Consequences of time-reversal-symmetry breaking in the light-matter interaction: Berry curvature, quantum metric, and diabatic motion

Nonlinear optical response is well studied in the context of semiconductors and has gained a renaissance in studies of topological materials in the recent decade. So far it mainly deals with nonmagnetic materials and it is believed to root in the Berry curvature of the material band structure. In th...

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Main Authors: Tobias Holder, Daniel Kaplan, Binghai Yan
Format: Article
Language:English
Published: American Physical Society 2020-07-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.2.033100
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author Tobias Holder
Daniel Kaplan
Binghai Yan
author_facet Tobias Holder
Daniel Kaplan
Binghai Yan
author_sort Tobias Holder
collection DOAJ
description Nonlinear optical response is well studied in the context of semiconductors and has gained a renaissance in studies of topological materials in the recent decade. So far it mainly deals with nonmagnetic materials and it is believed to root in the Berry curvature of the material band structure. In this work we revisit the general formalism for the second-order optical response and focus on the consequences of the time-reversal-symmetry (T) breaking, by a diagrammatic approach. We have identified three physical mechanisms to generate a DC photocurrent, i.e., the Berry curvature, a term closely related to the quantum metric, and the diabatic motion. All three effects can be understood intuitively from the anomalous acceleration. The first two terms are respectively the antisymmetric and symmetric parts of the quantum geometric tensor. The last term is due to the dynamical antilocalization that appears from the phase accumulation between time-reversed fermion loops. Additionally, we derive the semiclassical conductivity that includes both intra- and interband effects. We find that T breaking can lead to a greatly enhanced nonlinear anomalous Hall effect that is beyond the contribution by the Berry curvature dipole.
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spelling doaj.art-c1b724ffd0684a8583f9975731d0ab222024-04-12T16:57:25ZengAmerican Physical SocietyPhysical Review Research2643-15642020-07-012303310010.1103/PhysRevResearch.2.033100Consequences of time-reversal-symmetry breaking in the light-matter interaction: Berry curvature, quantum metric, and diabatic motionTobias HolderDaniel KaplanBinghai YanNonlinear optical response is well studied in the context of semiconductors and has gained a renaissance in studies of topological materials in the recent decade. So far it mainly deals with nonmagnetic materials and it is believed to root in the Berry curvature of the material band structure. In this work we revisit the general formalism for the second-order optical response and focus on the consequences of the time-reversal-symmetry (T) breaking, by a diagrammatic approach. We have identified three physical mechanisms to generate a DC photocurrent, i.e., the Berry curvature, a term closely related to the quantum metric, and the diabatic motion. All three effects can be understood intuitively from the anomalous acceleration. The first two terms are respectively the antisymmetric and symmetric parts of the quantum geometric tensor. The last term is due to the dynamical antilocalization that appears from the phase accumulation between time-reversed fermion loops. Additionally, we derive the semiclassical conductivity that includes both intra- and interband effects. We find that T breaking can lead to a greatly enhanced nonlinear anomalous Hall effect that is beyond the contribution by the Berry curvature dipole.http://doi.org/10.1103/PhysRevResearch.2.033100
spellingShingle Tobias Holder
Daniel Kaplan
Binghai Yan
Consequences of time-reversal-symmetry breaking in the light-matter interaction: Berry curvature, quantum metric, and diabatic motion
Physical Review Research
title Consequences of time-reversal-symmetry breaking in the light-matter interaction: Berry curvature, quantum metric, and diabatic motion
title_full Consequences of time-reversal-symmetry breaking in the light-matter interaction: Berry curvature, quantum metric, and diabatic motion
title_fullStr Consequences of time-reversal-symmetry breaking in the light-matter interaction: Berry curvature, quantum metric, and diabatic motion
title_full_unstemmed Consequences of time-reversal-symmetry breaking in the light-matter interaction: Berry curvature, quantum metric, and diabatic motion
title_short Consequences of time-reversal-symmetry breaking in the light-matter interaction: Berry curvature, quantum metric, and diabatic motion
title_sort consequences of time reversal symmetry breaking in the light matter interaction berry curvature quantum metric and diabatic motion
url http://doi.org/10.1103/PhysRevResearch.2.033100
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