Evaluation of the Radiation-Protective Properties of Bi (Pb)–Sr–Ca–Cu–O Ceramic Prepared at Different Temperatures with Silver Inclusion

The influences of the sintering process and AgNO<sub>3</sub> addition on the phase formation and radiation shielding characteristics of Bi<sub>1.6</sub>Pb<sub>0.4</sub>Sr<sub>2</sub>Ca<sub>2</sub>Cu<sub>3</sub>O<sub>10<...

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Main Authors: Essia Hannachi, K. A. Mahmoud, Aljawhara H. Almuqrin, M. I. Sayyed, Yassine Slimani
Format: Article
Language:English
Published: MDPI AG 2022-01-01
Series:Materials
Subjects:
Online Access:https://www.mdpi.com/1996-1944/15/3/1034
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author Essia Hannachi
K. A. Mahmoud
Aljawhara H. Almuqrin
M. I. Sayyed
Yassine Slimani
author_facet Essia Hannachi
K. A. Mahmoud
Aljawhara H. Almuqrin
M. I. Sayyed
Yassine Slimani
author_sort Essia Hannachi
collection DOAJ
description The influences of the sintering process and AgNO<sub>3</sub> addition on the phase formation and radiation shielding characteristics of Bi<sub>1.6</sub>Pb<sub>0.4</sub>Sr<sub>2</sub>Ca<sub>2</sub>Cu<sub>3</sub>O<sub>10</sub> were studied. Three ceramics (code: C0, C1, and C2) were prepared as follows: C0 was obtained after calcination and only one sintering step, C1 was obtained after calcination and two sintering cycles, and C2 was prepared after the addition of AgNO<sub>3</sub> at the beginning of the final sintering stage. C2 displayed the maximum volume fraction of the Bi-2223 phase (76.4 vol%), the greatest crystallite size, and high density. The linear mass attenuation coefficient (µ) has been simulated using the Monte Carlo simulation. The µ values are high at 15 keV (257.2 cm<sup>−1</sup> for C0, 417.57 cm<sup>−1</sup> for C1, and 421.16 cm<sup>−1</sup> for C2), and these values dropped and became 72.58, 117.83 and 133.19 cm<sup>−1</sup> at 30 keV. The µ value for the ceramics after sintering is much higher than the ceramic before sintering. In addition, the µ value for C2 is higher than that of C1, suggesting that the AgNO<sub>3</sub> improves the radiation attenuation performance for the fabricated ceramics. It was demonstrated that the sintering and AgNO<sub>3</sub> addition have a considerable influence on the ceramic thickness required to attenuate the radiation.
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spelling doaj.art-c0803799eefe4cfe97b164699e42363c2023-11-23T17:01:11ZengMDPI AGMaterials1996-19442022-01-01153103410.3390/ma15031034Evaluation of the Radiation-Protective Properties of Bi (Pb)–Sr–Ca–Cu–O Ceramic Prepared at Different Temperatures with Silver InclusionEssia Hannachi0K. A. Mahmoud1Aljawhara H. Almuqrin2M. I. Sayyed3Yassine Slimani4Department of Nuclear Medicine Research, Institute for Research and Medical Consultations (IRMC), Imam Abdulrahman Bin Faisal University, Dammam 31441, Saudi ArabiaDepartment of Nuclear Power Plants and Renewable Energy, Ural Federal University, St. Mira 19, 620002 Yekaterinburg, RussiaDepartment of Physics, College of Science, Princess Nourah Bint Abdulrahman University, Riyadh 11671, Saudi ArabiaDepartment of Nuclear Medicine Research, Institute for Research and Medical Consultations (IRMC), Imam Abdulrahman Bin Faisal University, Dammam 31441, Saudi ArabiaDepartment of Biophysics, Institute for Research and Medical Consultations (IRMC), Imam Abdulrahman Bin Faisal University, Dammam 31441, Saudi ArabiaThe influences of the sintering process and AgNO<sub>3</sub> addition on the phase formation and radiation shielding characteristics of Bi<sub>1.6</sub>Pb<sub>0.4</sub>Sr<sub>2</sub>Ca<sub>2</sub>Cu<sub>3</sub>O<sub>10</sub> were studied. Three ceramics (code: C0, C1, and C2) were prepared as follows: C0 was obtained after calcination and only one sintering step, C1 was obtained after calcination and two sintering cycles, and C2 was prepared after the addition of AgNO<sub>3</sub> at the beginning of the final sintering stage. C2 displayed the maximum volume fraction of the Bi-2223 phase (76.4 vol%), the greatest crystallite size, and high density. The linear mass attenuation coefficient (µ) has been simulated using the Monte Carlo simulation. The µ values are high at 15 keV (257.2 cm<sup>−1</sup> for C0, 417.57 cm<sup>−1</sup> for C1, and 421.16 cm<sup>−1</sup> for C2), and these values dropped and became 72.58, 117.83 and 133.19 cm<sup>−1</sup> at 30 keV. The µ value for the ceramics after sintering is much higher than the ceramic before sintering. In addition, the µ value for C2 is higher than that of C1, suggesting that the AgNO<sub>3</sub> improves the radiation attenuation performance for the fabricated ceramics. It was demonstrated that the sintering and AgNO<sub>3</sub> addition have a considerable influence on the ceramic thickness required to attenuate the radiation.https://www.mdpi.com/1996-1944/15/3/1034ceramicphase formationsilverMonte Carlolinear attenuation coefficientradiation shielding efficiency factor
spellingShingle Essia Hannachi
K. A. Mahmoud
Aljawhara H. Almuqrin
M. I. Sayyed
Yassine Slimani
Evaluation of the Radiation-Protective Properties of Bi (Pb)–Sr–Ca–Cu–O Ceramic Prepared at Different Temperatures with Silver Inclusion
Materials
ceramic
phase formation
silver
Monte Carlo
linear attenuation coefficient
radiation shielding efficiency factor
title Evaluation of the Radiation-Protective Properties of Bi (Pb)–Sr–Ca–Cu–O Ceramic Prepared at Different Temperatures with Silver Inclusion
title_full Evaluation of the Radiation-Protective Properties of Bi (Pb)–Sr–Ca–Cu–O Ceramic Prepared at Different Temperatures with Silver Inclusion
title_fullStr Evaluation of the Radiation-Protective Properties of Bi (Pb)–Sr–Ca–Cu–O Ceramic Prepared at Different Temperatures with Silver Inclusion
title_full_unstemmed Evaluation of the Radiation-Protective Properties of Bi (Pb)–Sr–Ca–Cu–O Ceramic Prepared at Different Temperatures with Silver Inclusion
title_short Evaluation of the Radiation-Protective Properties of Bi (Pb)–Sr–Ca–Cu–O Ceramic Prepared at Different Temperatures with Silver Inclusion
title_sort evaluation of the radiation protective properties of bi pb sr ca cu o ceramic prepared at different temperatures with silver inclusion
topic ceramic
phase formation
silver
Monte Carlo
linear attenuation coefficient
radiation shielding efficiency factor
url https://www.mdpi.com/1996-1944/15/3/1034
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