Efficient low-power photon upconversion in core/shell heterostructured semiconductor nanowires
Photon energy upconversion, i.e. the conversion of several low-energy photons to a photon of higher energy, offers significant potential for nano-optoelectronics and nanophotonics applications. The primary challenge is to achieve high upconversion efficiency and a broad device performance range, ena...
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Format: | Article |
Language: | English |
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EDP Sciences
2023-01-01
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Series: | EPJ Web of Conferences |
Online Access: | https://www.epj-conferences.org/articles/epjconf/pdf/2023/13/epjconf_eosam2023_05022.pdf |
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author | Jansson Mattias Ishikawa Fumitaro Chen Weimin M. Buyanova Irina A. |
author_facet | Jansson Mattias Ishikawa Fumitaro Chen Weimin M. Buyanova Irina A. |
author_sort | Jansson Mattias |
collection | DOAJ |
description | Photon energy upconversion, i.e. the conversion of several low-energy photons to a photon of higher energy, offers significant potential for nano-optoelectronics and nanophotonics applications. The primary challenge is to achieve high upconversion efficiency and a broad device performance range, enabling effective upconversion even at low excitation power. This study demonstrates that core/shell semiconductor nanowire heterostructures can exhibit upconversion efficiencies exceeding what was previously reported for semiconductor nanostructures even at a low excitation power of 100 mW/cm2, by a two-photon absorption process through conduction band states of the narrow-bandgap nanowire shell region. By engineering the electric-field distribution of the excitation light inside the NWs, upconversion efficiency can be further improved by eight times. This work showcases the effectiveness of the proposed approach in achieving efficient photon upconversion using core/shell NW heterostructures, resulting in some of the highest upconversion efficiencies reported in semiconductor nanostructures. Additionally, it offers design guidelines for enhancing energy upconversion efficiency. |
first_indexed | 2024-03-11T12:14:06Z |
format | Article |
id | doaj.art-c1bfbdbc97b64491b7ea167c8b584078 |
institution | Directory Open Access Journal |
issn | 2100-014X |
language | English |
last_indexed | 2024-03-11T12:14:06Z |
publishDate | 2023-01-01 |
publisher | EDP Sciences |
record_format | Article |
series | EPJ Web of Conferences |
spelling | doaj.art-c1bfbdbc97b64491b7ea167c8b5840782023-11-07T10:20:48ZengEDP SciencesEPJ Web of Conferences2100-014X2023-01-012870502210.1051/epjconf/202328705022epjconf_eosam2023_05022Efficient low-power photon upconversion in core/shell heterostructured semiconductor nanowiresJansson Mattias0Ishikawa Fumitaro1Chen Weimin M.2Buyanova Irina A.3Department of Physics, Chemistry and Biology, Linköping UniversityResearch center for integrated quantum electronics, Hokkaido UniversityResearch center for integrated quantum electronics, Hokkaido UniversityDepartment of Physics, Chemistry and Biology, Linköping UniversityPhoton energy upconversion, i.e. the conversion of several low-energy photons to a photon of higher energy, offers significant potential for nano-optoelectronics and nanophotonics applications. The primary challenge is to achieve high upconversion efficiency and a broad device performance range, enabling effective upconversion even at low excitation power. This study demonstrates that core/shell semiconductor nanowire heterostructures can exhibit upconversion efficiencies exceeding what was previously reported for semiconductor nanostructures even at a low excitation power of 100 mW/cm2, by a two-photon absorption process through conduction band states of the narrow-bandgap nanowire shell region. By engineering the electric-field distribution of the excitation light inside the NWs, upconversion efficiency can be further improved by eight times. This work showcases the effectiveness of the proposed approach in achieving efficient photon upconversion using core/shell NW heterostructures, resulting in some of the highest upconversion efficiencies reported in semiconductor nanostructures. Additionally, it offers design guidelines for enhancing energy upconversion efficiency.https://www.epj-conferences.org/articles/epjconf/pdf/2023/13/epjconf_eosam2023_05022.pdf |
spellingShingle | Jansson Mattias Ishikawa Fumitaro Chen Weimin M. Buyanova Irina A. Efficient low-power photon upconversion in core/shell heterostructured semiconductor nanowires EPJ Web of Conferences |
title | Efficient low-power photon upconversion in core/shell heterostructured semiconductor nanowires |
title_full | Efficient low-power photon upconversion in core/shell heterostructured semiconductor nanowires |
title_fullStr | Efficient low-power photon upconversion in core/shell heterostructured semiconductor nanowires |
title_full_unstemmed | Efficient low-power photon upconversion in core/shell heterostructured semiconductor nanowires |
title_short | Efficient low-power photon upconversion in core/shell heterostructured semiconductor nanowires |
title_sort | efficient low power photon upconversion in core shell heterostructured semiconductor nanowires |
url | https://www.epj-conferences.org/articles/epjconf/pdf/2023/13/epjconf_eosam2023_05022.pdf |
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