Phase diagrams guide synthesis of highly ordered intermetallic electrocatalysts: separating alloying and ordering stages

The synthesis of highly ordered intermetallic compound catalysts remains a challenge owing to the limited understanding of their formation mechanism under high-temperature conditions. Here the authors identify phase-transition-temperature-dependent evolution process in the synthesis of intermetallic...

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Main Authors: Wei-Jie Zeng, Chang Wang, Qiang-Qiang Yan, Peng Yin, Lei Tong, Hai-Wei Liang
Format: Article
Language:English
Published: Nature Portfolio 2022-12-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-022-35457-1
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author Wei-Jie Zeng
Chang Wang
Qiang-Qiang Yan
Peng Yin
Lei Tong
Hai-Wei Liang
author_facet Wei-Jie Zeng
Chang Wang
Qiang-Qiang Yan
Peng Yin
Lei Tong
Hai-Wei Liang
author_sort Wei-Jie Zeng
collection DOAJ
description The synthesis of highly ordered intermetallic compound catalysts remains a challenge owing to the limited understanding of their formation mechanism under high-temperature conditions. Here the authors identify phase-transition-temperature-dependent evolution process in the synthesis of intermetallic Pt catalysts and propose a separate alloying/ordering annealing synthetic protocol.
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spelling doaj.art-c10409b35bda4b69bff54bfcc423cfc72022-12-22T03:50:42ZengNature PortfolioNature Communications2041-17232022-12-011311810.1038/s41467-022-35457-1Phase diagrams guide synthesis of highly ordered intermetallic electrocatalysts: separating alloying and ordering stagesWei-Jie Zeng0Chang Wang1Qiang-Qiang Yan2Peng Yin3Lei Tong4Hai-Wei Liang5Hefei National Research Center for Physical Sciences at the Microscale, Department of Chemistry, University of Science and Technology of ChinaDalian Institute of Chemical Physics, Chinese Academy of SciencesHefei National Research Center for Physical Sciences at the Microscale, Department of Chemistry, University of Science and Technology of ChinaHefei National Research Center for Physical Sciences at the Microscale, Department of Chemistry, University of Science and Technology of ChinaHefei National Research Center for Physical Sciences at the Microscale, Department of Chemistry, University of Science and Technology of ChinaHefei National Research Center for Physical Sciences at the Microscale, Department of Chemistry, University of Science and Technology of ChinaThe synthesis of highly ordered intermetallic compound catalysts remains a challenge owing to the limited understanding of their formation mechanism under high-temperature conditions. Here the authors identify phase-transition-temperature-dependent evolution process in the synthesis of intermetallic Pt catalysts and propose a separate alloying/ordering annealing synthetic protocol.https://doi.org/10.1038/s41467-022-35457-1
spellingShingle Wei-Jie Zeng
Chang Wang
Qiang-Qiang Yan
Peng Yin
Lei Tong
Hai-Wei Liang
Phase diagrams guide synthesis of highly ordered intermetallic electrocatalysts: separating alloying and ordering stages
Nature Communications
title Phase diagrams guide synthesis of highly ordered intermetallic electrocatalysts: separating alloying and ordering stages
title_full Phase diagrams guide synthesis of highly ordered intermetallic electrocatalysts: separating alloying and ordering stages
title_fullStr Phase diagrams guide synthesis of highly ordered intermetallic electrocatalysts: separating alloying and ordering stages
title_full_unstemmed Phase diagrams guide synthesis of highly ordered intermetallic electrocatalysts: separating alloying and ordering stages
title_short Phase diagrams guide synthesis of highly ordered intermetallic electrocatalysts: separating alloying and ordering stages
title_sort phase diagrams guide synthesis of highly ordered intermetallic electrocatalysts separating alloying and ordering stages
url https://doi.org/10.1038/s41467-022-35457-1
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