CO2‐Induced Spin‐Lattice Coupling for Strong Magnetoelectric Materials
Abstract The preparation of 2D magnetoelectric (ME) nanomaterials with strong ME coupling is crucial for the fast reading and writing processes in the next generation of storage devices. Herein, 2D BaTiO3 (BTO)‐CoFe2O4 (CFO) ME nanocomposites are prepared through a substrate‐free coupling strategy u...
| Main Authors: | , , |
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| Format: | Article |
| Language: | English |
| Published: |
Wiley
2024-02-01
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| Series: | Advanced Science |
| Subjects: | |
| Online Access: | https://doi.org/10.1002/advs.202303692 |
| _version_ | 1797329392665362432 |
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| author | Bo Gao Song Xu Qun Xu |
| author_facet | Bo Gao Song Xu Qun Xu |
| author_sort | Bo Gao |
| collection | DOAJ |
| description | Abstract The preparation of 2D magnetoelectric (ME) nanomaterials with strong ME coupling is crucial for the fast reading and writing processes in the next generation of storage devices. Herein, 2D BaTiO3 (BTO)‐CoFe2O4 (CFO) ME nanocomposites are prepared through a substrate‐free coupling strategy using supercritical CO2. Such 2D BTO‐CFO with strong coupling is built through alternating in‐plane and out‐of‐plane epitaxy stacking, leading to remarkable mutual biaxial strain effects for spin‐lattice coupling. As a results, such strain effect significantly enhances the ferroelectricity of BTO and the ferrimagnetism of CFO, where an unexceptionally high ME coupling coefficient of (325.8 mV cm−1 Oe−1) is obtained for the BTO‐CFO nanocomposites. |
| first_indexed | 2024-03-08T07:05:08Z |
| format | Article |
| id | doaj.art-c1359cbe5cda41c98658aa425ce017da |
| institution | Directory Open Access Journal |
| issn | 2198-3844 |
| language | English |
| last_indexed | 2024-03-08T07:05:08Z |
| publishDate | 2024-02-01 |
| publisher | Wiley |
| record_format | Article |
| series | Advanced Science |
| spelling | doaj.art-c1359cbe5cda41c98658aa425ce017da2024-02-03T05:02:44ZengWileyAdvanced Science2198-38442024-02-01115n/an/a10.1002/advs.202303692CO2‐Induced Spin‐Lattice Coupling for Strong Magnetoelectric MaterialsBo Gao0Song Xu1Qun Xu2College of Materials Science & Engineering Zhengzhou University Zhengzhou 450001 P. R. ChinaInstitute of Advanced Technology Zhengzhou University Zhengzhou 450001 P. R. ChinaCollege of Materials Science & Engineering Zhengzhou University Zhengzhou 450001 P. R. ChinaAbstract The preparation of 2D magnetoelectric (ME) nanomaterials with strong ME coupling is crucial for the fast reading and writing processes in the next generation of storage devices. Herein, 2D BaTiO3 (BTO)‐CoFe2O4 (CFO) ME nanocomposites are prepared through a substrate‐free coupling strategy using supercritical CO2. Such 2D BTO‐CFO with strong coupling is built through alternating in‐plane and out‐of‐plane epitaxy stacking, leading to remarkable mutual biaxial strain effects for spin‐lattice coupling. As a results, such strain effect significantly enhances the ferroelectricity of BTO and the ferrimagnetism of CFO, where an unexceptionally high ME coupling coefficient of (325.8 mV cm−1 Oe−1) is obtained for the BTO‐CFO nanocomposites.https://doi.org/10.1002/advs.202303692biaxial strainmagnetoelectric nanomaterialsnanocompositesself‐assemblyspin‐lattice coupling |
| spellingShingle | Bo Gao Song Xu Qun Xu CO2‐Induced Spin‐Lattice Coupling for Strong Magnetoelectric Materials Advanced Science biaxial strain magnetoelectric nanomaterials nanocomposites self‐assembly spin‐lattice coupling |
| title | CO2‐Induced Spin‐Lattice Coupling for Strong Magnetoelectric Materials |
| title_full | CO2‐Induced Spin‐Lattice Coupling for Strong Magnetoelectric Materials |
| title_fullStr | CO2‐Induced Spin‐Lattice Coupling for Strong Magnetoelectric Materials |
| title_full_unstemmed | CO2‐Induced Spin‐Lattice Coupling for Strong Magnetoelectric Materials |
| title_short | CO2‐Induced Spin‐Lattice Coupling for Strong Magnetoelectric Materials |
| title_sort | co2 induced spin lattice coupling for strong magnetoelectric materials |
| topic | biaxial strain magnetoelectric nanomaterials nanocomposites self‐assembly spin‐lattice coupling |
| url | https://doi.org/10.1002/advs.202303692 |
| work_keys_str_mv | AT bogao co2inducedspinlatticecouplingforstrongmagnetoelectricmaterials AT songxu co2inducedspinlatticecouplingforstrongmagnetoelectricmaterials AT qunxu co2inducedspinlatticecouplingforstrongmagnetoelectricmaterials |