Effects of additives and electrolytic treatment to remove tritium from contaminated water

As a method for separating tritiated water from radioactively contaminated water, an additive was mixed into the contaminated water and their treatments of agitation/circulation and electrolytic was considered to improve of the separation efficiency. Carbide powder and ore (silica stone) powder were...

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Main Authors: Shizutoshi Ando, Takashi Komatsuzaki, Mitsukiyo Okada, Noriaki Kataoka
Format: Article
Language:English
Published: Elsevier 2023-06-01
Series:Heliyon
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2405844023042391
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author Shizutoshi Ando
Takashi Komatsuzaki
Mitsukiyo Okada
Noriaki Kataoka
author_facet Shizutoshi Ando
Takashi Komatsuzaki
Mitsukiyo Okada
Noriaki Kataoka
author_sort Shizutoshi Ando
collection DOAJ
description As a method for separating tritiated water from radioactively contaminated water, an additive was mixed into the contaminated water and their treatments of agitation/circulation and electrolytic was considered to improve of the separation efficiency. Carbide powder and ore (silica stone) powder were used as additives. The radioactivity concentration of the tritium-contaminated water (tritiated water; HTO) was 366 Bq/mL before treatment, however it obtained 333 Bq/mL and decreasing rate of 9.02%, and a high separation efficiency after treatment. Furthermore, in the reproducibility experiments (five times) using high content of HTO, the average HTO/H2O separation efficiency was obtained about 5.59% indicating good reproducibility. The agitation/circulation treatment process was dissociated and ionized HTO, and was prepared colloidal particles by OT− and 3T+. In the electrolytic treatment process, the colloidal particles in HTO were deposited on the both electrodes applied DC voltage, and was efficiently removed tritium. These treatment processes using additives were found to be useful for removal of tritium.
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spelling doaj.art-c1f095c9eff94313a42060f139b6dec42023-06-14T04:33:49ZengElsevierHeliyon2405-84402023-06-0196e17031Effects of additives and electrolytic treatment to remove tritium from contaminated waterShizutoshi Ando0Takashi Komatsuzaki1Mitsukiyo Okada2Noriaki Kataoka3Department of Electrical Engineering, Tokyo University of Science, 6-3-1 Niijuku, Katsushika-ku, Tokyo, 125-8585, Japan; Corresponding author.Gabriel Co., Ltd., 4-5-10 Nishi-shinjuku, Shinjuku-ku, Tokyo, 160-0023, JapanGabriel Co., Ltd., 4-5-10 Nishi-shinjuku, Shinjuku-ku, Tokyo, 160-0023, JapanResearch and Development Department, Tokyo Metropolitan Industrial Technology Research Institute, 2-4-10 Aomi, Koutou-ku, Tokyo, 135-0064, JapanAs a method for separating tritiated water from radioactively contaminated water, an additive was mixed into the contaminated water and their treatments of agitation/circulation and electrolytic was considered to improve of the separation efficiency. Carbide powder and ore (silica stone) powder were used as additives. The radioactivity concentration of the tritium-contaminated water (tritiated water; HTO) was 366 Bq/mL before treatment, however it obtained 333 Bq/mL and decreasing rate of 9.02%, and a high separation efficiency after treatment. Furthermore, in the reproducibility experiments (five times) using high content of HTO, the average HTO/H2O separation efficiency was obtained about 5.59% indicating good reproducibility. The agitation/circulation treatment process was dissociated and ionized HTO, and was prepared colloidal particles by OT− and 3T+. In the electrolytic treatment process, the colloidal particles in HTO were deposited on the both electrodes applied DC voltage, and was efficiently removed tritium. These treatment processes using additives were found to be useful for removal of tritium.http://www.sciencedirect.com/science/article/pii/S2405844023042391Radioactive contamination waterTritiated water (HTO)Electrolytic treatmentCarbide powderSilica stoneTritium recovery
spellingShingle Shizutoshi Ando
Takashi Komatsuzaki
Mitsukiyo Okada
Noriaki Kataoka
Effects of additives and electrolytic treatment to remove tritium from contaminated water
Heliyon
Radioactive contamination water
Tritiated water (HTO)
Electrolytic treatment
Carbide powder
Silica stone
Tritium recovery
title Effects of additives and electrolytic treatment to remove tritium from contaminated water
title_full Effects of additives and electrolytic treatment to remove tritium from contaminated water
title_fullStr Effects of additives and electrolytic treatment to remove tritium from contaminated water
title_full_unstemmed Effects of additives and electrolytic treatment to remove tritium from contaminated water
title_short Effects of additives and electrolytic treatment to remove tritium from contaminated water
title_sort effects of additives and electrolytic treatment to remove tritium from contaminated water
topic Radioactive contamination water
Tritiated water (HTO)
Electrolytic treatment
Carbide powder
Silica stone
Tritium recovery
url http://www.sciencedirect.com/science/article/pii/S2405844023042391
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AT mitsukiyookada effectsofadditivesandelectrolytictreatmenttoremovetritiumfromcontaminatedwater
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