Fully Phase-Locked Fiber Dual Comb Enables Accurate Frequency and Phase Detection in Multidimensional Coherent Spectroscopy
High-resolution optical multidimensional coherent spectroscopy (MDCS) requires frequency-stable laser sources and high-resolution heterodyne spectra. Fully phase-locked dual-comb spectroscopy (DCS) enables the achievement of high resolution, high accuracy, broad bandwidth, and a rapid multi-heterody...
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| Format: | Article |
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MDPI AG
2024-01-01
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| Series: | Photonics |
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| Online Access: | https://www.mdpi.com/2304-6732/11/2/120 |
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| author | Shiping Xiong Zejiang Deng Zhong Zuo Jiayi Pan Zilin Zhao Gehui Xie Wenxue Li |
| author_facet | Shiping Xiong Zejiang Deng Zhong Zuo Jiayi Pan Zilin Zhao Gehui Xie Wenxue Li |
| author_sort | Shiping Xiong |
| collection | DOAJ |
| description | High-resolution optical multidimensional coherent spectroscopy (MDCS) requires frequency-stable laser sources and high-resolution heterodyne spectra. Fully phase-locked dual-comb spectroscopy (DCS) enables the achievement of high resolution, high accuracy, broad bandwidth, and a rapid multi-heterodyne spectrum, which results in the DCS’s potential to replace the spectrometer and phase detection system in MDCS. We verified the phase measurement capability of the MDCS system based on fully phase-locked fiber DCS by studying phase-sensitive photon echoes and double-quantum processes. The accurate phase and frequency of linear and nonlinear signals were obtained simultaneously using a single detector without subsequent frequency drift correction. Subsequently, the acquisition of longtime quantum beat signals demonstrates the high phase coherence between excitation pulses. Additionally, the two-dimensional coherent spectrum (2DCS) with high signal-to-noise-ratio and 100 MHz resolution was obtained via the MDCS system based on fully phase-locked fiber DCS. These results exhibit that fully phase-locked fiber DCS is an effective method for high-resolution 2DCS measurement, which facilitates further research on cold atoms, higher-order nonlinear spectra, and molecular fingerprint vibrational spectroscopy. |
| first_indexed | 2024-03-07T22:17:22Z |
| format | Article |
| id | doaj.art-c7f03f54358745288b009f962e368628 |
| institution | Directory Open Access Journal |
| issn | 2304-6732 |
| language | English |
| last_indexed | 2024-03-07T22:17:22Z |
| publishDate | 2024-01-01 |
| publisher | MDPI AG |
| record_format | Article |
| series | Photonics |
| spelling | doaj.art-c7f03f54358745288b009f962e3686282024-02-23T15:31:36ZengMDPI AGPhotonics2304-67322024-01-0111212010.3390/photonics11020120Fully Phase-Locked Fiber Dual Comb Enables Accurate Frequency and Phase Detection in Multidimensional Coherent SpectroscopyShiping Xiong0Zejiang Deng1Zhong Zuo2Jiayi Pan3Zilin Zhao4Gehui Xie5Wenxue Li6State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, ChinaState Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, ChinaState Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, ChinaState Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, ChinaState Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, ChinaState Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, ChinaState Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, ChinaHigh-resolution optical multidimensional coherent spectroscopy (MDCS) requires frequency-stable laser sources and high-resolution heterodyne spectra. Fully phase-locked dual-comb spectroscopy (DCS) enables the achievement of high resolution, high accuracy, broad bandwidth, and a rapid multi-heterodyne spectrum, which results in the DCS’s potential to replace the spectrometer and phase detection system in MDCS. We verified the phase measurement capability of the MDCS system based on fully phase-locked fiber DCS by studying phase-sensitive photon echoes and double-quantum processes. The accurate phase and frequency of linear and nonlinear signals were obtained simultaneously using a single detector without subsequent frequency drift correction. Subsequently, the acquisition of longtime quantum beat signals demonstrates the high phase coherence between excitation pulses. Additionally, the two-dimensional coherent spectrum (2DCS) with high signal-to-noise-ratio and 100 MHz resolution was obtained via the MDCS system based on fully phase-locked fiber DCS. These results exhibit that fully phase-locked fiber DCS is an effective method for high-resolution 2DCS measurement, which facilitates further research on cold atoms, higher-order nonlinear spectra, and molecular fingerprint vibrational spectroscopy.https://www.mdpi.com/2304-6732/11/2/120optical frequency combatomic coherent spectrumfour wave maxing |
| spellingShingle | Shiping Xiong Zejiang Deng Zhong Zuo Jiayi Pan Zilin Zhao Gehui Xie Wenxue Li Fully Phase-Locked Fiber Dual Comb Enables Accurate Frequency and Phase Detection in Multidimensional Coherent Spectroscopy Photonics optical frequency comb atomic coherent spectrum four wave maxing |
| title | Fully Phase-Locked Fiber Dual Comb Enables Accurate Frequency and Phase Detection in Multidimensional Coherent Spectroscopy |
| title_full | Fully Phase-Locked Fiber Dual Comb Enables Accurate Frequency and Phase Detection in Multidimensional Coherent Spectroscopy |
| title_fullStr | Fully Phase-Locked Fiber Dual Comb Enables Accurate Frequency and Phase Detection in Multidimensional Coherent Spectroscopy |
| title_full_unstemmed | Fully Phase-Locked Fiber Dual Comb Enables Accurate Frequency and Phase Detection in Multidimensional Coherent Spectroscopy |
| title_short | Fully Phase-Locked Fiber Dual Comb Enables Accurate Frequency and Phase Detection in Multidimensional Coherent Spectroscopy |
| title_sort | fully phase locked fiber dual comb enables accurate frequency and phase detection in multidimensional coherent spectroscopy |
| topic | optical frequency comb atomic coherent spectrum four wave maxing |
| url | https://www.mdpi.com/2304-6732/11/2/120 |
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