performed with the datasets averaged over broad latitude bands, i.e. 60–35<span class="inline-formula"><sup>∘</sup></span> S, 20<span class="inline-formula"><sup>∘</sup></span> S–20<span class="inline-formula"><sup>∘</sup></span> N and 35–60<span class="inline-formula"><sup>∘</sup></span> N. The same methodology as in the last assessment is applied to combine trends in these broad latitude bands in order to compare the results with the previous studies. Longitudinally resolved merged satellite records are also considered in order to provide a better comparison with trends retrieved from ground-based records, e.g. lidar, ozonesondes, Umkehr, microwave and Fourier transform infrared (FTIR) spectrometers at selected stations where long-term time series are available. The study includes a comparison with trends derived from the REF-C2 simulations of the Chemistry Climate Model Initiative (CCMI-1). This work confirms past results showing an ozone increase in the upper stratosphere, which is now significant in the three broad latitude bands. The increase is largest in the Northern and Southern Hemisphere midlatitudes, with <span class="inline-formula">∼2.2</span> <span class="inline-formula">±</span> 0.7 % per decade at <span class="inline-formula">∼2.1</span> hPa and <span class="inline-formula">∼2.1</span> <span class="inline-formula">±</span> 0.6 % per decade at <span class="inline-formula">∼3.2</span> hPa respectively compared to <span class="inline-formula">∼1.6</span> <span class="inline-formula">±</span> 0.6 % per decade at <span class="inline-formula">∼2.6</span> hPa in the tropics. New trend signals have emerged from the records, such as a significant decrease in ozone in the tropics around 35 hPa and a non-significant increase in ozone in the southern midlatitudes at about 20 hPa. Non-significant negative ozone trends are derived in the lowermost stratosphere, with the most pronounced trends in the tropics. While a very good agreement is obtained between trends from merged satellite records and the CCMI-1 REF-C2 simulation in the upper stratosphere, observed negative trends in the lower stratosphere are not reproduced by models at southern and, in particular, at northern midlatitudes, where models report an ozone increase. However, the lower-stratospheric trend uncertainties are quite large, for both measured and modelled trends. Finally, 2000–2020 stratospheric ozone trends derived from the ground-based and longitudinally resolved satellite records are in reasonable agreement over the European Alpine and tropical regions, while at the Lauder station in the Southern Hemisphere midlatitudes they show some differences.</p>https://acp.copernicus.org/articles/22/11657/2022/acp-22-11657-2022.pdf
spellingShingle S. Godin-Beekmann
N. Azouz
V. F. Sofieva
D. Hubert
I. Petropavlovskikh
P. Effertz
G. Ancellet
D. A. Degenstein
D. Zawada
L. Froidevaux
S. Frith
J. Wild
S. Davis
W. Steinbrecht
T. Leblanc
R. Querel
K. Tourpali
R. Damadeo
E. Maillard Barras
R. Stübi
C. Vigouroux
C. Arosio
G. Nedoluha
I. Boyd
R. Van Malderen
E. Mahieu
D. Smale
R. Sussmann
Updated trends of the stratospheric ozone vertical distribution in the 60°&thinsp;S–60°&thinsp;N latitude range based on the LOTUS regression model
Atmospheric Chemistry and Physics
title Updated trends of the stratospheric ozone vertical distribution in the 60°&thinsp;S–60°&thinsp;N latitude range based on the LOTUS regression model
title_full Updated trends of the stratospheric ozone vertical distribution in the 60°&thinsp;S–60°&thinsp;N latitude range based on the LOTUS regression model
title_fullStr Updated trends of the stratospheric ozone vertical distribution in the 60°&thinsp;S–60°&thinsp;N latitude range based on the LOTUS regression model
title_full_unstemmed Updated trends of the stratospheric ozone vertical distribution in the 60°&thinsp;S–60°&thinsp;N latitude range based on the LOTUS regression model
title_short Updated trends of the stratospheric ozone vertical distribution in the 60°&thinsp;S–60°&thinsp;N latitude range based on the LOTUS regression model
title_sort updated trends of the stratospheric ozone vertical distribution in the 60° thinsp s 60° thinsp n latitude range based on the lotus regression model
url https://acp.copernicus.org/articles/22/11657/2022/acp-22-11657-2022.pdf
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