Ti3C2Tx MXene‐Based Superhydrophobic Broadband Terahertz Absorber with Large Pore‐Size Foam Architecture

Abstract Porous polymer‐based Terahertz (THz) absorbers possess strong absorption with broadband, lightweight, and flexible features. Thus these are widely desired in THz electromagnetic shielding, radar‐cross‐section reduction, radiometer calibration, etc. However, the harsh environment of humidity...

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Main Authors: Min Luo, Junchang Guo, Wenchao Shui, Yao Tan, Haoming Huang, Qinghui Yang, Huaiwu Zhang, Xu Deng, Qi‐Ye Wen
Format: Article
Language:English
Published: Wiley-VCH 2023-01-01
Series:Advanced Materials Interfaces
Subjects:
Online Access:https://doi.org/10.1002/admi.202201767
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author Min Luo
Junchang Guo
Wenchao Shui
Yao Tan
Haoming Huang
Qinghui Yang
Huaiwu Zhang
Xu Deng
Qi‐Ye Wen
author_facet Min Luo
Junchang Guo
Wenchao Shui
Yao Tan
Haoming Huang
Qinghui Yang
Huaiwu Zhang
Xu Deng
Qi‐Ye Wen
author_sort Min Luo
collection DOAJ
description Abstract Porous polymer‐based Terahertz (THz) absorbers possess strong absorption with broadband, lightweight, and flexible features. Thus these are widely desired in THz electromagnetic shielding, radar‐cross‐section reduction, radiometer calibration, etc. However, the harsh environment of humidity, corrosiveness, and dustiness undermines the performance and service lifetime of the porous absorbers. Here, based on Ti3C2Tx MXene sponge composite foam (MSF), a superhydrophobic broadband THz absorber on a large pore‐size porous architecture by a joint hydrophobic strategy is realized. Results show that the apparent contact angles and roll‐off angles of the modified MSF reached 159.0° and 7.6°, while maintaining an ultra‐high absorption rate of 99.6% in the frequency range of 0.3–1.2 THz. Furthermore, the special Micro‐Nano hierarchical structures render the absorber a strong bounce‐off ability to the droplets of an aqueous solution. These water‐repellent properties endow the absorber the versatility of self‐cleaning and anti‐corrosion, thus can be widely applied in many scenarios including THz remote sensing, communication, and security screening as well.
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spelling doaj.art-c0053fe8e3db46a192c10bc28f5d7ff22023-08-31T09:03:07ZengWiley-VCHAdvanced Materials Interfaces2196-73502023-01-01102n/an/a10.1002/admi.202201767Ti3C2Tx MXene‐Based Superhydrophobic Broadband Terahertz Absorber with Large Pore‐Size Foam ArchitectureMin Luo0Junchang Guo1Wenchao Shui2Yao Tan3Haoming Huang4Qinghui Yang5Huaiwu Zhang6Xu Deng7Qi‐Ye Wen8State Key Laboratory of Electronic Thin Film and Integrated Devices Department of Electronic Science and Engineering University of Electronic Science and Technology of China Chengdu Sichuan 611731 ChinaInstitute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China Chengdu Sichuan 611731 ChinaState Key Laboratory of Electronic Thin Film and Integrated Devices Department of Electronic Science and Engineering University of Electronic Science and Technology of China Chengdu Sichuan 611731 ChinaInstitute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China Chengdu Sichuan 611731 ChinaState Key Laboratory of Electronic Thin Film and Integrated Devices Department of Electronic Science and Engineering University of Electronic Science and Technology of China Chengdu Sichuan 611731 ChinaState Key Laboratory of Electronic Thin Film and Integrated Devices Department of Electronic Science and Engineering University of Electronic Science and Technology of China Chengdu Sichuan 611731 ChinaState Key Laboratory of Electronic Thin Film and Integrated Devices Department of Electronic Science and Engineering University of Electronic Science and Technology of China Chengdu Sichuan 611731 ChinaInstitute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China Chengdu Sichuan 611731 ChinaState Key Laboratory of Electronic Thin Film and Integrated Devices Department of Electronic Science and Engineering University of Electronic Science and Technology of China Chengdu Sichuan 611731 ChinaAbstract Porous polymer‐based Terahertz (THz) absorbers possess strong absorption with broadband, lightweight, and flexible features. Thus these are widely desired in THz electromagnetic shielding, radar‐cross‐section reduction, radiometer calibration, etc. However, the harsh environment of humidity, corrosiveness, and dustiness undermines the performance and service lifetime of the porous absorbers. Here, based on Ti3C2Tx MXene sponge composite foam (MSF), a superhydrophobic broadband THz absorber on a large pore‐size porous architecture by a joint hydrophobic strategy is realized. Results show that the apparent contact angles and roll‐off angles of the modified MSF reached 159.0° and 7.6°, while maintaining an ultra‐high absorption rate of 99.6% in the frequency range of 0.3–1.2 THz. Furthermore, the special Micro‐Nano hierarchical structures render the absorber a strong bounce‐off ability to the droplets of an aqueous solution. These water‐repellent properties endow the absorber the versatility of self‐cleaning and anti‐corrosion, thus can be widely applied in many scenarios including THz remote sensing, communication, and security screening as well.https://doi.org/10.1002/admi.202201767broadbandMXeneporous architecturesuperhydrophobicityterahertz absorber
spellingShingle Min Luo
Junchang Guo
Wenchao Shui
Yao Tan
Haoming Huang
Qinghui Yang
Huaiwu Zhang
Xu Deng
Qi‐Ye Wen
Ti3C2Tx MXene‐Based Superhydrophobic Broadband Terahertz Absorber with Large Pore‐Size Foam Architecture
Advanced Materials Interfaces
broadband
MXene
porous architecture
superhydrophobicity
terahertz absorber
title Ti3C2Tx MXene‐Based Superhydrophobic Broadband Terahertz Absorber with Large Pore‐Size Foam Architecture
title_full Ti3C2Tx MXene‐Based Superhydrophobic Broadband Terahertz Absorber with Large Pore‐Size Foam Architecture
title_fullStr Ti3C2Tx MXene‐Based Superhydrophobic Broadband Terahertz Absorber with Large Pore‐Size Foam Architecture
title_full_unstemmed Ti3C2Tx MXene‐Based Superhydrophobic Broadband Terahertz Absorber with Large Pore‐Size Foam Architecture
title_short Ti3C2Tx MXene‐Based Superhydrophobic Broadband Terahertz Absorber with Large Pore‐Size Foam Architecture
title_sort ti3c2tx mxene based superhydrophobic broadband terahertz absorber with large pore size foam architecture
topic broadband
MXene
porous architecture
superhydrophobicity
terahertz absorber
url https://doi.org/10.1002/admi.202201767
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