All-optical nuclear quantum sensing using nitrogen-vacancy centers in diamond

Abstract Solid state spins have demonstrated significant potential in quantum sensing with applications including fundamental science, medical diagnostics and navigation. The quantum sensing schemes showing best performance under ambient conditions all utilize microwave or radio-frequency driving, w...

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Main Authors: B. Bürgler, T. F. Sjolander, O. Brinza, A. Tallaire, J. Achard, P. Maletinsky
Format: Article
Language:English
Published: Nature Portfolio 2023-06-01
Series:npj Quantum Information
Online Access:https://doi.org/10.1038/s41534-023-00724-6
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author B. Bürgler
T. F. Sjolander
O. Brinza
A. Tallaire
J. Achard
P. Maletinsky
author_facet B. Bürgler
T. F. Sjolander
O. Brinza
A. Tallaire
J. Achard
P. Maletinsky
author_sort B. Bürgler
collection DOAJ
description Abstract Solid state spins have demonstrated significant potential in quantum sensing with applications including fundamental science, medical diagnostics and navigation. The quantum sensing schemes showing best performance under ambient conditions all utilize microwave or radio-frequency driving, which poses a significant limitation for miniaturization, energy efficiency, and non-invasiveness of quantum sensors. We overcome this limitation by demonstrating a purely optical approach to coherent quantum sensing. Our scheme involves the 15N nuclear spin of the Nitrogen-Vacancy (NV) center in diamond as a sensing resource, and exploits NV spin dynamics in oblique magnetic fields near the NV’s excited state level anti-crossing to optically pump the nuclear spin into a quantum superposition state. We demonstrate all-optical free-induction decay measurements—the key protocol for low-frequency quantum sensing—both on single spins and spin ensembles. Our results pave the way for highly compact quantum sensors to be employed for magnetometry or gyroscopy applications in challenging environments.
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spelling doaj.art-c1083986c64f43b8bd6b4bae5634b8382023-06-11T11:21:30ZengNature Portfolionpj Quantum Information2056-63872023-06-01911710.1038/s41534-023-00724-6All-optical nuclear quantum sensing using nitrogen-vacancy centers in diamondB. Bürgler0T. F. Sjolander1O. Brinza2A. Tallaire3J. Achard4P. Maletinsky5Department of Physics, University of BaselDepartment of Physics, University of BaselLaboratoire des Sciences des Procédés et des Matériaux, LSPM, CNRS-UPR 3407, Université Sorbonne Paris NordLaboratoire des Sciences des Procédés et des Matériaux, LSPM, CNRS-UPR 3407, Université Sorbonne Paris NordLaboratoire des Sciences des Procédés et des Matériaux, LSPM, CNRS-UPR 3407, Université Sorbonne Paris NordDepartment of Physics, University of BaselAbstract Solid state spins have demonstrated significant potential in quantum sensing with applications including fundamental science, medical diagnostics and navigation. The quantum sensing schemes showing best performance under ambient conditions all utilize microwave or radio-frequency driving, which poses a significant limitation for miniaturization, energy efficiency, and non-invasiveness of quantum sensors. We overcome this limitation by demonstrating a purely optical approach to coherent quantum sensing. Our scheme involves the 15N nuclear spin of the Nitrogen-Vacancy (NV) center in diamond as a sensing resource, and exploits NV spin dynamics in oblique magnetic fields near the NV’s excited state level anti-crossing to optically pump the nuclear spin into a quantum superposition state. We demonstrate all-optical free-induction decay measurements—the key protocol for low-frequency quantum sensing—both on single spins and spin ensembles. Our results pave the way for highly compact quantum sensors to be employed for magnetometry or gyroscopy applications in challenging environments.https://doi.org/10.1038/s41534-023-00724-6
spellingShingle B. Bürgler
T. F. Sjolander
O. Brinza
A. Tallaire
J. Achard
P. Maletinsky
All-optical nuclear quantum sensing using nitrogen-vacancy centers in diamond
npj Quantum Information
title All-optical nuclear quantum sensing using nitrogen-vacancy centers in diamond
title_full All-optical nuclear quantum sensing using nitrogen-vacancy centers in diamond
title_fullStr All-optical nuclear quantum sensing using nitrogen-vacancy centers in diamond
title_full_unstemmed All-optical nuclear quantum sensing using nitrogen-vacancy centers in diamond
title_short All-optical nuclear quantum sensing using nitrogen-vacancy centers in diamond
title_sort all optical nuclear quantum sensing using nitrogen vacancy centers in diamond
url https://doi.org/10.1038/s41534-023-00724-6
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