Sorption-Assisted Ultrafiltration Hybrid Method for Treatment of the Radioactive Aqueous Solutions
The paper presents results of studies on the possibility of using the ultrafiltration method supported by sorption on low-cost, easily accessible aluminosilicates to purify water contaminated with radionuclides. An aqueous solution contaminated with radionuclides in the form of cations at different...
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MDPI AG
2022-09-01
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author | Leon Fuks Agnieszka Miśkiewicz Grażyna Zakrzewska-Kołtuniewicz |
author_facet | Leon Fuks Agnieszka Miśkiewicz Grażyna Zakrzewska-Kołtuniewicz |
author_sort | Leon Fuks |
collection | DOAJ |
description | The paper presents results of studies on the possibility of using the ultrafiltration method supported by sorption on low-cost, easily accessible aluminosilicates to purify water contaminated with radionuclides. An aqueous solution contaminated with radionuclides in the form of cations at different oxidation states—Cs(I)-137, Co(II)-60 and Am(III)-241—as well as pertechnetate anions—TcO<sub>4</sub><sup>−</sup>-99m—was treated by the proposed hybrid method. In the presented work, the influence of the important process parameters (i.e., pH, sorbent dosage, temperature and feed flow rate) on the removal efficiency of radionuclides was studied. The obtained results showed that hazardous impurities, both in the form of cations and anions, may be effectively removed from water by the application of sorption-assisted UF (SAUF) using the clay-salt slimes as a sorbent. As a final stage of the work, we treated the simulated liquid radioactive waste using the SAUF method, also showing satisfactory results in its purification efficiency. |
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language | English |
last_indexed | 2024-03-10T00:25:03Z |
publishDate | 2022-09-01 |
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spelling | doaj.art-beab95fc5d3c43fc97f49ce9d71260912023-11-23T15:35:32ZengMDPI AGChemistry2624-85492022-09-01431076109110.3390/chemistry4030073Sorption-Assisted Ultrafiltration Hybrid Method for Treatment of the Radioactive Aqueous SolutionsLeon Fuks0Agnieszka Miśkiewicz1Grażyna Zakrzewska-Kołtuniewicz2Centre for Radiochemistry and Nuclear Chemistry, Institute of Nuclear Chemistry and Technology, Dorodna 16, 03-195 Warszawa, PolandCentre for Radiochemistry and Nuclear Chemistry, Institute of Nuclear Chemistry and Technology, Dorodna 16, 03-195 Warszawa, PolandCentre for Radiochemistry and Nuclear Chemistry, Institute of Nuclear Chemistry and Technology, Dorodna 16, 03-195 Warszawa, PolandThe paper presents results of studies on the possibility of using the ultrafiltration method supported by sorption on low-cost, easily accessible aluminosilicates to purify water contaminated with radionuclides. An aqueous solution contaminated with radionuclides in the form of cations at different oxidation states—Cs(I)-137, Co(II)-60 and Am(III)-241—as well as pertechnetate anions—TcO<sub>4</sub><sup>−</sup>-99m—was treated by the proposed hybrid method. In the presented work, the influence of the important process parameters (i.e., pH, sorbent dosage, temperature and feed flow rate) on the removal efficiency of radionuclides was studied. The obtained results showed that hazardous impurities, both in the form of cations and anions, may be effectively removed from water by the application of sorption-assisted UF (SAUF) using the clay-salt slimes as a sorbent. As a final stage of the work, we treated the simulated liquid radioactive waste using the SAUF method, also showing satisfactory results in its purification efficiency.https://www.mdpi.com/2624-8549/4/3/73water contaminationradioactive wastedecontaminationsorption-assisted ultrafiltrationSAUFlow-cost adsorbent |
spellingShingle | Leon Fuks Agnieszka Miśkiewicz Grażyna Zakrzewska-Kołtuniewicz Sorption-Assisted Ultrafiltration Hybrid Method for Treatment of the Radioactive Aqueous Solutions Chemistry water contamination radioactive waste decontamination sorption-assisted ultrafiltration SAUF low-cost adsorbent |
title | Sorption-Assisted Ultrafiltration Hybrid Method for Treatment of the Radioactive Aqueous Solutions |
title_full | Sorption-Assisted Ultrafiltration Hybrid Method for Treatment of the Radioactive Aqueous Solutions |
title_fullStr | Sorption-Assisted Ultrafiltration Hybrid Method for Treatment of the Radioactive Aqueous Solutions |
title_full_unstemmed | Sorption-Assisted Ultrafiltration Hybrid Method for Treatment of the Radioactive Aqueous Solutions |
title_short | Sorption-Assisted Ultrafiltration Hybrid Method for Treatment of the Radioactive Aqueous Solutions |
title_sort | sorption assisted ultrafiltration hybrid method for treatment of the radioactive aqueous solutions |
topic | water contamination radioactive waste decontamination sorption-assisted ultrafiltration SAUF low-cost adsorbent |
url | https://www.mdpi.com/2624-8549/4/3/73 |
work_keys_str_mv | AT leonfuks sorptionassistedultrafiltrationhybridmethodfortreatmentoftheradioactiveaqueoussolutions AT agnieszkamiskiewicz sorptionassistedultrafiltrationhybridmethodfortreatmentoftheradioactiveaqueoussolutions AT grazynazakrzewskakołtuniewicz sorptionassistedultrafiltrationhybridmethodfortreatmentoftheradioactiveaqueoussolutions |