Identifying the seeding signature in cloud particles from hydrometeor residuals

<p>Cloud seeding experiments for modifying clouds and precipitation have been underway for nearly a century; yet practically all the attempts to link precipitation enhancement or suppression to the presence of seeding materials within clouds remain elusive. In 2019, the Cloud–Aerosol Interacti...

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Main Authors: M. Konwar, B. Werden, E. C. Fortner, S. Bera, M. Varghese, S. Chowdhuri, K. Hibert, P. Croteau, J. Jayne, M. Canagaratna, N. Malap, S. Jayakumar, S. A. Dixit, P. Murugavel, D. Axisa, D. Baumgardner, P. F. DeCarlo, D. R. Worsnop, T. Prabhakaran
Format: Article
Language:English
Published: Copernicus Publications 2024-04-01
Series:Atmospheric Measurement Techniques
Online Access:https://amt.copernicus.org/articles/17/2387/2024/amt-17-2387-2024.pdf
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author M. Konwar
B. Werden
B. Werden
E. C. Fortner
S. Bera
M. Varghese
S. Chowdhuri
S. Chowdhuri
K. Hibert
P. Croteau
J. Jayne
M. Canagaratna
N. Malap
S. Jayakumar
S. A. Dixit
P. Murugavel
D. Axisa
D. Baumgardner
P. F. DeCarlo
D. R. Worsnop
T. Prabhakaran
author_facet M. Konwar
B. Werden
B. Werden
E. C. Fortner
S. Bera
M. Varghese
S. Chowdhuri
S. Chowdhuri
K. Hibert
P. Croteau
J. Jayne
M. Canagaratna
N. Malap
S. Jayakumar
S. A. Dixit
P. Murugavel
D. Axisa
D. Baumgardner
P. F. DeCarlo
D. R. Worsnop
T. Prabhakaran
author_sort M. Konwar
collection DOAJ
description <p>Cloud seeding experiments for modifying clouds and precipitation have been underway for nearly a century; yet practically all the attempts to link precipitation enhancement or suppression to the presence of seeding materials within clouds remain elusive. In 2019, the Cloud–Aerosol Interaction and Precipitation Enhancement Experiment (CAIPEEX) investigated residuals of cloud hydrometeors in seeded and non-seeded clouds with an airborne mini aerosol mass spectrometer (mAMS). The mAMS was utilized in conjunction with a counterflow virtual impactor (CVI) inlet with a cutoff diameter size of approximately 7 <span class="inline-formula">µ</span>m. The evaporated cloud droplets from the CVI inlet as cloud residuals were evaluated through the mAMS. The chlorine (Cl) associated with hygroscopic materials, i.e. calcium chloride (CaCl<span class="inline-formula"><sub>2</sub></span>) and potassium (K), which serve as the oxidizing agents in the flares, is found in relatively higher concentrations in the seeded clouds compared to the non-seeded clouds. In convective clouds, Cl and K as cloud residuals were found even at a vertical distance of 2.25 km from the cloud base. Major findings from the seeding impact are an increase in the number concentration of small (<span class="inline-formula">&lt;</span> 20 <span class="inline-formula">µ</span>m) droplets and an indication of raindrop formation at 2.25 km above the cloud base. It is demonstrated that the seed particle signature can be traced inside clouds along with the microphysical impacts.</p>
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spelling doaj.art-c6550a1926664ae08de962dd52885cf22024-04-19T14:11:06ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482024-04-01172387240010.5194/amt-17-2387-2024Identifying the seeding signature in cloud particles from hydrometeor residualsM. Konwar0B. Werden1B. Werden2E. C. Fortner3S. Bera4M. Varghese5S. Chowdhuri6S. Chowdhuri7K. Hibert8P. Croteau9J. Jayne10M. Canagaratna11N. Malap12S. Jayakumar13S. A. Dixit14P. Murugavel15D. Axisa16D. Baumgardner17P. F. DeCarlo18D. R. Worsnop19T. Prabhakaran20Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, 411008, IndiaAerodyne Research Inc., Billerica, MA 01821, USAnow at: Department of Environmental Health and Engineering, Johns Hopkins University, Baltimore, MD 21218, USAAerodyne Research Inc., Billerica, MA 01821, USAIndian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, 411008, IndiaIndian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, 411008, IndiaIndian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, 411008, Indianow at: Department of Civil and Environmental Engineering, University of California, Irvine, CA 92697-2700, USAWeather Modification Inc., Fargo, ND 58102, USAAerodyne Research Inc., Billerica, MA 01821, USAAerodyne Research Inc., Billerica, MA 01821, USAAerodyne Research Inc., Billerica, MA 01821, USAIndian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, 411008, IndiaIndian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, 411008, IndiaIndian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, 411008, IndiaIndian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, 411008, IndiaCenter for Western Weather and Water Extremes, Scripps Institution of Oceanography, La Jolla, CA 92037, USADroplet Measurement Technologies, LLC, Longmont, CO 80503, USADepartment of Environmental Health and Engineering, Johns Hopkins University, Baltimore, MD 21218, USAAerodyne Research Inc., Billerica, MA 01821, USAIndian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, 411008, India<p>Cloud seeding experiments for modifying clouds and precipitation have been underway for nearly a century; yet practically all the attempts to link precipitation enhancement or suppression to the presence of seeding materials within clouds remain elusive. In 2019, the Cloud–Aerosol Interaction and Precipitation Enhancement Experiment (CAIPEEX) investigated residuals of cloud hydrometeors in seeded and non-seeded clouds with an airborne mini aerosol mass spectrometer (mAMS). The mAMS was utilized in conjunction with a counterflow virtual impactor (CVI) inlet with a cutoff diameter size of approximately 7 <span class="inline-formula">µ</span>m. The evaporated cloud droplets from the CVI inlet as cloud residuals were evaluated through the mAMS. The chlorine (Cl) associated with hygroscopic materials, i.e. calcium chloride (CaCl<span class="inline-formula"><sub>2</sub></span>) and potassium (K), which serve as the oxidizing agents in the flares, is found in relatively higher concentrations in the seeded clouds compared to the non-seeded clouds. In convective clouds, Cl and K as cloud residuals were found even at a vertical distance of 2.25 km from the cloud base. Major findings from the seeding impact are an increase in the number concentration of small (<span class="inline-formula">&lt;</span> 20 <span class="inline-formula">µ</span>m) droplets and an indication of raindrop formation at 2.25 km above the cloud base. It is demonstrated that the seed particle signature can be traced inside clouds along with the microphysical impacts.</p>https://amt.copernicus.org/articles/17/2387/2024/amt-17-2387-2024.pdf
spellingShingle M. Konwar
B. Werden
B. Werden
E. C. Fortner
S. Bera
M. Varghese
S. Chowdhuri
S. Chowdhuri
K. Hibert
P. Croteau
J. Jayne
M. Canagaratna
N. Malap
S. Jayakumar
S. A. Dixit
P. Murugavel
D. Axisa
D. Baumgardner
P. F. DeCarlo
D. R. Worsnop
T. Prabhakaran
Identifying the seeding signature in cloud particles from hydrometeor residuals
Atmospheric Measurement Techniques
title Identifying the seeding signature in cloud particles from hydrometeor residuals
title_full Identifying the seeding signature in cloud particles from hydrometeor residuals
title_fullStr Identifying the seeding signature in cloud particles from hydrometeor residuals
title_full_unstemmed Identifying the seeding signature in cloud particles from hydrometeor residuals
title_short Identifying the seeding signature in cloud particles from hydrometeor residuals
title_sort identifying the seeding signature in cloud particles from hydrometeor residuals
url https://amt.copernicus.org/articles/17/2387/2024/amt-17-2387-2024.pdf
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