Modeling the Effect of Material Viscoelasticity on the Dielectric Permittivity of Deformed Elastomers

Elastomers, as a typical category of soft dielectrics, have shown great potential for developing stretchable electronics and soft transducers. However, the performance of dielectric elastomers (DEs) is susceptible to the dielectric permittivity of the material, whether as insulators or actuators. On...

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Main Authors: Xianghe Zheng, Jianyou Zhou
Format: Article
Language:English
Published: MDPI AG 2023-12-01
Series:Polymers
Subjects:
Online Access:https://www.mdpi.com/2073-4360/16/1/113
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author Xianghe Zheng
Jianyou Zhou
author_facet Xianghe Zheng
Jianyou Zhou
author_sort Xianghe Zheng
collection DOAJ
description Elastomers, as a typical category of soft dielectrics, have shown great potential for developing stretchable electronics and soft transducers. However, the performance of dielectric elastomers (DEs) is susceptible to the dielectric permittivity of the material, whether as insulators or actuators. On the other hand, experiments suggest that the material viscoelasticity significantly influences the dielectric permittivity of DEs. Based on the theory of finite-deformation viscoelasticity, this work adopts the Brillouin function to develop a modeling framework to examine the effect of material viscoelasticity on the dielectric permittivity for the first time. A comparison of the data fitting results between the models with and without consideration of the material viscoelasticity is presented. Simulation results also reveal that the viscous network of the elastomer exerts a mitigation effect on the decrease in the dielectric permittivity when the material is deformed. Furthermore, it is found that the loading rate is a key parameter that strongly affects the dielectric permittivity, mainly through the inelastic deformation.
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spelling doaj.art-c0088780d46247998f9c56efb7ea38372024-01-10T15:06:53ZengMDPI AGPolymers2073-43602023-12-0116111310.3390/polym16010113Modeling the Effect of Material Viscoelasticity on the Dielectric Permittivity of Deformed ElastomersXianghe Zheng0Jianyou Zhou1School of Science, Harbin Institute of Technology, Shenzhen 518055, ChinaSchool of Science, Harbin Institute of Technology, Shenzhen 518055, ChinaElastomers, as a typical category of soft dielectrics, have shown great potential for developing stretchable electronics and soft transducers. However, the performance of dielectric elastomers (DEs) is susceptible to the dielectric permittivity of the material, whether as insulators or actuators. On the other hand, experiments suggest that the material viscoelasticity significantly influences the dielectric permittivity of DEs. Based on the theory of finite-deformation viscoelasticity, this work adopts the Brillouin function to develop a modeling framework to examine the effect of material viscoelasticity on the dielectric permittivity for the first time. A comparison of the data fitting results between the models with and without consideration of the material viscoelasticity is presented. Simulation results also reveal that the viscous network of the elastomer exerts a mitigation effect on the decrease in the dielectric permittivity when the material is deformed. Furthermore, it is found that the loading rate is a key parameter that strongly affects the dielectric permittivity, mainly through the inelastic deformation.https://www.mdpi.com/2073-4360/16/1/113dielectric elastomersdielectric permittivitymaterial viscoelasticitypolarizationrate-dependency
spellingShingle Xianghe Zheng
Jianyou Zhou
Modeling the Effect of Material Viscoelasticity on the Dielectric Permittivity of Deformed Elastomers
Polymers
dielectric elastomers
dielectric permittivity
material viscoelasticity
polarization
rate-dependency
title Modeling the Effect of Material Viscoelasticity on the Dielectric Permittivity of Deformed Elastomers
title_full Modeling the Effect of Material Viscoelasticity on the Dielectric Permittivity of Deformed Elastomers
title_fullStr Modeling the Effect of Material Viscoelasticity on the Dielectric Permittivity of Deformed Elastomers
title_full_unstemmed Modeling the Effect of Material Viscoelasticity on the Dielectric Permittivity of Deformed Elastomers
title_short Modeling the Effect of Material Viscoelasticity on the Dielectric Permittivity of Deformed Elastomers
title_sort modeling the effect of material viscoelasticity on the dielectric permittivity of deformed elastomers
topic dielectric elastomers
dielectric permittivity
material viscoelasticity
polarization
rate-dependency
url https://www.mdpi.com/2073-4360/16/1/113
work_keys_str_mv AT xianghezheng modelingtheeffectofmaterialviscoelasticityonthedielectricpermittivityofdeformedelastomers
AT jianyouzhou modelingtheeffectofmaterialviscoelasticityonthedielectricpermittivityofdeformedelastomers