Electric control of spin transitions at the atomic scale

Abstract Electric control of spins has been a longstanding goal in the field of solid state physics due to the potential for increased efficiency in information processing. This efficiency can be optimized by transferring spintronics to the atomic scale. We present electric control of spin resonance...

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Main Authors: Piotr Kot, Maneesha Ismail, Robert Drost, Janis Siebrecht, Haonan Huang, Christian R. Ast
Format: Article
Language:English
Published: Nature Portfolio 2023-10-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-023-42287-2
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author Piotr Kot
Maneesha Ismail
Robert Drost
Janis Siebrecht
Haonan Huang
Christian R. Ast
author_facet Piotr Kot
Maneesha Ismail
Robert Drost
Janis Siebrecht
Haonan Huang
Christian R. Ast
author_sort Piotr Kot
collection DOAJ
description Abstract Electric control of spins has been a longstanding goal in the field of solid state physics due to the potential for increased efficiency in information processing. This efficiency can be optimized by transferring spintronics to the atomic scale. We present electric control of spin resonance transitions in single TiH molecules by employing electron spin resonance scanning tunneling microscopy (ESR-STM). We find strong bias voltage dependent shifts in the ESR signal of about ten times its line width. We attribute this to the electric field in the tunnel junction, which induces a displacement of the spin system changing the g-factor and the effective magnetic field of the tip. We demonstrate direct electric control of the spin transitions in coupled TiH dimers. Our findings open up new avenues for fast coherent control of coupled spin systems and expands on the understanding of spin electric coupling.
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spelling doaj.art-c4ba6fb27ac34ddf9d8ea038f5612ad32023-11-20T09:57:06ZengNature PortfolioNature Communications2041-17232023-10-011411710.1038/s41467-023-42287-2Electric control of spin transitions at the atomic scalePiotr Kot0Maneesha Ismail1Robert Drost2Janis Siebrecht3Haonan Huang4Christian R. Ast5Max-Planck-Institut für FestkörperforschungMax-Planck-Institut für FestkörperforschungMax-Planck-Institut für FestkörperforschungMax-Planck-Institut für FestkörperforschungMax-Planck-Institut für FestkörperforschungMax-Planck-Institut für FestkörperforschungAbstract Electric control of spins has been a longstanding goal in the field of solid state physics due to the potential for increased efficiency in information processing. This efficiency can be optimized by transferring spintronics to the atomic scale. We present electric control of spin resonance transitions in single TiH molecules by employing electron spin resonance scanning tunneling microscopy (ESR-STM). We find strong bias voltage dependent shifts in the ESR signal of about ten times its line width. We attribute this to the electric field in the tunnel junction, which induces a displacement of the spin system changing the g-factor and the effective magnetic field of the tip. We demonstrate direct electric control of the spin transitions in coupled TiH dimers. Our findings open up new avenues for fast coherent control of coupled spin systems and expands on the understanding of spin electric coupling.https://doi.org/10.1038/s41467-023-42287-2
spellingShingle Piotr Kot
Maneesha Ismail
Robert Drost
Janis Siebrecht
Haonan Huang
Christian R. Ast
Electric control of spin transitions at the atomic scale
Nature Communications
title Electric control of spin transitions at the atomic scale
title_full Electric control of spin transitions at the atomic scale
title_fullStr Electric control of spin transitions at the atomic scale
title_full_unstemmed Electric control of spin transitions at the atomic scale
title_short Electric control of spin transitions at the atomic scale
title_sort electric control of spin transitions at the atomic scale
url https://doi.org/10.1038/s41467-023-42287-2
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