Nonlinear Magneto-Electro-Mechanical Response of Physical Cross-Linked Magneto-Electric Polymer Gel

This work reports on a novel magnetorheological polymer gel with carbon nanotubes and carbonyl iron particles mixed into the physical cross-linked polymer gel matrix. The resulting composites show unusual nonlinear magneto-electro-mechanical responses. Because of the low matrix viscosity, effective...

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Main Authors: Xiwen Fan, Yu Wang, Bochao Wang, Longjiang Shen, Jun Li, Zhenbang Xu, Sheng Wang, Xinglong Gong
Format: Article
Language:English
Published: Frontiers Media S.A. 2021-06-01
Series:Frontiers in Materials
Subjects:
Online Access:https://www.frontiersin.org/articles/10.3389/fmats.2021.665814/full
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author Xiwen Fan
Yu Wang
Bochao Wang
Longjiang Shen
Jun Li
Zhenbang Xu
Sheng Wang
Xinglong Gong
author_facet Xiwen Fan
Yu Wang
Bochao Wang
Longjiang Shen
Jun Li
Zhenbang Xu
Sheng Wang
Xinglong Gong
author_sort Xiwen Fan
collection DOAJ
description This work reports on a novel magnetorheological polymer gel with carbon nanotubes and carbonyl iron particles mixed into the physical cross-linked polymer gel matrix. The resulting composites show unusual nonlinear magneto-electro-mechanical responses. Because of the low matrix viscosity, effective conductive paths formed by the CNTs were mobile and high-performance sensing characteristics were observed. In particular, due to the transient and mutable physical cross-linked bonds in the polymer gel, the electromechanical behavior acted in a rate-dependent manner. External stimulus at a high rate significantly enhanced the electrical resistance response during mechanical deformation. Meanwhile, the rheological properties were regulated by the external magnetic field when magnetic particles were added. This dual enhancement mechanism further contributes to the active control of electromechanical performance. These polymer composites could be adopted as electromechanical sensitive sensors to measure impact and vibration under different frequencies. There is great potential for this magnetorheological polymer gel in the application of intelligent vibration controls.
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spelling doaj.art-c095288756434fceac8a68415fbde38c2022-12-21T22:08:29ZengFrontiers Media S.A.Frontiers in Materials2296-80162021-06-01810.3389/fmats.2021.665814665814Nonlinear Magneto-Electro-Mechanical Response of Physical Cross-Linked Magneto-Electric Polymer GelXiwen Fan0Yu Wang1Bochao Wang2Longjiang Shen3Jun Li4Zhenbang Xu5Sheng Wang6Xinglong Gong7CAS Key Laboratory of Mechanical Behavior and Design of Materials, CAS Center for Excellence in Complex System Mechanics, Department of Modern Mechanics, University of Science and Technology of China, Hefei, ChinaCAS Key Laboratory of Mechanical Behavior and Design of Materials, CAS Center for Excellence in Complex System Mechanics, Department of Modern Mechanics, University of Science and Technology of China, Hefei, ChinaCAS Key Laboratory of Mechanical Behavior and Design of Materials, CAS Center for Excellence in Complex System Mechanics, Department of Modern Mechanics, University of Science and Technology of China, Hefei, ChinaHunan Bogie Engineering Research Center, Zhuzhou, ChinaAnhui Weiwei Rubber Parts Group Co. Ltd., Tongcheng, ChinaCAS Key Laboratory of On-orbit Manufacturing and Integration for Space Optics System, Fine Mechanics and Physics, Changchun Institute of Optics, Chinese Academy of Sciences, Changchun, ChinaCAS Key Laboratory of Mechanical Behavior and Design of Materials, CAS Center for Excellence in Complex System Mechanics, Department of Modern Mechanics, University of Science and Technology of China, Hefei, ChinaCAS Key Laboratory of Mechanical Behavior and Design of Materials, CAS Center for Excellence in Complex System Mechanics, Department of Modern Mechanics, University of Science and Technology of China, Hefei, ChinaThis work reports on a novel magnetorheological polymer gel with carbon nanotubes and carbonyl iron particles mixed into the physical cross-linked polymer gel matrix. The resulting composites show unusual nonlinear magneto-electro-mechanical responses. Because of the low matrix viscosity, effective conductive paths formed by the CNTs were mobile and high-performance sensing characteristics were observed. In particular, due to the transient and mutable physical cross-linked bonds in the polymer gel, the electromechanical behavior acted in a rate-dependent manner. External stimulus at a high rate significantly enhanced the electrical resistance response during mechanical deformation. Meanwhile, the rheological properties were regulated by the external magnetic field when magnetic particles were added. This dual enhancement mechanism further contributes to the active control of electromechanical performance. These polymer composites could be adopted as electromechanical sensitive sensors to measure impact and vibration under different frequencies. There is great potential for this magnetorheological polymer gel in the application of intelligent vibration controls.https://www.frontiersin.org/articles/10.3389/fmats.2021.665814/fullpiezo-resistivitycarbon nanotubessoft sensorshear stiffeningmagnetorheological gel
spellingShingle Xiwen Fan
Yu Wang
Bochao Wang
Longjiang Shen
Jun Li
Zhenbang Xu
Sheng Wang
Xinglong Gong
Nonlinear Magneto-Electro-Mechanical Response of Physical Cross-Linked Magneto-Electric Polymer Gel
Frontiers in Materials
piezo-resistivity
carbon nanotubes
soft sensor
shear stiffening
magnetorheological gel
title Nonlinear Magneto-Electro-Mechanical Response of Physical Cross-Linked Magneto-Electric Polymer Gel
title_full Nonlinear Magneto-Electro-Mechanical Response of Physical Cross-Linked Magneto-Electric Polymer Gel
title_fullStr Nonlinear Magneto-Electro-Mechanical Response of Physical Cross-Linked Magneto-Electric Polymer Gel
title_full_unstemmed Nonlinear Magneto-Electro-Mechanical Response of Physical Cross-Linked Magneto-Electric Polymer Gel
title_short Nonlinear Magneto-Electro-Mechanical Response of Physical Cross-Linked Magneto-Electric Polymer Gel
title_sort nonlinear magneto electro mechanical response of physical cross linked magneto electric polymer gel
topic piezo-resistivity
carbon nanotubes
soft sensor
shear stiffening
magnetorheological gel
url https://www.frontiersin.org/articles/10.3389/fmats.2021.665814/full
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AT longjiangshen nonlinearmagnetoelectromechanicalresponseofphysicalcrosslinkedmagnetoelectricpolymergel
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AT zhenbangxu nonlinearmagnetoelectromechanicalresponseofphysicalcrosslinkedmagnetoelectricpolymergel
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