Shape Evolution of Indium Sulfide Heterostructures via Carbon Nanotube Scrambling: Towards Reliable Sustainability and Mitigating Leakage Current in Supercapacitors
For sustainable energy storage devices with long-term endurance, exploring novel electrode materials can be a realistic focus in the areas of robust structures, surface area control, high channel conductivity, and others. A composite of a hierarchical series of single-walled carbon nanotubes (SWNTs)...
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MDPI AG
2023-02-01
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| author | Niraj Kumar Dhananjay Mishra Seungyeob Kim Krishnaiah Mokurala Rajneesh Kumar Mishra Junyoung Song Sung Hun Jin |
| author_facet | Niraj Kumar Dhananjay Mishra Seungyeob Kim Krishnaiah Mokurala Rajneesh Kumar Mishra Junyoung Song Sung Hun Jin |
| author_sort | Niraj Kumar |
| collection | DOAJ |
| description | For sustainable energy storage devices with long-term endurance, exploring novel electrode materials can be a realistic focus in the areas of robust structures, surface area control, high channel conductivity, and others. A composite of a hierarchical series of single-walled carbon nanotubes (SWNTs) with In<sub>2</sub>S<sub>3</sub> was synthesized by applying a simple one-step solvothermal method. A SWNT scaffold yields a good conductive pathway, leading to the improved electron transportation and catalytic behaviors. This promotes the robust formation of materials and their enhancement in surface activity and specific capacitance. Herein, the nucleated nanocomposites based on SWNT-mediated In<sub>2</sub>S<sub>3</sub> improve the specific capacitance (1268 F·g<sup>−1</sup> at 10 mVs<sup>−1</sup>) to a remarkable 92.4% of its capacitance even after 10,000 cycles, and furthermore, the robust cocoon-like structure of INS5 (5 mL SWNT doped in In<sub>2</sub>S<sub>3</sub>) shows an excellent 97.8% of cyclic retention (10,000 cycles). As a conceptual demonstration of system integration, the as-fabricated symmetric supercapacitor (SSC) device is successfully integrated into the Bluetooth/photoplethysmography (BLE/PPG) module for a wireless sensor network. These findings, through indium sulfides with SWNT scrambling, are expected to contribute to the next-generation solid-state-supercapacitor (SSC)-integrated module in the wireless health monitoring system. |
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| format | Article |
| id | doaj.art-c487e8320a1e438097828f9f04ac3591 |
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| issn | 2076-3417 |
| language | English |
| last_indexed | 2024-03-11T07:32:12Z |
| publishDate | 2023-02-01 |
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| series | Applied Sciences |
| spelling | doaj.art-c487e8320a1e438097828f9f04ac35912023-11-17T07:17:22ZengMDPI AGApplied Sciences2076-34172023-02-01135295810.3390/app13052958Shape Evolution of Indium Sulfide Heterostructures via Carbon Nanotube Scrambling: Towards Reliable Sustainability and Mitigating Leakage Current in SupercapacitorsNiraj Kumar0Dhananjay Mishra1Seungyeob Kim2Krishnaiah Mokurala3Rajneesh Kumar Mishra4Junyoung Song5Sung Hun Jin6Department of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Physics, Yeungnam University, Gyeongsan 38541, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaFor sustainable energy storage devices with long-term endurance, exploring novel electrode materials can be a realistic focus in the areas of robust structures, surface area control, high channel conductivity, and others. A composite of a hierarchical series of single-walled carbon nanotubes (SWNTs) with In<sub>2</sub>S<sub>3</sub> was synthesized by applying a simple one-step solvothermal method. A SWNT scaffold yields a good conductive pathway, leading to the improved electron transportation and catalytic behaviors. This promotes the robust formation of materials and their enhancement in surface activity and specific capacitance. Herein, the nucleated nanocomposites based on SWNT-mediated In<sub>2</sub>S<sub>3</sub> improve the specific capacitance (1268 F·g<sup>−1</sup> at 10 mVs<sup>−1</sup>) to a remarkable 92.4% of its capacitance even after 10,000 cycles, and furthermore, the robust cocoon-like structure of INS5 (5 mL SWNT doped in In<sub>2</sub>S<sub>3</sub>) shows an excellent 97.8% of cyclic retention (10,000 cycles). As a conceptual demonstration of system integration, the as-fabricated symmetric supercapacitor (SSC) device is successfully integrated into the Bluetooth/photoplethysmography (BLE/PPG) module for a wireless sensor network. These findings, through indium sulfides with SWNT scrambling, are expected to contribute to the next-generation solid-state-supercapacitor (SSC)-integrated module in the wireless health monitoring system.https://www.mdpi.com/2076-3417/13/5/2958supercapacitorsInS-SWNT heterostructurewireless power transmissionmitigation leakage currentwireless power transmissionhealth monitoring system |
| spellingShingle | Niraj Kumar Dhananjay Mishra Seungyeob Kim Krishnaiah Mokurala Rajneesh Kumar Mishra Junyoung Song Sung Hun Jin Shape Evolution of Indium Sulfide Heterostructures via Carbon Nanotube Scrambling: Towards Reliable Sustainability and Mitigating Leakage Current in Supercapacitors Applied Sciences supercapacitors InS-SWNT heterostructure wireless power transmission mitigation leakage current wireless power transmission health monitoring system |
| title | Shape Evolution of Indium Sulfide Heterostructures via Carbon Nanotube Scrambling: Towards Reliable Sustainability and Mitigating Leakage Current in Supercapacitors |
| title_full | Shape Evolution of Indium Sulfide Heterostructures via Carbon Nanotube Scrambling: Towards Reliable Sustainability and Mitigating Leakage Current in Supercapacitors |
| title_fullStr | Shape Evolution of Indium Sulfide Heterostructures via Carbon Nanotube Scrambling: Towards Reliable Sustainability and Mitigating Leakage Current in Supercapacitors |
| title_full_unstemmed | Shape Evolution of Indium Sulfide Heterostructures via Carbon Nanotube Scrambling: Towards Reliable Sustainability and Mitigating Leakage Current in Supercapacitors |
| title_short | Shape Evolution of Indium Sulfide Heterostructures via Carbon Nanotube Scrambling: Towards Reliable Sustainability and Mitigating Leakage Current in Supercapacitors |
| title_sort | shape evolution of indium sulfide heterostructures via carbon nanotube scrambling towards reliable sustainability and mitigating leakage current in supercapacitors |
| topic | supercapacitors InS-SWNT heterostructure wireless power transmission mitigation leakage current wireless power transmission health monitoring system |
| url | https://www.mdpi.com/2076-3417/13/5/2958 |
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